Hollow Fiber Membrane Composition for High Flux and Strength

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Solution Overview

Problem

Conventional methods for producing hollow fiber porous membranes result in products with low porosity, poor hydrophilicity, and low water flux, often requiring high spinning temperatures and large amounts of organic solvents, which increase production costs and environmental concerns.

Innovation Solution

A composition comprising a polymer matrix, an organic mixed solution, and a water-soluble substance, where the organic mixed solution is stable at the melting temperature of the polymer matrix, promoting microphase separation and porosity, and a low molecular weight water-soluble particle or polymer, allowing for melt spinning at a controlled temperature with easy washing, resulting in high-strength and high-flux membranes.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If conventional methods use hard elastic polymers like PP and PE to produce hollow fiber porous membranes, then the membranes have good mechanical strength, but they exhibit low porosity, poor hydrophilicity, and low water flux

Engineering Contradiction:
Improvemechanical strengthVSAvoidporosity and water flux
Core Design Contradiction:
StrengthVSQuantity of substance

Solution Approach 1:

The invention uses composite materials by combining PVDF polymer matrix with water-soluble pore-forming agents (PVA, PEG, or starch). This composite approach allows the membrane to simultaneously achieve mechanical strength from PVDF and high porosity/water flux from the water-soluble additives that create interconnected pore structures after dissolution.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The invention employs porous materials by incorporating water-soluble pore-forming agents (PVA, PEG, or starch) that dissolve during the membrane formation process, creating permanent porous structures. These porous structures significantly increase porosity and water flux while maintaining mechanical integrity through the PVDF matrix.

Inventive Principle:
Principle #31Porous materials

2Quantity of substance

If a polymeric pore forming agent is used with a surfactant and liquid insoluble to the polymer, then the membrane can achieve permeable micropores, but organic solvents like isopropyl alcohol and ethanol must be used for washing, increasing production cost and causing secondary pollution

Engineering Contradiction:
Improvepermeable microporesVSAvoidproduction cost and secondary pollution
Core Design Contradiction:
Quantity of substanceVSObject-generated harmful factors

Solution Approach 1:

The invention converts the harmful effect of using organic solvents into a benefit by selecting water-soluble pore-forming agents (PVA, PEG, or starch) that can be removed using only water for washing. This eliminates the need for expensive and environmentally harmful organic solvents like isopropyl alcohol and ethanol, reducing both production costs and secondary pollution while maintaining permeable micropore structures.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

3Ease of manufacture

If water-soluble polymers like polyoxyethylene and PVDF are mixed with a diluent, then the mixture can be melted, but the compatibility difference and viscosity difference at spinning temperature make it very difficult to form a uniform porous structure

Engineering Contradiction:
Improvemelt processingVSAvoiduniform porous structure
Core Design Contradiction:
Ease of manufactureVSManufacturing precision

Solution Approach 1:

The invention applies parameter changes by carefully controlling the composition ratios of PVDF to water-soluble additives (PVA, PEG, or starch) within specific ranges (95:5 to 80:20). This parameter optimization, combined with controlling the spinning temperature and cooling rate, ensures uniform phase separation and formation of homogeneous porous structures despite the inherent viscosity differences between components.

Inventive Principle:
Principle #35Parameter changes

4Ease of manufacture

If conventional methods require high spinning temperatures (60°C or more higher than the melting point of the resin), then the polymer can be melted and extruded, but the organic liquid used is a poor solvent at room temperature, worsening spinnability and requiring large amounts that increase cost

Engineering Contradiction:
Improvemelt extrusionVSAvoidspinnability and production cost
Core Design Contradiction:
Ease of manufactureVSDevice complexity

Solution Approach 1:

The invention uses water as an intermediary solvent that serves multiple functions: it acts as a good solvent for the water-soluble pore-forming agents (PVA, PEG, or starch) at spinning temperature, enables proper phase separation, and allows for easy washing without requiring large amounts of organic liquids. This eliminates the need for high spinning temperatures and poor solvents, improving spinnability and reducing costs.

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method achieves high-strength and large-flux hollow fiber membranes with reduced production costs and environmental impact, featuring a simple and cost-effective process suitable for industrialization.

Implementation Method 1

promoting microphase separation and porosity

Methodology Applied
Scientific EffectMicrophase separation:

Implementation Method 2

melt spinning at a controlled temperature

Methodology Applied
Scientific EffectMelting: Melting

Implementation Method 3

easy washing

Methodology Applied
Scientific EffectDissolution: Solvation

Data Source

PatentUS9095819B2Composition for preparation of hollow fiber porous membrane and preparation method using the same
Publication Date: 2015.08.04 TIANJIN POLYTECHNIC UNIV

AI summary

A composition for preparation of a hollow fiber porous membrane including 40-60 wt. % a polymer matrix, 20-30 wt. % an organic mixed solution, and 20-40 wt. % a water-soluble substance. The polymer matrix is a polymer capable of dissolving in an organic solvent and melt processing. The organic mixed solution is a mixture comprising 60-90 wt. % a first liquid soluble to the polymer matrix and 10-40 wt. % a second liquid insoluble to the polymer matrix. The water-soluble substance is a water-soluble polymer, a low molecular weight water-soluble particle, or a mixture thereof. A method for producing the hollow fiber porous membrane using the composition including a) preparing the organic mixed solution, b) mixing the components of the composition, c) applying melt spinning, d) drawing, and e) washing. The hollow fiber membrane has high strength, large flux, and low cost.