HVPE III-N Crystal Growth Hydrogen Concentration Control

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Solution Overview

Problem

Conventional methods for producing III-N semiconductor materials face challenges in achieving high crystallinity and layer thickness homogeneity due to difficulties in controlling gas flow profiles and hydrogen concentration during vapor phase epitaxy, leading to suboptimal crystal quality and efficiency.

Innovation Solution

A method is developed where the hydrogen concentration is independently adjusted on the substrate surface, allowing for flexible control of the gas flow profile, decoupling it from the reactor's flow profile, using a mixture of hydrogen, nitrogen, and argon to optimize crystallinity and layer thickness homogeneity by compensating for hydrogen's influence on the flow profile.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional gas phase epitaxy methods are used to produce III-N semiconductor materials, then the production process can be carried out, but the crystal quality and layer thickness homogeneity are suboptimal due to inability to independently control hydrogen concentration and gas flow profile

Engineering Contradiction:
Improvelayer thickness homogeneityVSAvoidcontrol system complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent divides the gas delivery system into separate channels: one for hydrogen and one for nitrogen. This segmentation allows independent control of hydrogen concentration and gas flow profile, enabling precise control of both crystallinity and layer thickness homogeneity without requiring complex coupled control systems.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent independently adjusts hydrogen concentration and gas flow profile as separate controllable parameters. By changing these parameters independently through separate delivery channels, the process achieves optimal crystal quality and layer uniformity without the trade-offs inherent in conventional single-channel systems.

Inventive Principle:
Principle #35Parameter changes

2Reliability

If hydrogen concentration is increased to improve crystallinity, then crystal quality improves, but the gas flow profile is disrupted leading to poor layer thickness homogeneity

Engineering Contradiction:
ImprovecrystallinityVSAvoidlayer thickness homogeneity
Core Design Contradiction:
ReliabilityVSManufacturing precision

Solution Approach 1:

By separating hydrogen and nitrogen delivery into independent channels, the patent allows hydrogen concentration to be increased for improved crystallinity without disrupting the gas flow profile. The nitrogen channel compensates for flow changes, maintaining layer thickness homogeneity even at higher hydrogen concentrations.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent enables independent variation of hydrogen concentration and gas flow profile parameters. This allows optimization of crystallinity through hydrogen concentration adjustment while simultaneously maintaining layer thickness homogeneity through separate flow profile control, eliminating the trade-off between these two quality metrics.

Inventive Principle:
Principle #35Parameter changes

3Manufacturing precision

If gas flow profile is optimized for layer thickness homogeneity, then manufacturing precision improves, but hydrogen concentration control is compromised leading to reduced crystallinity

Engineering Contradiction:
Improvelayer thickness homogeneityVSAvoidcrystallinity
Core Design Contradiction:
Manufacturing precisionVSReliability

Solution Approach 1:

The patent's segmented gas delivery system allows the nitrogen channel to optimize gas flow profile for layer thickness homogeneity while the hydrogen channel independently maintains optimal hydrogen concentration for crystallinity. This segmentation resolves the conflict between these two competing optimization goals.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

By treating hydrogen concentration and gas flow profile as independently controllable parameters through separate delivery channels, the patent allows simultaneous optimization of both layer thickness homogeneity and crystallinity, eliminating the compromise required in conventional single-channel systems.

Inventive Principle:
Principle #35Parameter changes

4Ease of manufacture

If conventional HVPE method is used with foreign substrates, then substrate availability improves, but crystal quality deteriorates due to lattice mismatch

Engineering Contradiction:
Improvesubstrate availabilityVSAvoidcrystal quality
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent employs optimized gas phase epitaxy parameters including controlled hydrogen concentration and gas flow profile to achieve high crystal quality on foreign substrates. This parameter optimization reduces the impact of lattice mismatch, enabling production of高质量 crystals on readily available foreign substrate materials.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach results in III-N crystals with enhanced crystallinity and layer thickness homogeneity, with standard deviations in rocking curve mappings and micro-Raman measurements indicating improved crystal quality and homogeneity, specifically achieving less than 10% standard deviation in layer thickness homogeneity and exceptional crystallinity.

Implementation Method 1

A flow profile in the form of local mass flow rates is formed in a mixture of carrier gases, wherein the mixture can carry one or more reaction gases towards a substrate

Methodology Applied
Scientific EffectGas flow: Convection

Implementation Method 2

A concentration of hydrogen at the surface of the substrate, which is important for the reaction and deposition of the reaction gases, is thereby established independently of the flow profile formed in the reactor

Methodology Applied
Scientific EffectDiffusion: Diffusion

Implementation Method 3

Method for the production of a compound semiconductor material by means of gas phase epitaxy

Methodology Applied
Scientific EffectChemical vapor deposition: Chemical Vapour Deposition

Implementation Method 4

production of a compound semiconductor material by means of gas phase epitaxy

Methodology Applied
Scientific EffectEpitaxy: Epitaxy

Data Source

PatentEP2129815B1Method for the production of a compound semiconductor material by means of gas phase epitaxy
Publication Date: 2020.05.13 FREIBERGER COMPOUND MATERIALS GMBH
  • EP2129815B1 patent drawingFigure 1
  • EP2129815B1 patent drawingFigure 2~3
  • EP2129815B1 patent drawingFigure 4

AI summary

The invention relates to the production of a compound semiconductor material, preferably a III-N bulk crystal, or a III-N layer, by means of hydride gas phase epitaxy (HVPE) in a reactor, in which a flow profile represented by local mass flow rates is formed in the reactor in a mixture of carrier gases. The mixture can include one or more reaction gases in the direction toward a substrate. For this purpose, a concentration of hydrogen critical for the reaction and precipitation of the reaction gases is adjusted on the surface of the substrate independently from the flow profile formed in the reactor.