Hybrid Catalyst Pressure Control for Fischer-Tropsch Activity

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Solution Overview

Problem

Conventional hybrid catalysts used in converting carbon-containing feed streams to light hydrocarbons have a short lifetime, leading to costly and time-consuming regeneration cycles, as they quickly deactivate during the conversion process.

Innovation Solution

Increasing the pressure within the reaction zone containing a hybrid catalyst comprising a methanol synthesis component and a solid microporous acid material, such as Cu, Zn, Cr, and Al-based catalysts with molecular sieves, while maintaining a constant temperature, to enhance catalyst activity and extend its operational life.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If conventional hybrid catalysts are used to convert carbon-containing feed streams to light hydrocarbons, then the conversion process can proceed, but the catalyst quickly deactivates leading to short operational lifetime

Engineering Contradiction:
Improvecatalyst activityVSAvoidcatalyst lifetime
Core Design Contradiction:
ProductivityVSDuration of action of stationary object

Solution Approach 1:

The patent applies parameter changes by increasing the pressure within the reaction zone during the conversion process. This pressure increase compensates for catalyst deactivation and maintains catalyst activity without requiring temperature increases, thereby extending catalyst operational lifetime while preserving productivity

Inventive Principle:
Principle #35Parameter changes

2Productivity

If temperature is increased to compensate for catalyst activity loss, then catalyst activity can be maintained, but this approach was previously thought necessary and may have drawbacks

Engineering Contradiction:
Improvecatalyst activityVSAvoidreaction temperature
Core Design Contradiction:
ProductivityVSTemperature

Solution Approach 1:

The patent changes the pressure parameter instead of temperature to compensate for catalyst deactivation. By increasing pressure within the reaction zone, the system maintains catalyst activity and productivity without requiring temperature increases, offering an alternative parameter adjustment strategy

Inventive Principle:
Principle #35Parameter changes

3Duration of action of stationary object

If pressure is increased within the reaction zone, then catalyst activity is maintained and lifetime extended, but this requires pressure control mechanisms

Engineering Contradiction:
Improvecatalyst lifetimeVSAvoidpressure control system
Core Design Contradiction:
Duration of action of stationary objectVSDevice complexity

Solution Approach 1:

The patent utilizes pressure as the controlling parameter to extend catalyst lifetime. While pressure control systems are required, this approach avoids temperature increases and provides a controlled method to maintain catalyst activity over extended periods

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach effectively maintains the activity of the hybrid catalyst, ensuring a higher percentage yield of C2 to C5 hydrocarbons over a longer period without the need for simultaneous temperature increases, which were previously thought to be necessary for compensating activity loss.

Implementation Method 1

contacting the feed stream to a hybrid catalyst positioned in the reaction zone, wherein the hybrid catalyst comprises a methanol synthesis component and a solid microporous acid material

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 2

increasing a pressure within the reaction zone during the contacting of the feed stream to the hybrid catalyst from the initial reactor pressure to a final reactor pressure

Methodology Applied
Scientific EffectPressure increase effect: Pressure Increase

Data Source

PatentEP3577096B1Processes for improving the activity of hybrid catalysts for fischer-tropsch reactions
Publication Date: 2022.01.05 DOW GLOBAL TECHNOLOGIES LLC
  • EP3577096B1 patent drawingFigure 1
  • EP3577096B1 patent drawingFigure 2

AI summary

A process for converting a feed stream to C2 to C5 hydrocarbons includes introducing a feed stream of hydrogen and at least one carbon-containing component selected from CO, CO2, and mixtures thereof into a reaction zone at an initial reactor pressure and an initial reactor temperature. The feed stream is contacted to a hybrid catalyst positioned in the reaction zone, and the hybrid catalyst includes a methanol synthesis component and a solid microporous acid material. The pressure within the reaction zone is increased during the contacting of the feed stream to the hybrid catalyst from the initial reactor pressure to a final reactor pressure. A temperature within the reaction zone at any time during the contacting of the feed stream to the hybrid catalyst is within ± 20° C of the initial reactor temperature.