Hybrid Polymer Dots With Silica Networks for Stable Bioimaging

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Solution Overview

Problem

Conventional organic dye molecules used in fluorescence microscopy and biosensors face limitations such as low absorptivity and poor photostability, hindering the development of high-sensitivity imaging techniques and high-throughput assays, and traditional chromophoric polymer dots suffer from instability and aggregation in biological buffers.

Innovation Solution

Development of organic-inorganic hybrid polymer dots comprising a semiconducting chromophoric polymer and an inorganic network that form an interpenetrated network, which are functionalized for bioconjugation and stabilized to prevent aggregation and enhance photostability.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional organic dye molecules are used as probes, then fluorescence imaging and biosensing can be performed, but low absorptivity and poor photostability limit sensitivity and reliability

Engineering Contradiction:
ImprovephotostabilityVSAvoidabsorptivity
Core Design Contradiction:
ReliabilityVSQuantity of substance

Solution Approach 1:

The patent creates hybrid polymer dots by combining organic chromophoric polymers with inorganic silica networks. This composite structure merges the high absorptivity and tunable fluorescence of organic dyes with the photostability and chemical inertness of inorganic materials, resolving the contradiction between absorptivity and photostability

Inventive Principle:
Principle #40Composite materials

2Adaptability or versatility

If traditional chromophoric polymer dots are functionalized for bioconjugation, then bioimaging applications are enabled, but polymer dot swelling, instability, and aggregation occur in biological buffer solutions

Engineering Contradiction:
Improvebioconjugation capabilityVSAvoidcolloidal stability
Core Design Contradiction:
Adaptability or versatilityVSStability of the object's composition

Solution Approach 1:

The inorganic silica network provides structural rigidity and colloidal stability to the hybrid polymer dots, preventing the swelling and aggregation that plague traditional organic polymer dots in aqueous biological buffers, while still allowing bioconjugation functionality

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The hybrid structure creates a protective inorganic shell around the organic chromophoric core, maintaining stability in biological environments while preserving the functional properties needed for bioconjugation and imaging

Inventive Principle:
Principle #30Flexible shells and thin films

3Illumination intensity

If traditional chromophoric polymer dots are used, then fluorescence imaging is possible, but aggregation in biological media reduces measurement precision

Engineering Contradiction:
Improvefluorescence brightnessVSAvoidimaging accuracy
Core Design Contradiction:
Illumination intensityVSMeasurement precision

Solution Approach 1:

The hybrid organic-inorganic structure prevents aggregation through the stabilizing inorganic silica network, maintaining uniform dispersion in biological media and ensuring consistent fluorescence signal for accurate imaging measurements

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The hybrid polymer dots exhibit improved fluorescence brightness, photostability, and colloidal stability, allowing for robust and compact particles that maintain performance in biological media without swelling or aggregation, thus advancing imaging and detection techniques.

Implementation Method 1

Traditional chromophoric polymer dots have been studied for imaging and detection techniques

Methodology Applied
Scientific EffectFluorescence: Fluorescence

Implementation Method 2

intrinsic limitations of these conventional dyes such as low absorptivity

Methodology Applied
Scientific EffectAbsorption: Absorption (EM radiation)

Implementation Method 3

an inorganic network that is covalently bonded to the semiconducting chromophoric polymer

Methodology Applied
Scientific EffectCovalent bonding: Chemical Bonding

Data Source

PatentEP3988631B1Polymer-silica hybrid pdots
Publication Date: 2023.11.22 UNIV OF WASHINGTON
  • EP3988631B1 patent drawingFigure 1
  • EP3988631B1 patent drawingFigure 2
  • EP3988631B1 patent drawingFigure 3

AI summary

The present disclosure provides organic-inorganic hybrid polymer particles, which have desirable surface chemistry and optical properties that make them particularly suitable for biological and optical applications. The present disclosure also provides methods of making organic-inorganic hybrid polymer particles. The present disclosure also provides methods of using the organic-inorganic hybrid polymer particles for biological and optical applications.