Hydrocracker Recycle Stream Solvent Deasphalting for Polycyclic Aromatic Removal

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Solution Overview

Problem

The hydrocracking process faces issues with the buildup of polycyclic aromatic hydrocarbons in the heavy oil recycle stream, leading to catalyst deactivation, reduced conversion yields, and equipment fouling, particularly when processing heavy and aromatic feedstocks under high severity conditions.

Innovation Solution

Integrating a solvent deasphalting unit into the hydrocracking process to separate and remove heavy poly-aromatic hydrocarbons from the heavy oil recycle stream, with the deasphalted paraffinic oil being recycled back to the hydrocracker reactor, while controlling the weight ratio of the solvent deasphalting stream to the recycle stream to maintain optimal polycyclic aromatic concentrations.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If high severity hydrocracker reactor conditions are used to achieve high conversion of heavy feedstock, then conversion yield is improved, but heavy polycyclic aromatic compounds accumulate in the heavy oil recycle stream causing catalyst deactivation and equipment fouling

Engineering Contradiction:
Improveconversion yieldVSAvoidheavy polycyclic aromatic buildup
Core Design Contradiction:
ProductivityVSObject-generated harmful factors

Solution Approach 1:

The patent extracts and removes heavy polycyclic aromatic compounds from the heavy oil recycle stream using a solvent deasphalting unit. The solvent deasphalting unit selectively separates these harmful compounds from the recycle stream, preventing their accumulation and subsequent harmful effects on catalyst and equipment while maintaining high conversion yields.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent introduces a solvent deasphalting unit as an intermediary component between the hydrocracker reactor and the fractionator. This intermediary unit processes the heavy oil recycle stream to remove polycyclic aromatics before recycling, acting as a mediator that eliminates the harmful buildup problem without interfering with the main hydrocracking conversion process.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Productivity

If heavy oil recycle rate is increased to achieve desired conversion of heavy feedstock, then conversion is improved, but the accumulation rate of heavy polycyclic aromatics in the recycle stream increases

Engineering Contradiction:
ImproveconversionVSAvoidheavy polycyclic aromatic concentration
Core Design Contradiction:
ProductivityVSQuantity of substance

Solution Approach 1:

The solvent deasphalting unit continuously extracts and removes heavy polycyclic aromatic compounds from the heavy oil recycle stream. This extraction process prevents the accumulation that would otherwise occur with high recycle rates, allowing the system to maintain high conversion while controlling polycyclic aromatic concentration through selective removal.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent changes the composition parameter of the heavy oil recycle stream by removing polycyclic aromatic compounds through solvent deasphalting. This parameter change (reducing PCA concentration) allows the system to operate at high recycle rates for improved conversion without suffering from the harmful effects of polycyclic aromatic buildup.

Inventive Principle:
Principle #35Parameter changes

3Object-generated harmful factors

If solvent deasphalting is integrated to remove heavy polycyclic aromatics from the heavy oil recycle stream, then polycyclic aromatic buildup is reduced, but process complexity increases

Engineering Contradiction:
Improvepolycyclic aromatic accumulationVSAvoidprocess configuration
Core Design Contradiction:
Object-generated harmful factorsVSDevice complexity

Solution Approach 1:

The patent merges the solvent deasphalting function with the existing hydrocracking process by integrating the solvent deasphalting unit into the heavy oil recycle stream configuration. This integration combines multiple functions (hydrocracking, fractionation, and solvent deasphalting) into a unified process system, reducing overall complexity compared to separate standalone units.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The heavy oil recycle stream serves multiple functions: it provides unconverted feedstock back to the reactor for continued conversion and simultaneously serves as the feed stream for the solvent deasphalting unit. This multi-functionality reduces the need for additional separate processing lines and simplifies the overall process configuration.

Inventive Principle:
Principle #6Universality (Multi-functionality)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach effectively reduces the concentration of polycyclic aromatics in the heavy oil recycle stream, preventing catalyst deactivation and fouling, while maintaining high conversion yields and process efficiency by recycling a deasphalted paraffinic oil that is depleted of heavy polycyclic aromatic compounds.

Implementation Method 1

a second portion of the heavy oil recycle stream is passed to a solvent deasphalting unit for separating the heavy poly-aromatic hydrocarbons from the second portion of the heavy oil recycle stream

Methodology Applied
Scientific EffectSolvent deasphalting: Liquid-Liquid Extraction

Implementation Method 2

contacting in a hydrocracking reaction vessel or zone the heavy feedstock with a suitable hydrocracking catalyst under conditions of elevated temperature and pressure in the presence of hydrogen so as to yield the upgraded products

Methodology Applied
Scientific EffectHydrocracking: Chemical Bonding

Data Source

PatentEP3204473B1A hydrocracking process integrated with solvent deasphalting to reduce heavy polycyclic aromatic buildup in heavy oil hydrocracker recycle stream
Publication Date: 2020.05.06 SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ BV
  • EP3204473B1 patent drawingFigure 1

AI summary

An integrated hydrocracking and solvent deasphalting process that provides for removal from the heavy oil recycle stream heavy polycyclic aromatic compounds formed in the hydrocracking step and recycling the resulting deasphalted paraffinic oil as a feed to the hydrocracker reactor of the process for further conversion.