Hydrocracking Distillate Yield via Segmented Hydrotreatment

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Current hydrocracking processes for producing distillate products face challenges in maximizing yield while minimizing conversion to naphtha or lower boiling range products, often resulting in reduced lubricant base oil production and requiring severe processing conditions.

Innovation Solution

A multi-stage process involving hydrotreating, separation or fractionation of the effluent to remove contaminant gases, and subsequent hydrocracking with a large pore molecular sieve catalyst, which allows for milder reaction conditions and increased distillate yield by minimizing exposure of distillate boiling range products to additional hydroprocessing stages.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If severe processing conditions are used to maximize distillate yield, then distillate production increases, but conversion to naphtha and lighter products increases excessively

Engineering Contradiction:
Improvedistillate yieldVSAvoidconversion to naphtha and lighter products
Core Design Contradiction:
ProductivityVSLoss of substance

Solution Approach 1:

The hydroprocessing is divided into two distinct stages: a first hydroprocessing stage followed by a second hydroprocessing stage. This segmentation allows each stage to be optimized for different functions - the first stage handles initial conversion while the second stage completes the process, preventing excessive conversion to light products while maximizing distillate yield.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The first hydroprocessing stage performs preliminary conversion of the feedstock before the second stage. By conducting initial hydroprocessing separately, the process prepares the feed for the second stage while preventing premature over-conversion that would lead to excessive naphtha and lighter product formation.

Inventive Principle:
Principle #10Preliminary action

2Device complexity

If single-stage hydrocracking is used to produce distillate, then process complexity is reduced, but distillate yield is decreased and lubricant base oil production is reduced

Engineering Contradiction:
Improveprocess complexityVSAvoiddistillate yield
Core Design Contradiction:
Device complexityVSProductivity

Solution Approach 1:

The process is segmented into two hydroprocessing stages with distinct functions. The first stage performs initial conversion and the second stage completes the hydroprocessing, allowing each stage to be optimized for its specific role. This segmentation increases distillate yield and lubricant base oil production compared to single-stage processes.

Inventive Principle:
Principle #1Segmentation

3Quantity of substance

If extended hydroprocessing exposure is used to increase conversion, then feed conversion increases, but distillate yield decreases due to over-cracking

Engineering Contradiction:
Improvefeed conversionVSAvoiddistillate yield
Core Design Contradiction:
Quantity of substanceVSProductivity

Solution Approach 1:

The hydroprocessing is segmented into two stages where the first stage performs initial conversion and the second stage completes the process. This prevents extended exposure to hydroprocessing conditions that would cause over-cracking, thereby maintaining high distillate yield while achieving the desired level of feed conversion.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The first hydroprocessing stage performs preliminary conversion before the second stage. This preliminary action prepares the feedstock for the second stage while controlling the extent of conversion to prevent over-cracking and maintain optimal distillate yield.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach significantly enhances distillate product yield while maintaining a desired level of feed conversion, reducing the need for recycle and improving overall process efficiency, allowing for increased production of distillate boiling range products such as kerosene and diesel without excessive conversion to naphtha or lighter products.

Implementation Method 1

contacting a feedstock having a T5 boiling point of at least about 473°F (245°C) with a first hydrotreating catalyst under first effective hydrotreating conditions

Methodology Applied
Scientific EffectHydrodesulfurization:

Implementation Method 2

contacting a feedstock having a T5 boiling point of at least about 473°F (245°C) with a first hydrotreating catalyst under first effective hydrotreating conditions

Methodology Applied
Scientific EffectHydrodenitrogenation:

Implementation Method 3

performing a separation on the first hydrotreated effluent to form at least a first separated effluent portion and a first remaining effluent portion

Methodology Applied
Scientific EffectGas-liquid separation:

Implementation Method 4

fractionating the second hydrotreated effluent to form at least a hydrotreated distillate boiling range product and a second remaining effluent portion

Methodology Applied
Scientific EffectFractionation: Fractionation

Implementation Method 5

contacting the second remaining effluent portion with a hydrocracking catalyst under effective hydrocracking conditions to produce a hydrocracked effluent

Methodology Applied
Scientific EffectCatalytic cracking:

Data Source

PatentEP3077485B1Hydrocracking of gas oils with increased distillate yield
Publication Date: 2018.10.03 EXXONMOBIL TECHNOLOGY & ENGINEERING CO
  • EP3077485B1 patent drawingFigure 1
  • EP3077485B1 patent drawingFigure 2
  • EP3077485B1 patent drawingFigure 3

AI summary

Methods are provided for improving the yield of distillate products from hydroprocessing of gas oil feedstocks, such as vacuum gas oils. It has been unexpectedly found that stripping of gases or fractionation to separate out a distillate fraction during initial hydrotreatment of a feed can provide a substantial increase in distillate yield at a desired amount of feedstock conversion. The improvement in yield of distillate products can allow a desired level of conversion to be performed on a feedstock for generating lubricating base oil products while reducing or minimizing the amount of naphtha (or lower) boiling range products. Alternatively, the improvement in yield of distillate products can correspond to an improved yield during a single pass through a reaction system, so that distillate yield is increased even though a lubricant boiling range product is not generated.