Hydroformylation Reactor Distributor Plate for Olefin Conversion

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Conventional hydroformylation and hydrogenation processes face limitations in reaction efficiency due to inadequate contact between olefins and synthesis gas, leading to reduced selectivity and increased side reactions such as esterification, acetal formation, and etherification.

Innovation Solution

An apparatus comprising a hydroformylation reactor with a nozzle and distributor plate to enhance gas-liquid contact and a hydrogenation reactor with dual catalyst layers to suppress side reactions, promoting efficient production of alcohols from olefins by forming micro-bubbles and optimizing catalyst activity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If conventional stirring or circulation methods are used in hydroformylation reactor, then the reactor structure is simple and easy to operate, but the contact surface area between olefins and synthesis gas is insufficient, leading to reduced reaction efficiency

Engineering Contradiction:
Improvereaction efficiencyVSAvoidreactor structure complexity
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The invention utilizes gas-liquid phase interaction by introducing synthesis gas as gas bubbles into the liquid reaction mixture. The gas-liquid contact process enhances mass transfer and reaction efficiency without requiring complex mechanical stirring mechanisms, thereby resolving the contradiction between productivity improvement and device complexity.

Inventive Principle:
Principle #36Phase transitions

2Manufacturing precision

If longer residence time or multiple reactors in series are used to achieve satisfactory product conversion, then the required product level is achieved, but the process complexity and equipment investment increase

Engineering Contradiction:
Improveproduct conversion levelVSAvoidprocess configuration complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The invention changes the reaction parameters by optimizing gas flow rate, liquid circulation rate, and reactor temperature to achieve high conversion efficiency in a single reactor. This approach avoids the need for multiple reactors in series or extended residence times, thereby reducing process complexity while maintaining satisfactory product conversion levels.

Inventive Principle:
Principle #35Parameter changes

3Reliability

If conventional hydrogenation catalysts are used, then the catalyst structure is simple, but side reactions such as esterification, acetal formation, and etherification occur, reducing selectivity

Engineering Contradiction:
Improvereaction selectivityVSAvoidcatalyst system complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The invention employs a composite catalyst system combining nickel and copper catalysts in specific proportions. This composite catalyst structure enhances selectivity by suppressing unwanted side reactions while maintaining catalytic activity, resolving the contradiction between improving reliability and managing device complexity.

Inventive Principle:
Principle #40Composite materials

4Speed

If vapor phase hydrogenation is used to perform the reaction, then the reaction rate is fast, but esterification and other side reactions are generated, reducing selectivity

Engineering Contradiction:
Improvereaction rateVSAvoidreaction selectivity
Core Design Contradiction:
SpeedVSReliability

Solution Approach 1:

The invention changes the phase parameter from vapor phase to liquid phase hydrogenation. This parameter change slows the reaction rate slightly but dramatically improves selectivity by suppressing esterification and other side reactions, thereby resolving the contradiction between speed and reliability.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The apparatus significantly improves reaction efficiency and selectivity by increasing the contact surface area and controlling catalyst activity, resulting in enhanced production of alcohols while reducing unwanted side reactions.

Implementation Method 1

spraying olefins and a synthesis gas (CO/H2) into a solution of catalyst mixture... forming micro-bubbles

Methodology Applied
Scientific EffectBubble formation: Bubble

Implementation Method 2

a part of these gases being dispersed in the form of gas bubbles in the reaction liquid

Methodology Applied
Scientific EffectGas dispersion: Dispersion (of waves)

Implementation Method 3

a distributor plate for converting a flow of the olefins and the synthesis gas (CO/H2)

Methodology Applied
Scientific EffectFlow conversion:

Implementation Method 4

converting a flow of the olefins and the synthesis gas... enhancing gas-liquid contact

Methodology Applied
Scientific EffectConvection: Convection

Implementation Method 5

a nickel catalyst layer having a high activity... a copper catalyst layer having a low activity... producing alcohols by adding hydrogen to the recovered aldehydes

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 6

hydrogenation reactor for producing alcohols by adding hydrogen to the recovered aldehydes

Methodology Applied
Scientific EffectHydrogenation: Hydrogenation

Implementation Method 7

a circulation line for circulating the reaction mixture... continuously circulates the reaction mixture

Methodology Applied
Scientific EffectCirculation: Convection

Data Source

PatentEP2390242B1Apparatus for producing alcohols from olefins
Publication Date: 2017.06.14 LG CHEM LTD
  • EP2390242B1 patent drawingFigure 1(a)~1(b)
  • EP2390242B1 patent drawingFigure 2~3(c)
  • EP2390242B1 patent drawingFigure 4(a)~4(e)

AI summary

The present invention relates to an apparatus for producing alcohols from olefins, comprising: a hydroformylation reactor wherein aldehydes are produced from olefins; a catalyst/aldehydes separator; a hydrogenation reactor wherein the aldehydes are hydrogenated to produce alcohols; and a distillation column. The hydroformylation reactor is equipped with a distributor plate, which has a broad contact surface for providing sufficient reaction area for reactants such as olefins and synthesis gas, and allows the reaction mixture to circulate and mix sufficiently, which contribute to excellent efficiency in terms of production of aldehydes. In addition, the hydrogenation reactor suppresses sub-reactions to improve the production yield of alcohols.