Hydrophilic Polymer Layer for SPFS Sensor S/N Ratio

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Solution Overview

Problem

Conventional surface plasmon-field enhanced Fluorescence Spectrometry (SPFS) methods face challenges in achieving high sensitivity and accuracy for detecting extremely small or low concentrations of analytes due to limitations in the signal-to-noise ratio (S/N ratio) caused by enhanced nonspecific reactions and high viscosity issues with polyethylene glycol concentrations.

Innovation Solution

The implementation of a hydrophilic high molecule layer on a self-assembled monolayer (SAM) with immobilized ligands, using a moisturizer to enhance antigen-antibody reactions, and controlling the concentration and thickness of the hydrophilic high molecule layer to improve the S/N ratio without increasing viscosity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If polyethylene glycol is mixed in the liquid to improve antigen-antibody reaction, then reactivity is enhanced, but viscosity increases too much which lowers reactivity and decreases assay light emission signal

Engineering Contradiction:
Improvereactivity of antigen-antibody reactionVSAvoidviscosity increase
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent changes the concentration parameter of polyethylene glycol from high (conventional method) to specifically controlled low concentration (0.01-10%, preferably 0.1-5%). This parameter optimization resolves the contradiction by finding the optimal point where reactivity is sufficiently enhanced while viscosity remains low enough to maintain good reactivity and signal intensity.

Inventive Principle:
Principle #35Parameter changes

2Measurement precision

If antibodies and antigens are made to react under coexistence of polyethylene glycol and urea, then measurement sensitivity is improved, but S/N ratio increase is restrictive and cannot achieve high accuracy detection for extremely small amount analytes

Engineering Contradiction:
Improvemeasurement sensitivityVSAvoidS/N ratio
Core Design Contradiction:
Measurement precisionVSLoss of information

Solution Approach 1:

The patent optimizes the concentration parameter of polyethylene glycol to a specific range (0.01-10%) and removes urea from the reaction system. This parameter change resolves the contradiction by achieving both high measurement sensitivity and high S/N ratio, enabling accurate detection of extremely small amounts of analytes without the limitations of conventional methods.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach significantly enhances the reactivity of antigen-antibody reactions, stabilizes assay light emission signals, and improves the S/N ratio, enabling high sensitivity detection of analytes without the limitations of conventional methods.

Implementation Method 1

utilizing plasmon resonance which is increased to some tens of times to some hundreds of times by resonance between surface plasmon and evanescent wave which is transmitted through a metal layer when the surface of the metal layer formed on a dielectric substance is irradiated with exciting light such as laser light on the condition that total-reflection decrement is caused

Methodology Applied
Scientific EffectSurface plasmon resonance: Resonance

Implementation Method 2

evanescent wave which is transmitted through a metal layer when the surface of the metal layer formed on a dielectric substance is irradiated with exciting light such as laser light on the condition that total-reflection decrement is caused

Methodology Applied
Scientific EffectEvanescent wave transmission: Total Internal Reflection

Implementation Method 3

efficiently exciting fluorescent dyes to label analytes (analysis target material) captured in the vicinity of a metal film

Methodology Applied
Scientific EffectFluorescence: Fluorescence

Data Source

PatentEP2482073B1Assay method and kit for assay employing sensor chip for fluorescent measuring apparatus utilizing surface plasmon-field enhanced fluorescence spectrometry
Publication Date: 2017.05.31 KONICA MINOLTA INC
  • EP2482073B1 patent drawingFigure 1
  • EP2482073B1 patent drawingFigure 2
  • EP2482073B1 patent drawing

AI summary

An assay method with use of a sensor chip which includes a metal member, a self-assembled monolayer (SAM), and ligands on a support, and is configured to be used fur a fluorescence measuring apparatus with utilization of a surface plasmon-field enhanced Fluorescence Spectrometry, including the steps of: forming a hydrophilic high molecule layer on the self-assembled monolayer in the sensor chip; immobilizing the ligands at least one of in the hydrophilic high molecule layer and on the surface of the hydrophilic high molecule layer; and bringing a moisturizer in contact with the hydrophilic high molecule layer.