Indium Alloy Diffusion Barrier for Copper-Gold Electroplating

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Solution Overview

Problem

Current electroplating technologies face challenges in preventing copper diffusion into precious metal layers, particularly gold, without using toxic nickel or expensive palladium, and existing cyanide-free solutions fail to maintain a bright and shiny aspect while effectively blocking copper migration.

Innovation Solution

An electroplating method using an indium alloy as a diffusion barrier layer between a copper-based underlayer and a precious metal top layer, with an indium concentration of 0.1 to 20 g/L and a thickness of 10 to 200 nm, which prevents copper migration and maintains the brightness and thickness distribution of the electroplated product.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If nickel or palladium intermediate layers are used to prevent copper diffusion into precious metal layers, then the diffusion barrier function is improved, but the toxicity (nickel) or cost (palladium) worsens

Engineering Contradiction:
Improvediffusion barrier functionVSAvoidtoxicity and cost
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent replaces expensive palladium with a much cheaper indium-based diffusion barrier layer. The indium layer, though thin (10-200 nm), provides effective copper diffusion prevention without the high cost of palladium, embodying the principle of using cheaper materials to achieve the same protective function.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The patent changes the chemical composition parameter of the diffusion barrier layer from nickel/palladium to indium-based alloys. This parameter change eliminates the toxicity associated with nickel and the high cost of palladium, while maintaining the essential diffusion barrier function through carefully controlled indium concentration (0.1 to 20 g/L) and layer thickness.

Inventive Principle:
Principle #35Parameter changes

2Object-affected harmful factors

If cyanide-free electroplating solutions are used, then the toxicity is reduced, but the ability to prevent copper diffusion and maintain brightness deteriorates

Engineering Contradiction:
ImprovetoxicityVSAvoiddiffusion barrier function and surface quality
Core Design Contradiction:
Object-affected harmful factorsVSReliability

Solution Approach 1:

The indium-based layer acts as an intermediary between the cyanide-free plating solution and the substrate. It provides the necessary diffusion barrier function that was previously achieved by cyanide complexes, mediating between the non-toxic electrolyte and the requirement for copper diffusion prevention while maintaining surface brightness.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent uses composite indium-based alloys (indium with other metals) as the diffusion barrier layer. This composite material approach allows the system to achieve both non-toxicity (replacing cyanide) and effective copper diffusion prevention, with the indium alloy providing multiple functions simultaneously.

Inventive Principle:
Principle #40Composite materials

3Reliability

If indium alloy concentration is increased to improve diffusion barrier function, then the copper migration prevention is improved, but the thickness control and brightness distribution worsen

Engineering Contradiction:
Improvecopper migration preventionVSAvoidthickness control and brightness distribution
Core Design Contradiction:
ReliabilityVSManufacturing precision

Solution Approach 1:

The patent optimizes the indium concentration parameter within a specific range (0.1 to 20 g/L) and controls the layer thickness (10 to 200 nm) to achieve the desired balance. By carefully adjusting these parameters, the system maintains effective copper diffusion prevention while ensuring uniform brightness and precise thickness control across the electroplated surface.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The indium alloy effectively blocks copper migration into the gold layer, maintaining the aesthetic properties of the electroplated product even after thermal treatment, and is non-toxic, replacing hazardous materials like nickel and cyanide-based systems.

Implementation Method 1

providing a diffusion barrier layer which prevents the interdiffusion between the underlayer and the top layer under a precious metal top layer

Methodology Applied
Scientific EffectDiffusion barrier: Diffusion Barrier

Implementation Method 2

electroplating bath for electrochemical deposition of a novel Cu-Sn-Zn-Pd alloy

Methodology Applied
Scientific EffectElectroplating: Electroplating

Data Source

PatentEP3765658B1Electroplated products and electroplating bath for providing such products
Publication Date: 2023.06.14 COVENTYA SRL
  • EP3765658B1 patent drawingFigure 1~2
  • EP3765658B1 patent drawingFigure 3
  • EP3765658B1 patent drawingFigure 4~4b

AI summary

The present invention relates to electroplated products having a combination of layers used to provide a diffusion barrier layer under a precious metal top layer on a substrate comprising a copper based material and/or a copper based underlayer, such that the layer or combination of layers prevents or retards the migration of copper into the precious metal layer or the opposite. The diffusion barrier layer comprises indium or an indium alloy. Moreover, the present invention refers a method for preparing such an electroplated product.