Indolocarbazole Terphenyl Hosts for PHOLED Efficiency

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Solution Overview

Problem

There is a need for novel materials in the field of PHOLED devices to enhance performance metrics such as luminance efficiency, external quantum efficiency, and operating voltage.

Innovation Solution

The development of compounds with specific structures, including indolocarbazole and terphenyl building blocks, which can be used as hosts in organic light-emitting diodes (OLEDs) to improve device performance by incorporating these materials into the organic layer, enabling enhanced luminance efficiency and reduced operating voltage.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If conventional organic materials are used in OLEDs, then device fabrication is simpler and cost is lower, but luminance efficiency and external quantum efficiency are insufficient

Engineering Contradiction:
Improveluminance efficiencyVSAvoidenergy efficiency
Core Design Contradiction:
ProductivityVSLoss of energy

Solution Approach 1:

The patent modifies the molecular structure of organic emissive materials by incorporating specific heterocyclic rings (triazole, tetrazole, oxadiazole, isoxadiazole) and adjusting substituent groups to optimize HOMO-LUMO energy gaps. This changes the electronic parameters of the material to achieve higher luminance efficiency and external quantum efficiency while maintaining solution processability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates composite organic emissive materials that combine multiple functional units within a single molecular structure. These compounds integrate electron-donating groups, electron-withdrawing groups, and heterocyclic cores to achieve synergistic effects that improve both efficiency and processability simultaneously

Inventive Principle:
Principle #40Composite materials

2Productivity

If novel organic emissive materials with optimized performance are developed, then luminance efficiency and external quantum efficiency improve, but material synthesis complexity increases

Engineering Contradiction:
Improveexternal quantum efficiencyVSAvoidmaterial structure complexity
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The patent divides the organic emissive material into distinct functional segments: a core heterocyclic unit (providing structural framework), electron-donating substituents (controlling HOMO level), and electron-withdrawing substituents (controlling LUMO level). This modular approach allows systematic optimization of each segment to achieve target efficiency metrics while maintaining reasonable synthesis complexity

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent introduces specific heterocyclic rings (triazole, tetrazole, oxadiazole, isoxadiazole) at strategic positions within the molecular structure to locally enhance electron mobility and luminescence properties. These localized structural modifications provide targeted improvements in external quantum efficiency without requiring complete redesign of the entire molecular architecture

Inventive Principle:
Principle #3Local quality

3Productivity

If organic materials with tuned energy levels are used, then device performance improves, but material stability and lifetime may be compromised

Engineering Contradiction:
Improvedevice performanceVSAvoidmaterial stability
Core Design Contradiction:
ProductivityVSReliability

Solution Approach 1:

The patent employs heterocyclic rings (triazole, tetrazole, oxadiazole, isoxadiazole) as intermediary structural elements that mediate between electron-donating and electron-withdrawing groups. These intermediary units provide stable bonding frameworks that maintain molecular integrity while enabling efficient charge transport and energy transfer, thus improving device performance without sacrificing material stability

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent incorporates robust heterocyclic cores and stable aromatic substituents that provide inherent structural stability and resistance to degradation. These pre-engineered stable structural elements act as a cushion against chemical and thermal stress during device operation, preserving material reliability even as energy levels are optimized for enhanced performance

Inventive Principle:
Principle #11Beforehand cushioning (Prior cushioning)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The use of these compounds results in improved luminance efficacy, external quantum efficiency, and lower operating voltage in OLED devices, demonstrating their effectiveness in PHOLED applications.

Implementation Method 1

OLEDs make use of thin organic films that emit light when voltage is applied across the device

Methodology Applied
Scientific EffectElectroluminescence: Electroluminescence

Data Source

PatentEP4141010A1Organic electroluminescent materials and devices
Publication Date: 2023.03.01 UNIVERSAL DISPLAY CORP
  • EP4141010A1 patent drawingFigure 1
  • EP4141010A1 patent drawingFigure 2
  • EP4141010A1 patent drawing

AI summary

The present invention includes novel organic materials containing indolo[3,2-b]carbazoles and terphenyls. The compounds and materials of the present invention may be useful for PHOLED devices.