Inkjet Metallic Pattern Formation via Plasma-Treated Substrate

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Solution Overview

Problem

Existing methods for forming metallic patterns, such as those used in circuits and electrodes, face challenges with adhesion to substrates, fine line reproducibility, and conductivity, particularly due to limitations in temperature conditions and the stability of metal nano-particles and ion solutions.

Innovation Solution

A method involving an inkjet process with ink containing a nonelectric plating catalyst precursor, where the substrate undergoes plasma treatment and the ink has a pH of 9.0 to 14.0, enhancing adhesion and reproducibility by forming functional groups and improving surface energy, allowing for effective nonelectric plating.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If metallic nano-particles are used and sintered at 200-300°C, then processing steps are decreased and utilization efficiency of starting materials is improved, but complete fusing of metallic particles together is difficult and severe limitations of temperature and conditions remain to reduce electric resistance

Engineering Contradiction:
Improveprocessing stepsVSAvoidelectric resistance
Core Design Contradiction:
ProductivityVSReliability

Solution Approach 1:

The patent changes the chemical composition parameters of the ink by incorporating specific complexing agents (EDTA, DTPA, or their salts) with metal salts at controlled ratios. This chemical parameter modification enables the metal particles to fuse completely at the low sintering temperature of 200-300°C, achieving both low electric resistance (≤10 μΩ·cm) and complete particle fusion without requiring higher temperatures

Inventive Principle:
Principle #35Parameter changes

2Ease of manufacture

If metal salt with insufficient complexing agent ability is used, then a conductive pattern can be formed from solution, but reducing reaction of metal salt easily proceeds resulting in poor storage stability of solution

Engineering Contradiction:
Improveconductive pattern formationVSAvoidstorage stability
Core Design Contradiction:
Ease of manufactureVSStability of the object's composition

Solution Approach 1:

The patent introduces strong complexing agents (EDTA, DTPA, or their salts) as intermediary substances that coordinate with metal ions to form stable complexes. These complexing agents act as mediators between the metal salt and the reducing environment, preventing spontaneous reducing reactions during storage while still allowing controlled reduction during the sintering process to form conductive patterns

Inventive Principle:
Principle #24Intermediary (Mediator)

3Reliability

If inkjet method with catalyst is used to form circuit pattern followed by nonelectric plating, then adhesion and conductivity are improved, but additional layer should be provided on support reducing production efficiency

Engineering Contradiction:
ImproveadhesionVSAvoidproduction efficiency
Core Design Contradiction:
ReliabilityVSProductivity

Solution Approach 1:

The patent merges multiple functions into a single ink formulation: the ink simultaneously serves as the pattern deposition medium, the catalyst source for nonelectric plating, and the adhesion promoter. By incorporating nonelectric plating catalysts (Pd, Pt, Rh, Ir, or their compounds) along with complexing agents and surfactants in the ink, the process eliminates the need for separate additional layers while maintaining excellent adhesion and productivity

Inventive Principle:
Principle #5Merging (Combining)

4Manufacturing precision

If conventional resist method is used to form metallic pattern, then precise pattern formation is achieved, but process is manifold and consumes plenty of time with many useless points

Engineering Contradiction:
Improvepattern formation precisionVSAvoidmanufacturing time
Core Design Contradiction:
Manufacturing precisionVSLoss of time

Solution Approach 1:

The patent extracts and eliminates the unnecessary intermediate steps from the conventional resist method. Instead of coating resist, performing development, etching, and peeling, the invention directly deposits metal-containing ink that self-organizes into precise patterns through the nonelectric plating reaction, keeping only the essential pattern formation step and eliminating all wasteful intermediate processes

Inventive Principle:
Principle #2Taking out (Extraction)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method achieves excellent adhesion and fine line reproducibility with improved conductivity, reducing the complexity and energy consumption of the process while maintaining stability and efficiency.

Implementation Method 1

the surface of said substrate is constituted of ink non-absorptive resin and has been subjected to a plasma treatment

Methodology Applied
Scientific EffectPlasma treatment: Plasma

Implementation Method 2

a printing process to print a pattern portion on a substrate by means of an inkjet method utilizing ink containing a precursor of a nonelectric plating catalyst

Methodology Applied
Scientific EffectInkjet printing:

Implementation Method 3

a plating process to form a metallic pattern by nonelectric plating on said pattern portion

Methodology Applied
Scientific EffectNonelectric plating: Electroplating

Implementation Method 4

ability of a complexing agent, which coordinates to metal salt and stabilizes said metal salt

Methodology Applied
Scientific EffectComplexation: Chemical Bonding

Data Source

PatentUS8440263B2Forming method of metallic pattern and metallic pattern
Publication Date: 2013.05.14 KONICA MINOLTA IJ TECHNOLOGIES INC

AI summary

A method for forming a metallic pattern, which is provided with a printing process to print a pattern portion on a substrate by means of an inkjet method utilizing ink containing a precursor of a nonelectric plating catalyst and a plating process to form a metallic pattern by nonelectric plating on said pattern portion, wherein the surface of said substrate is constituted of ink non-absorptive resin and has been subjected to a plasma treatment, and said ink has a pH value at 25° C. of not less than 9.0.