Inkjet Recording Medium with Temperature-Dependent Gelation

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Solution Overview

Problem

The ink jet recording medium's ink receiving layer tends to color over time and lacks sufficient water resistance, especially under harsh conditions, and the existing crosslinkable systems have a short pot life due to high gelation rates at ambient temperature, leading to non-uniform mixing and characteristics.

Innovation Solution

An ink jet recording medium using an acetoacetic ester group-containing polyvinyl alcohol resin (AA-PVA-based resin) crosslinked by glyoxylates, with a coating solution containing AA-PVA-based resin, glyoxylate, and water, which exhibits a significant difference in gelation rate between ambient temperature and heating, allowing for stable storage and rapid gelling when heated.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Speed

If a crosslinking agent with high gelation rate at ambient temperature is used, then gelling occurs rapidly, but the coating solution has short pot life and cannot be uniformly mixed

Engineering Contradiction:
Improvegelation rateVSAvoidpot life
Core Design Contradiction:
SpeedVSDuration of action of moving object

Solution Approach 1:

The patent uses a modified PVA resin with keto groups that changes its gelation behavior based on temperature parameters. At ambient temperature, the gelation rate is slow allowing long pot life and uniform mixing. When heated, the gelation rate accelerates rapidly to achieve quick gelling and eliminate fluidity. This parameter-based control resolves the contradiction between rapid gelling and long pot life.

Inventive Principle:
Principle #35Parameter changes

2Quantity of substance

If the ink receiving layer is made relatively thick to improve ink absorptivity, then ink absorption increases, but drying time increases and surface defects occur

Engineering Contradiction:
Improveink absorptivityVSAvoiddrying time
Core Design Contradiction:
Quantity of substanceVSLoss of time

Solution Approach 1:

The patent applies preliminary gelling action before the drying process. By gelling the coating layer first (either at ambient temperature or under heating), the fluidity is eliminated in advance, preventing wind ripple patterns and surface defects during subsequent drying. This allows the use of thicker coating for better ink absorptivity without suffering from extended drying time penalties, as the gelling step prepares the layer for faster, defect-free drying.

Inventive Principle:
Principle #10Preliminary action

3Stability of the object's composition

If cooling is applied to gel the PVA resin with boric acid, then gelling occurs, but productivity decreases and production cost increases

Engineering Contradiction:
ImprovegellingVSAvoidproduction efficiency
Core Design Contradiction:
Stability of the object's compositionVSProductivity

Solution Approach 1:

Instead of using cooling to achieve gelling (as with boric acid crosslinking), the patent inverts the approach by using heating to accelerate gelation. The modified PVA resin with keto groups gels slowly at ambient temperature but gels rapidly when heated. This eliminates the need for cooling steps, thereby maintaining high productivity and reducing production costs while achieving the desired gelling and stability.

Inventive Principle:
Principle #13The other way round (Inversion)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution provides an ink jet recording medium with excellent coloration resistance and water resistance, long pot life of the coating solution, and enhanced uniformity, enabling efficient production with improved productivity and reduced production costs.

Implementation Method 1

an ink receiving layer containing an acetoacetic ester group-containing polyvinyl alcohol resin crosslinked by a glyoxylate

Methodology Applied
Scientific EffectCrosslinking reaction: Chemical Bonding

Implementation Method 2

the coating solution applied on a supporting base is gelled and then dried

Methodology Applied
Scientific EffectGelation: Gel

Implementation Method 3

a modified PVA resin having a keto group is used as a crosslinkable system allowing for progress of gelling at ambient temperature or under heating

Methodology Applied
Scientific EffectTemperature-dependent gelation: Gel

Implementation Method 4

drying the coating by heating to remove water

Methodology Applied
Scientific EffectEvaporation: Evaporation

Data Source

PatentEP2383124B1Method for producing inkjet recording medium
Publication Date: 2014.08.20 THE NIPPON SYNTHETIC CHEM IND CO LTD
  • EP2383124B1 patent drawingFigure 1~2
  • EP2383124B1 patent drawingFigure 3(a)~3(b)
  • EP2383124B1 patent drawing

AI summary

The present invention provides an ink jet recording medium having an ink receiving layer excellent in the coloration resistance and water resistance; and a coating solution for forming an ink receiving layer, which exhibits a large difference in the gelation rate between at ambient temperature and under heating, and is stable at ambient temperature and swiftly gelled when heated. The present invention relates to an ink jet recording medium comprising an ink receiving layer containing an acetoacetic ester group-containing polyvinyl alcohol resin crosslinked by a glyoxylate on a supporting base; and a coating solution for forming an ink receiving layer containing an acetoacetic ester group-containing polymer compound, a glyoxylate and water.