Insulating Porous Layer for Battery Separator Discharge Output

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Solution Overview

Problem

Conventional nonaqueous electrolyte secondary batteries, particularly lithium secondary batteries, face issues with insufficient discharge output characteristics due to limitations in their separator designs, which affect safety and performance.

Innovation Solution

The introduction of an insulating porous layer with specific capacitance and thickness ranges, containing fine metal oxide particles like titanium oxide and aluminum, improves the discharge output characteristic by optimizing the desolvation process of cations, thereby enhancing the battery's performance and safety.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If a porous film made of meltable material is used as separator to provide shutdown function, then safety is improved, but discharge output characteristic deteriorates

Engineering Contradiction:
ImprovesafetyVSAvoiddischarge output characteristic
Core Design Contradiction:
ReliabilityVSProductivity

Solution Approach 1:

The separator is constructed as a composite structure consisting of a porous base material layer and an insulating porous layer containing inorganic fine particles (such as alumina, silica, or titania) dispersed in a binder polymer. This composite structure combines the shutdown function of the porous base material with the ion conductivity and thermal stability of the insulating porous layer, thereby improving discharge output characteristic while maintaining safety

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The insulating porous layer is designed with controlled porosity (30-80%) and specific pore structure to facilitate ion transport while providing thermal stability. The porous structure allows efficient ion passage during normal operation, improving discharge output, while the inorganic fine particles maintain structural integrity at elevated temperatures

Inventive Principle:
Principle #31Porous materials

2Reliability

If inorganic fine particles and binder polymer are used in active layer, then shutdown function is achieved, but discharge output characteristic remains insufficient

Engineering Contradiction:
Improveshutdown functionVSAvoiddischarge output characteristic
Core Design Contradiction:
ReliabilityVSProductivity

Solution Approach 1:

The invention optimizes several key parameters of the insulating porous layer: capacitance (0.01-0.5 μF/cm²), thickness (1-20 μm), porosity (30-80%), and inorganic fine particle content (10-90 wt%). By carefully controlling these parameters, the layer achieves both adequate shutdown function and improved ion conductivity for better discharge output

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The separator structure is designed with spatial differentiation: the porous base material layer provides the shutdown function through its meltable structure, while the insulating porous layer with inorganic fine particles provides ion conductivity and thermal stability. Each layer has localized properties optimized for its specific function, resolving the contradiction between shutdown capability and discharge performance

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The implementation of the insulating porous layer with controlled capacitance and thickness improves the discharge output characteristic of nonaqueous electrolyte secondary batteries, leading to superior performance compared to conventional designs, while ensuring safety through enhanced ion management and thermal stability.

Implementation Method 1

improves the discharge output characteristic by optimizing the desolvation process of cations

Methodology Applied
Scientific EffectDesolvation:

Implementation Method 2

an insulating porous layer with specific capacitance and thickness ranges

Methodology Applied
Scientific EffectDielectric: Dielectric

Data Source

PatentUS10211442B2Nonaqueous electrolyte secondary battery insulating porous layer and nonaqueous electrolyte secondary battery laminated separator
Publication Date: 2019.02.19 SSLM

AI summary

As a nonaqueous electrolyte secondary battery insulating porous layer and nonaqueous electrolyte secondary battery laminated separator each of which allows a nonaqueous electrolyte secondary battery to have an improved discharge output characteristic, there are provided (i) a nonaqueous electrolyte secondary battery insulating porous layer containing a filler including a metal oxide and having a capacitance of not less than 0.0390 nF and not more than 0.142 nF per 19.6 mm2 and a thickness of not less than 0.1 μm and not more than 20 μm and (ii) a nonaqueous electrolyte secondary battery laminated separator including the porous layer.