Ionic Liquid Coated Catalyst for Selective Hydrogenation

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Solution Overview

Problem

Existing catalysts used in selective hydrogenation reactions, such as those for aromatic compounds and polyunsaturated compounds, suffer from high levels of undesirable by-products, particularly at high conversion rates, due to limited selectivity.

Innovation Solution

A porous heterogeneous transition metal catalyst coated with an ionic liquid is used, which enhances selectivity and allows for high conversion rates by maintaining the ionic liquid coating under reaction conditions that prevent its detachment, utilizing metals like nickel, cobalt, and palladium, and specific ionic liquids with organic cations and anions.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If conventional supported metal catalysts are used for selective hydrogenation, then the desired hydrogenation reaction is accelerated, but the proportion of undesirable by-products is high, particularly at high conversion rates

Engineering Contradiction:
Improveconversion rateVSAvoidundesirable by-products
Core Design Contradiction:
ProductivityVSObject-generated harmful factors

Solution Approach 1:

An ionic liquid coating is applied to the catalyst surface to act as an intermediary layer between the reactants and the metal catalyst. This coating selectively interacts with polyunsaturated compounds, allowing them to access the catalyst surface while blocking less reactive monounsaturated compounds, thereby improving selectivity at high conversion rates

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The ionic liquid coating changes the surface properties and local environment of the catalyst. By modifying the chemical and physical parameters at the catalyst surface, the coating enhances selectivity for specific reactions while maintaining high conversion rates through optimized reactant-catalyst interactions

Inventive Principle:
Principle #35Parameter changes

2Manufacturing precision

If the ionic liquid coating is applied to enhance selectivity, then high selectivity is achieved, but the catalyst must be subjected to specific reaction conditions to prevent the IL coating from detaching

Engineering Contradiction:
ImproveselectivityVSAvoidreaction condition constraints
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The ionic liquid coating is designed to be stable under specific reaction conditions but can be easily removed or replaced. This allows for simple regeneration of the catalyst by removing the coating and applying a fresh layer, maintaining high selectivity without complex permanent modifications to the catalyst structure

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Volume of moving object

If larger catalyst forms are used, then the catalyst can be used in various configurations, but there is significant loss in selectivity

Engineering Contradiction:
Improvecatalyst form sizeVSAvoidselectivity
Core Design Contradiction:
Volume of moving objectVSManufacturing precision

Solution Approach 1:

The catalyst employs a porous structure with controlled pore sizes that allow reactants to access internal surface areas. The ionic liquid coating is applied within these pores, ensuring that even in larger catalyst forms, the active sites remain accessible and selective through the porous architecture that maintains high surface area to volume ratio

Inventive Principle:
Principle #31Porous materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The catalyst achieves high selectivity and conversion rates in hydrogenation reactions, reducing the formation of undesirable by-products and maintaining activity, even in larger catalyst forms without significant loss in selectivity.

Implementation Method 1

A porous heterogeneous transition metal catalyst, the inner surface of which is coated with an ionic liquid

Methodology Applied
Scientific EffectCatalysis: Catalysis

Data Source

PatentEP2024088B2Porous heterogeneous catalyst coated with an ionic fluid
Publication Date: 2018.08.01 CLARIANT PRODUKTE (DEUTSCHLAND) GMBH GROUP INTELLECTUAL PROPERTY
  • EP2024088B2 patent drawingFigure 1
  • EP2024088B2 patent drawingFigure 2
  • EP2024088B2 patent drawingFigure 3

AI summary

The invention relates to a porous heterogeneous catalyst. In order to prepare a catalyst that, with relatively high selectivity, catalyzes the hydrogenation of isolated unsaturated bindings of multiple unsaturated compounds, it is recommended according to the present invention that the inner surface of the catalyst is covered with an ionic fluid.