Ionic Liquid Catalysts for Sulfur Sealant Curing Balance

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Solution Overview

Problem

Aerospace sealants require a balance between long working time and short curing time, but conventional catalysts like amine catalysts and manganese dioxide can compromise the tensile strength and elongation of the cured sealant.

Innovation Solution

The use of ionic liquid catalysts in sulfur-containing prepolymer compositions to achieve extended working time and rapid curing while maintaining the mechanical properties of the sealant.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If conventional catalysts (amine catalysts or manganese dioxide) are used to cure thiol-terminated sulfur-containing prepolymers, then the curing reaction proceeds, but the tensile strength and elongation of the cured sealant are reduced

Engineering Contradiction:
Improvecuring rateVSAvoidtensile strength and elongation
Core Design Contradiction:
ProductivityVSStrength

Solution Approach 1:

The patent changes the chemical parameters of the catalyst system by replacing conventional amine catalysts or manganese dioxide with ionic liquid catalysts. This parameter change maintains adequate curing rate while eliminating the detrimental effect on tensile strength and elongation, as ionic liquids do not compromise the mechanical properties of the cured sealant

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent employs a composite catalyst system using ionic liquids, which combine organic cations and inorganic or organic anions in a liquid state at room temperature. This composite material approach allows the catalyst to facilitate the curing reaction effectively while maintaining the integrity and mechanical properties of the final sealant product

Inventive Principle:
Principle #40Composite materials

2Loss of time

If an increased amount of catalyst is added to shorten the curing time, then the curing time is reduced, but the properties of the cured sealant are detrimentally affected

Engineering Contradiction:
Improvecuring timeVSAvoidtensile strength and elongation
Core Design Contradiction:
Loss of timeVSStrength

Solution Approach 1:

The patent changes the catalytic activity parameters by using ionic liquids with optimized cation-anion combinations. This allows achieving fast curing rates with minimal catalyst amounts, thereby avoiding the detrimental effects that would result from using higher catalyst concentrations

Inventive Principle:
Principle #35Parameter changes

3Productivity

If conventional catalysts are used to achieve fast curing, then the curing time is shortened, but the working time of the sealant is reduced

Engineering Contradiction:
Improvecuring rateVSAvoidworking time
Core Design Contradiction:
ProductivityVSDuration of action of moving object

Solution Approach 1:

The patent utilizes the dynamic properties of ionic liquids, which can be adjusted by changing the cation and anion types. This allows optimizing the catalyst activity to provide an extended working time for application while ensuring rapid curing once applied, achieving a dynamic balance between workability and curing speed

Inventive Principle:
Principle #15Dynamics

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The ionic liquid catalysts enable a balance of extended working time and rapid curing, resulting in aerospace sealants with enhanced properties such as improved tensile strength and elongation.

Implementation Method 1

Ionic liquids are used to catalyze the curing reaction of thiol-terminated sulfur-containing prepolymers

Methodology Applied
Scientific EffectCatalysis: Catalysis

Data Source

PatentEP3445499B1Ionic liquid catalyst in sulfur-containing polymer compositions
Publication Date: 2022.06.08 PRC DESOTO INTERNATIONAL INC
  • EP3445499B1 patent drawingFigure 1
  • EP3445499B1 patent drawingFigure 2
  • EP3445499B1 patent drawingFigure 3~4

AI summary

Compositions comprising thiol-terminated sulfur-containing prepolymers, curing agents reactive with the thiol-terminated sulfur-containing prepolymers, and ionic liquid catalysts, useful in aerospace sealant applications are disclosed. The use of ionic liquid catalysts provides curable sealant compositions having an extended working time and a rapid cure rate.