Ionic Polymer Bio-electrode Composition for Stable Conductivity

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Solution Overview

Problem

Current bio-electrodes face challenges in maintaining electric conductivity and biocompatibility, particularly when exposed to water or used for extended periods, due to issues with water evaporation, skin allergies, and reduced adhesion and stretchability, which affect the reliability of long-term biological signal detection.

Innovation Solution

A bio-electrode composition comprising an ionic polymer material bonded to carbon particles, specifically using salts of ammonium, lithium, sodium, and silver with fluorosulfonic acid, fluorosulfonimide, or N-carbonyl-fluorosulfonamide, combined with an adhesive resin and electro-conductive powders, to enhance both ionic and electron conductivity while preventing permeation and irritation.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If water-soluble gel containing water and electrolyte is used as bio-electrode material, then electric conductivity is improved, but water evaporation during drying process causes loss of electric conductivity

Engineering Contradiction:
Improveelectric conductivityVSAvoidwater evaporation
Core Design Contradiction:
ReliabilityVSLoss of substance

Solution Approach 1:

The patent uses an adhesive resin as an intermediary substance that binds the ionic polymer material to the carbon particles. This composite structure allows the ionic polymer to maintain its ion-conducting properties while the carbon particles provide structural stability and prevent water loss, resolving the contradiction between maintaining electric conductivity and preventing water evaporation.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent creates a composite material consisting of ionic polymer material bonded to carbon particles. This composite combines the ion-conducting properties of the polymer with the structural stability and water-retention capabilities of carbon particles, enabling the bio-electrode to maintain electric conductivity even when dried.

Inventive Principle:
Principle #40Composite materials

2Reliability

If higher-ionization-tendency metal such as copper is used to improve electric conductivity, then conductivity is enhanced, but skin allergy occurs

Engineering Contradiction:
Improveelectric conductivityVSAvoidskin allergy
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent changes the material parameter from reactive metals (copper) to ionic polymer materials that provide ionization without causing skin allergies. The ionic polymer material achieves the necessary ionization for conductivity while being biocompatible, thus resolving the contradiction between electric conductivity and skin allergy prevention.

Inventive Principle:
Principle #35Parameter changes

3Reliability

If electro-conductive polymer such as PEDOT-PSS is used to improve conductivity, then electric conductivity is enhanced, but skin allergy occurs due to strong acidity and peeling during washing

Engineering Contradiction:
Improveelectric conductivityVSAvoidskin allergy and peeling
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent changes the chemical properties of the electro-conductive material by using ionic polymer materials with appropriate ionization tendencies that do not exhibit strong acidity. This eliminates skin allergy while maintaining conductivity. Additionally, the bonding to carbon particles prevents peeling during washing by providing mechanical stability.

Inventive Principle:
Principle #35Parameter changes

4Reliability

If metal nanowire is used to improve electric conductivity with small quantities, then conductivity is enhanced, but skin allergies occur due to sharp tips and thin structure

Engineering Contradiction:
Improveelectric conductivityVSAvoidskin allergy
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent changes the physical form from thin metal nanowires with sharp tips to ionic polymer materials that can be applied as coatings. This eliminates the mechanical irritation caused by sharp tips while maintaining ionization capability for conductivity, thus preventing skin allergies.

Inventive Principle:
Principle #35Parameter changes

5Reliability

If noble metal film is used to improve electric conductivity, then conductivity is enhanced, but high impedance and high resistance to skin occur during electrical conduction

Engineering Contradiction:
Improveelectric conductivityVSAvoidhigh impedance and high resistance
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent changes the material from noble metals with low ionization tendency to ionic polymer materials that readily ionize. This enables efficient conversion of ions from skin to current, reducing impedance and resistance during electrical conduction while maintaining good electric conductivity.

Inventive Principle:
Principle #35Parameter changes

6Reliability

If ionic liquid with smaller molecular weight is used to improve electric conductivity, then conductivity is enhanced, but ionic liquid dissolves into water and is extracted by sweating, lowering conductivity and causing rough dry skin

Engineering Contradiction:
Improveelectric conductivityVSAvoidionic liquid extraction
Core Design Contradiction:
ReliabilityVSLoss of substance

Solution Approach 1:

The patent creates a composite where the ionic polymer material is bonded to carbon particles. This structure prevents the ionic material from dissolving into water or being extracted by sweating, as the carbon particle framework provides structural stability and anchors the ionic polymer in place, maintaining conductivity during perspiration.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The bio-electrode composition ensures stable and sensitive detection of biological signals over time, maintaining conductivity and biocompatibility, even when wet or dried, with improved adhesion and stretchability, thus addressing the limitations of existing technologies.

Implementation Method 1

The water-soluble gel contains sodium, potassium, or calcium as the electrolyte in a water-soluble polymer for retaining water, and converts changes of ion concentration from skin into electricity.

Methodology Applied
Scientific EffectIon-to-electricity conversion:

Implementation Method 2

By taking advantage of excellent electric conductivity, the use of metal nanowire, carbon black, carbon nanotube, and the like as electrode materials has been examined

Methodology Applied
Scientific EffectElectrical conduction: Conduction (electrical)

Data Source

PatentEP3995548A1Bio-electrode composition, bio-electrode, method for manufacturing bioelectrode, and reaction composite
Publication Date: 2022.05.11 SHIN ETSU CHEMICAL CO LTD
  • EP3995548A1 patent drawingFigure 1~2
  • EP3995548A1 patent drawingFigure 3
  • EP3995548A1 patent drawingFigure 4

AI summary

A bio-electrode composition contains (A) a reaction composite of an ionic polymer material and a carbon particle. The component (A) contains the carbon particle bonding to the polymer containing a repeating unit having a structure selected from the group consisting of salts of ammonium, lithium, sodium, potassium, and silver formed with any of fluorosulfonic acid, fluorosulfonimide, and N-carbonyl-fluorosulfonamide. Thus, the present invention provides: a bio-electrode composition capable of forming a living body contact layer for a bio-electrode which is excellent in electric conductivity and biocompatibility, light-weight, and manufacturable at low cost, and which prevents significant reduction in the electric conductivity even when wetted with water or dried; a bio-electrode including a living body contact layer formed of the bio-electrode composition; and a method for manufacturing the bio-electrode.