Isocyanate-Terminated Prepolymer Turbidity Control

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Solution Overview

Problem

Existing processes for producing polyisocyanates result in products with excessively high turbidity, limiting their use in optically demanding coating systems and finishes.

Innovation Solution

A process involving a stoichiometric excess of aliphatic or cycloaliphatic diisocyanates and polyols with high OH numbers, mixed with specific power input in the range of 0.5 kW/m3 to 40 kW/m3, to produce isocyanate-terminated prepolymers and subsequently polyisocyanates with isocyanurate and allophanate groups, ensuring turbidity levels of at most 2.0 NTU through controlled urethanization and distillative separation.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional urethanization reaction conditions are used to produce polyisocyanates, then the reaction can proceed to form higher molecular weight adducts, but the resulting products exhibit excessively high turbidity values that limit their use in optically demanding coating systems

Engineering Contradiction:
Improveoptical qualityVSAvoidturbidity
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The patent applies parameter changes by controlling the specific power input during mixing (0.5-40 kW/m³) and managing temperature profiles during the urethanization reaction. These parameter adjustments prevent formation of turbid by-products while maintaining desired polyisocyanate product characteristics, directly resolving the optical quality issue.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent replaces conventional mechanical mixing approaches with a more sophisticated control system that monitors and adjusts mixing intensity and temperature dynamically during the reaction. This substitution allows precise control over reaction conditions to eliminate turbidity without compromising product formation.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

2Quantity of substance

If high stoichiometric excess of diisocyanate is used to ensure complete reaction and high isocyanate functionality, then the polyisocyanate can achieve desired functionality ≥4, but the reaction mixture becomes more difficult to control and may produce higher turbidity

Engineering Contradiction:
Improveisocyanate functionalityVSAvoidreaction control complexity
Core Design Contradiction:
Quantity of substanceVSDevice complexity

Solution Approach 1:

The patent implements feedback control by monitoring reaction conditions (temperature, mixing intensity, conversion) and adjusting process parameters in real-time. This allows maintenance of high isocyanate functionality through controlled excess diisocyanate while preventing turbidity formation through dynamic process adjustment.

Inventive Principle:
Principle #23Feedback

Solution Approach 2:

The patent applies dynamics by making the mixing intensity and temperature profiles variable rather than constant. The specific power input is adjusted during the reaction course to optimize both high functionality achievement and turbidity prevention, transforming a static process into a dynamically controlled one.

Inventive Principle:
Principle #15Dynamics

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process effectively reduces turbidity to acceptable levels, enabling the production of turbidity-free polyisocyanates suitable for elastic coatings, improving their optical quality and reliability in coating systems.

Implementation Method 1

reacting a reaction mixture containing a stoichiometric excess of at least one aliphatic and/or cycloaliphatic diisocyanate and a polyol composition having an OH number >400

Methodology Applied
Scientific EffectUrethanization reaction: Chemical Bonding

Implementation Method 2

distillatively separating off monomeric diisocyanate from the polyisocyanate obtained in step (2)

Methodology Applied
Scientific EffectDistillation: Distillation

Implementation Method 3

the reaction mixture is mixed with a specific power input in the range from 0.5 kW/m3 to 40 kW/m3, based on the total volume of the reaction mixture

Methodology Applied
Scientific EffectMechanical mixing: Stirring

Data Source

PatentUS20240052085A1Producing Isocyanate-Terminated, Urethane Group-Containing Prepolymers
Publication Date: 2024.02.15 COVESTRO DEUTSCHLAND AG

AI summary

The invention relates to a method for producing isocyanate-terminated, urethane group-containing prepolymers, comprising reacting a reaction mixture that contains a stoichiometric excess of at least one aliphatic and/or cycloaliphatic diisocyanate and a polyol composition having an OH number >400, characterized in that the reaction mixture is mixed with a specific power input of 0.5 kW/m3 to 40 kW/m3, relative to the total volume of the reaction mixture.