Isomerization Dewaxing Catalyst for Biodiesel Cold Flow

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Solution Overview

Problem

Current methods for producing biodiesel fuels from biocomponent sources often result in blends with unfavorable cold flow properties and high cloud points, making them unsuitable for commercial use, particularly in extreme cold climates.

Innovation Solution

A method involving mixing a biocomponent feed with a mineral feedstock and contacting it with an isomerization/dewaxing catalyst, specifically a molecular sieve like ZSM-48 and a Group VIII metal, under effective isomerization/dewaxing conditions to achieve a cloud point of -20°C or less, while removing oxygen content and improving cetane values.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If biodiesel is blended with conventional diesel to meet diesel specifications, then fuel composition requirements are satisfied, but cloud point increases making the blend unsuitable for cold climates

Engineering Contradiction:
Improvediesel specification complianceVSAvoidcloud point
Core Design Contradiction:
Manufacturing precisionVSTemperature

Solution Approach 1:

The patent applies parameter changes by modifying the molecular structure of biodiesel components through isomerization. The process converts normal paraffins to iso-paraffins and branched structures, which have lower cloud points while maintaining diesel specification compliance. This chemical transformation changes the physical properties of the fuel without altering its fundamental composition.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite fuel system by combining conventional diesel with isomerized biodiesel components. The isomerization process produces a mixture of hydrocarbon isomers that blend with conventional diesel to create a composite fuel with improved cold flow properties while maintaining the benefits of biodiesel blending.

Inventive Principle:
Principle #40Composite materials

2Temperature

If isomerization catalysts are used to reduce cloud point, then cold flow properties improve, but n-paraffin content remains high limiting further cloud point reduction

Engineering Contradiction:
Improvecloud pointVSAvoidn-paraffin content
Core Design Contradiction:
TemperatureVSQuantity of substance

Solution Approach 1:

The patent merges two previously separate processes into a single integrated isomerization-dewaxing step. By combining the isomerization catalyst (for converting normal paraffins to iso-paraffins) with a dewaxing catalyst (for removing n-paraffins), the process achieves both cloud point reduction and n-paraffin removal simultaneously, breaking the limitation that prevented further cloud point improvement.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The patent employs a composite catalyst system containing both isomerization and dewaxing functional components. This composite catalyst enables dual functionality: isomerizing normal paraffins to improve cold flow while simultaneously dewaxing to remove n-paraffins that would otherwise limit cloud point reduction, achieving synergistic effects greater than either catalyst alone.

Inventive Principle:
Principle #40Composite materials

3Device complexity

If single step hydroprocessing is used to perform hydrodeoxygenation and hydroisomerization, then process complexity is reduced, but cloud points remain above -20°C

Engineering Contradiction:
Improveprocess stepsVSAvoidcloud point
Core Design Contradiction:
Device complexityVSTemperature

Solution Approach 1:

The patent merges hydrodeoxygenation and hydroisomerization-dewaxing into a single integrated process step. By using a multifunctional catalyst that performs deoxygenation, isomerization, and dewaxing simultaneously, the process achieves cloud points below -20°C without requiring multiple sequential processing steps, thus reducing overall process complexity while improving performance.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The patent employs a composite catalyst material that integrates multiple functional components: metal sites for hydrodeoxygenation, acid sites for isomerization, and dewaxing capabilities. This composite catalyst enables all necessary reactions to occur in one step, achieving superior cloud point reduction while maintaining process simplicity.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method effectively reduces cloud points and improves cold flow properties of biodiesel fuels, making them suitable for commercial use and enhancing cetane values, thus addressing the limitations of existing biodiesel production techniques.

Implementation Method 1

contacting the combined feedstock with an isomerization/dewaxing catalyst... under effective isomerization/dewaxing conditions including a temperature of at least about 350°C and being effective to remove about 99% of the oxygen content

Methodology Applied
Scientific EffectHydrodeoxygenation: Hydrogenation

Implementation Method 2

contacting the combined feedstock with an isomerization/dewaxing catalyst... under effective isomerization/dewaxing conditions

Methodology Applied
Scientific EffectIsomerization: Catalysis

Implementation Method 3

contacting the combined feedstock with an isomerization/dewaxing catalyst... to produce an isomerized/dewaxed product having a cloud point of about -20°C or less

Methodology Applied
Scientific EffectDewaxing: Adsorption

Data Source

PatentEP2545144B1Hydroprocessing of diesel range biomolecules
Publication Date: 2021.05.19 EXXONMOBIL TECHNOLOGY & ENGINEERING CO
  • EP2545144B1 patent drawingFigure 1
  • EP2545144B1 patent drawingFigure 2
  • EP2545144B1 patent drawingFigure 3a

AI summary

Non-hydrotreated biocomponent feeds can be mixed with mineral feeds and processed under catalytic isomerization/dewaxing conditions. The catalytic isomerization/dewaxing conditions can be selected to advantageously also substantially deoxygenate the mixed feed. Diesel fuel products with improved cold flow properties can be produced.