Indium Tin Oxide Powder Crystallinity and Surface Area Control

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Existing indium tin oxide (ITO) powders face a trade-off between high crystallinity and large specific surface area, which are necessary for forming transparent and conductive films, as increasing the specific surface area often decreases crystallinity and conductivity.

Innovation Solution

A surface-modified ITO powder with a specific surface area of 40 m²/g or more, a navy blue color tone, and a half-width of the (222) plane peak of 0.6° or less is produced through a method involving coprecipitation of indium tin hydroxide using a tin (Sn2+) compound and indium trichloride, followed by drying and calcining under specific conditions, including a nitrogen atmosphere with alcohol, to enhance crystallinity and conductivity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Illumination intensity

If the primary particle size of ITO powder is decreased to increase specific surface area, then transparency is improved, but crystallinity decreases and conductivity deteriorates

Engineering Contradiction:
ImprovetransparencyVSAvoidcrystallinity
Core Design Contradiction:
Illumination intensityVSStability of the object's composition

Solution Approach 1:

The patent applies parameter changes by carefully controlling the pH value (4.0-9.3) and temperature (5-80°C) during coprecipitation, as well as the calcination conditions, to achieve optimal crystallinity in fine ITO powder particles while maintaining high specific surface area

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses coprecipitation as a preliminary action to form ITO powder with controlled particle size and morphology before calcination, ensuring that the desired crystallinity and specific surface area are achieved in the final product

Inventive Principle:
Principle #10Preliminary action

2Illumination intensity

If the primary particle size of ITO powder is decreased to increase specific surface area, then transparency is improved, but conductivity deteriorates

Engineering Contradiction:
ImprovetransparencyVSAvoidconductivity
Core Design Contradiction:
Illumination intensityVSReliability

Solution Approach 1:

The patent changes process parameters including pH (4.0-9.3), temperature (5-80°C), and calcination conditions to produce ITO powder with optimal electrical conductivity while maintaining fine particle size for transparency

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The coprecipitation process serves as a preliminary action that pre-forms the ITO powder with controlled particle characteristics, ensuring both transparency and conductivity are achieved after calcination

Inventive Principle:
Principle #10Preliminary action

3Ease of manufacture

If existing ITO powder production methods are used, then manufacturing is simpler, but the resulting powder does not achieve both high specific surface area and high crystallinity

Engineering Contradiction:
Improvemanufacturing simplicityVSAvoidcrystallinity and specific surface area control
Core Design Contradiction:
Ease of manufactureVSManufacturing precision

Solution Approach 1:

The patent modifies production parameters by using coprecipitation with controlled pH (4.0-9.3) and temperature (5-80°C), followed by calcination under specific conditions, to achieve precise control over crystallinity and specific surface area while maintaining practical manufacturability

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The resulting ITO powder achieves high transparency and conductivity, with surface resistivity of 20,000 Ω/sq. or less and low Δ transmittance, making it suitable for transparent conductive films and infrared ray shielding applications.

Implementation Method 1

a process of coprecipitating an indium tin hydroxide by using a tin (Sn 2+) compound and indium trichloride

Methodology Applied
Scientific EffectCoprecipitation: Coprecipitation

Implementation Method 2

drying and calcining the indium tin hydroxide under specific conditions, including a nitrogen atmosphere with alcohol

Methodology Applied
Scientific EffectCalcining:

Implementation Method 3

the indium tin hydroxide is calcined to produce the indium tin oxide powder in which a surface is modified

Methodology Applied
Scientific EffectSurface modification:

Data Source

PatentEP2599751B1Indium tin oxide powder, production method therefor, and a transparent conductive composition
Publication Date: 2018.10.03 MITSUBISHI MATERIALS CORP
  • EP2599751B1 patent drawingFigure 1
  • EP2599751B1 patent drawingFigure 2
  • EP2599751B1 patent drawingFigure 3

AI summary

One aspect of an indium tin oxide powder has a specific surface area of 55 m2/g or more, wherein a color tone is from bright yellow to a color of persimmons or a half-width in the peak of (222) plane is 0.6° or less on an X-ray diffraction chart. Another aspect of the indium tin oxide powder has a modified surface, wherein a specific surface area is 40 m2/g or more, a half-width in the peak of (222) plane is 0.6° or less on an X-ray diffraction chart, and a color tone is navy blue (L is 30 or less in a Lab colorimetric system). A method for producing the indium tin oxide powder includes: coprecipitating an indium tin hydroxide by using a tin (Sn2+) compound under conditions in which pH is 4.0 to 9.3, and a temperature of a liquid is 5°C or higher, wherein the indium tin hydroxide has a color tone from bright yellow to a color of persimmons in a dried powder state; and drying and calcining the indium tin hydroxide.