Keratin Lanthionization Under Mild Conditions to Preserve Elasticity

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Solution Overview

Problem

Existing methods for treating keratin-containing materials, such as wool, using lanthionization in cosmetic treatments result in fragile or degraded products, and lack control over the formation of sulfonic acid groups and molecular weight, limiting their application in biomedical and other fields.

Innovation Solution

A process involving partial lanthionization of cystine disulfide bonds in keratin-containing materials under mild conditions, specifically at ambient temperature and in non-aqueous or semi-aqueous media, using hydroxide bases like NaOH or KOH, to create permanent thioether linkages, which can be further oxidized to control sulfonic acid groups and molecular weight, enhancing material properties like elasticity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If lanthionization is performed under conventional conditions (aqueous medium, elevated temperature, external agitation), then the reaction proceeds efficiently, but the keratin material becomes fragile and degraded

Engineering Contradiction:
Improvereaction efficiencyVSAvoidmaterial integrity
Core Design Contradiction:
ProductivityVSStrength

Solution Approach 1:

The patent changes the physical and chemical parameters of the reaction medium from aqueous to non-aqueous (using solvents like ethanol, methanol, acetone, or their mixtures with water). This parameter change allows the lanthionization reaction to proceed while preserving keratin material integrity, preventing the fragility and degradation that occurs under conventional aqueous conditions

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent introduces a new dimension to the reaction conditions by using non-aqueous media instead of traditional aqueous solutions. This dimensional change in the reaction environment fundamentally alters the reaction pathway and product characteristics, enabling controlled lanthionization without material degradation

Inventive Principle:
Principle #17Another dimension (Dimensionality change)

2Reliability

If oxidation is performed to break cystine bonds, then the reaction is irreversible and controls subsequent oxidation, but the material becomes too fragile for certain applications

Engineering Contradiction:
Improvecontrol over oxidationVSAvoidmaterial fragility
Core Design Contradiction:
ReliabilityVSStrength

Solution Approach 1:

The patent applies partial lanthionization rather than complete oxidation of cystine bonds. By performing partial conversion to lanthionine under controlled non-aqueous conditions, the patent achieves sufficient control over subsequent oxidation while avoiding the excessive damage and fragility that results from complete oxidation

Inventive Principle:
Principle #16Partial or excessive action

Solution Approach 2:

The patent uses non-aqueous solvents as intermediary media to facilitate the lanthionization reaction. These solvents act as intermediaries that enable the reaction to proceed controllably without directly causing the material degradation that occurs with conventional aqueous oxidation methods

Inventive Principle:
Principle #24Intermediary (Mediator)

3Adaptability or versatility

If lanthionization is applied to raw keratin materials, then new biomaterials can be prepared, but the process lacks control over molecular weight and sulfonic acid group formation

Engineering Contradiction:
Improvematerial application rangeVSAvoidcontrol over molecular weight
Core Design Contradiction:
Adaptability or versatilityVSManufacturing precision

Solution Approach 1:

The patent employs controlled lanthionization conditions that provide feedback mechanisms for regulating the reaction extent. By monitoring and controlling parameters such as solvent composition, temperature, and reaction time in non-aqueous media, the patent achieves precise control over molecular weight and sulfonic acid group formation, enabling tailored biomaterial production

Inventive Principle:
Principle #23Feedback

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process yields keratin materials with improved elasticity and controlled sulfonic acid groups, allowing for higher molecular weight derivatives and tailored biomaterials suitable for various applications, including biomedical uses, by preserving crosslinks and reducing the formation of insoluble fractions.

Implementation Method 1

A process is provided for the conversion of the disulfide groups (R—S—S—R) of the cystine residues in keratin to lanthionine residues (thioether groups, R—S—R)

Methodology Applied
Scientific EffectNucleophilic substitution: Chemical Bonding

Implementation Method 2

The lanthionized material may then be oxidized to produce cysteic acid groups from at least a portion of the remaining cystines

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 3

The residual H2S is removed by washing with water and by vacuum drying

Methodology Applied
Scientific EffectVacuum drying: Vacuum

Data Source

PatentUS8101202B2Gentle process for conversion of cystine in keratin-containing materials to lanthionine
Publication Date: 2012.01.24 KERAPLAST LTD

AI summary

Useful materials are produced from keratin containing raw materials by a process that includes gentle lanthionization of cystine disulfide bonds. Hydratable materials are produced for use in medical and cosmetic applications.