Laval Nozzle Gas Distribution in Polysilicon Reactors

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Solution Overview

Problem

Fluidized bed reactors experience pressure fluctuations and instabilities in gas mass streams, leading to non-uniform distribution and sintering issues during the production of polycrystalline silicon granules, which affect the chemical process and temperature distribution.

Innovation Solution

Incorporating Laval nozzles upstream of the openings in the reactor base to expand the gas mass streams supercritically, ensuring uniform distribution and stabilizing the pressure conditions, thereby preventing sintering and enhancing the production process.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If gas mass streams are fed through openings in the reactor base, then the fluidized bed can be operated, but pressure fluctuations and non-uniform distribution occur leading to sintering issues

Engineering Contradiction:
Improvestability of pressure conditionsVSAvoiduniform distribution of gas mass streams
Core Design Contradiction:
ReliabilityVSStability of the object's composition

Solution Approach 1:

A Laval nozzle is introduced as an intermediary component between the gas supply and the fluidized bed. The nozzle mediates the gas flow by accelerating it to supersonic speeds, which stabilizes the pressure conditions and ensures uniform distribution of the gas mass streams across the reactor base, preventing sintering issues while maintaining reliable operation.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The Laval nozzle changes the parameters of the gas flow by accelerating it from subsonic to supersonic speeds. This parameter change results in stabilized pressure conditions and improved uniformity of gas distribution, resolving the contradiction between reliability and composition stability.

Inventive Principle:
Principle #35Parameter changes

2Device complexity

If conventional openings are used in the reactor base, then the structure is simple, but pressure fluctuations cause sintering and affect temperature distribution

Engineering Contradiction:
Improvestructure of reactor baseVSAvoidsintering and temperature distribution issues
Core Design Contradiction:
Device complexityVSObject-affected harmful factors

Solution Approach 1:

The Laval nozzle serves as an intermediary device that addresses the harmful effects of pressure fluctuations without significantly complicating the overall reactor structure. By incorporating the nozzle into the existing opening system, the design maintains relative simplicity while effectively preventing sintering and improving temperature distribution.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The conventional mechanical opening system is enhanced by replacing simple openings with Laval nozzles that utilize fluid dynamics principles. This substitution transforms the gas flow mechanism from a simple pressure-driven system to one that leverages supersonic flow characteristics, eliminating sintering issues while maintaining structural efficiency.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The use of Laval nozzles provides a consistent and uniform distribution of gas mass streams, reducing pressure fluctuations and improving the stability of the fluidized bed reactor, resulting in improved polysilicon granule production by maintaining optimal temperature and chemical process stability.

Implementation Method 1

Laval nozzles upstream of the openings (2, 6) in the reactor base (1) are suitable for expanding supercritically at least one mass stream (5, 4) that is fed

Methodology Applied
Scientific EffectSupercritical expansion: Supercritical Fluid

Implementation Method 2

a Laval nozzle (3) upstream of at least one of the openings (2, 6) in the reactor base (1) outside the inner reactor tube (11), which is suitable for expanding supercritically

Methodology Applied
Scientific EffectLaval nozzle effect: De Laval Nozzle

Implementation Method 3

the fluidized bed being heated to high temperatures by means of a heating device

Methodology Applied
Scientific EffectThermal heating: Heating

Implementation Method 4

an inner reactor tube made of a material which has a high transmission for thermal radiation

Methodology Applied
Scientific EffectThermal radiation: Thermal Radiation

Implementation Method 5

fluidizing silicon particles by means of a gas flow in a fluidized bed

Methodology Applied
Scientific EffectFluidization: Fluidisation

Implementation Method 6

Addition of a silicon-containing reaction gas results in a pyrrolysis reaction on the hot particle surface. In the process, elemental silicon deposits on the silicon particles

Methodology Applied
Scientific EffectPyrolysis: Pyrolysis

Data Source

PatentUS10899626B2Fluidized bed reactor and method for producing granular polysilicon
Publication Date: 2021.01.26 WACKER CHEMIE AG
  • US10899626B2 patent drawing
  • US10899626B2 patent drawing
  • US10899626B2 patent drawing

AI summary

The fluidized bed process for preparing polysilicon by chemical vapor deposition is improved by positioning at least one Laval nozzle upstream from a gas inlet into the reactor.