LCO Hydroconversion Catalyst with Segmented Zeolite Core

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Solution Overview

Problem

The handling of light cycle oil (LCO) is challenging due to its poor cetane properties and high sulfur content, limiting its use in diesel and requiring effective conversion to meet stringent fuel and environmental regulations, with existing hydrocracking catalysts not efficiently achieving partial ring opening of multi-ring aromatics for petrochemical feedstock production.

Innovation Solution

A catalyst composition featuring ultra-stable Y zeolite as a carrier with alumina binder, incorporating Group VIB and VIIIB metals, and nitrogen-oxygen containing organic additives to form highly dispersed WS2 slabs, enabling selective ring opening of aromatics and efficient hydroconversion of LCO into petrochemical feedstocks.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If conventional hydrocracking catalysts are used for LCO conversion, then diesel blending is achieved, but selective partial ring opening of multi-ring aromatics for petrochemical feedstock production is not efficient

Engineering Contradiction:
Improveconversion efficiency of LCOVSAvoidselectivity for partial ring opening
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The patent applies local quality by creating distinct functional zones within the catalyst颗粒. The outer shell contains high acidity for cracking activity, while the inner core provides hydrogenation function. This spatial differentiation enables simultaneous cracking of multi-ring aromatics and selective hydrogenation, achieving both high conversion and selectivity for partial ring opening to produce petrochemical feedstocks like benzene, toluene and xylene.

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The patent employs composite materials by combining zeolite components (for acidity and cracking), metal components (for hydrogenation), and matrix materials into a structured catalyst. This composite structure integrates multiple catalytic functions within a single catalyst颗粒, enabling efficient LCO conversion with selective partial ring opening that conventional single-function catalysts cannot achieve.

Inventive Principle:
Principle #40Composite materials

2Manufacturing precision

If mild hydrocracking conditions are applied to convert di and tri-aromatics into alkyl benzene, then mono-aromatics are kept intact, but the catalyst requires optimum balance of acid sites and hydrogenation function which is difficult to achieve

Engineering Contradiction:
Improveselectivity for mono-aromatics preservationVSAvoidcatalyst composition optimization
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent applies segmentation by dividing the catalyst into functional segments or zones. The outer shell is designed with high acidity to facilitate cracking of di and tri-aromatics, while the inner core contains metal components for hydrogenation. This segmented structure allows independent optimization of cracking and hydrogenation functions, achieving selective conversion while preserving mono-aromatics without requiring complex overall composition optimization.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent applies preliminary action by pre-organizing the catalyst structure during preparation to establish the functional zones before the reaction occurs. The metal components are pre-positioned in the inner core and zeolite components in the outer shell, so that when LCO contacts the catalyst, the desired selective reaction pathway is immediately established, preserving mono-aromatics while converting di and tri-aromatics.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The catalyst composition achieves high conversion and selectivity in producing valuable petrochemical feedstocks like benzene, toluene, and xylene, with superior activity and stability, outperforming comparable catalysts in ring opening and hydrocracking of LCO.

Implementation Method 1

a catalyst composition comprising an ultra-stable Y zeolite as a carrier and alumina as binder

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 2

incorporating Group VIB and VIIIB metals, and nitrogen-oxygen containing organic additives to form highly dispersed WS2 slabs, enabling selective ring opening of aromatics and efficient hydroconversion of LCO

Methodology Applied
Scientific EffectHydrogenation: Hydrogenation

Data Source

PatentEP3590601B1Catalyst composition, and method of preparation of the same, for hydro-conversion of LCO involving partial ring opening of poly-aromatics
Publication Date: 2024.07.03 INDIAN OIL CORP LTD
  • EP3590601B1 patent drawingFigure 1

AI summary

The present invention relates to a catalyst composition and a process for preparing thereof, wherein the catalyst composition is specifically active for hydro-conversion of LCO involving mainly the partial ring opening of multi-ring aromatics leading to the production of petrochemical feedstock. The catalyst composition comprises of a carrier comprising ultra-stable Y zeolite and binder alumina, group VIB and VIIIB metal species, and organic additives. The carrier is impregnated with metal solution to form active sites of WS2 slabs of dimensions in the range of 35-45 Å.