Lead Alloy Grid Composition for Corrosion Resistance

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Solution Overview

Problem

Current lead-acid battery grid alloys face challenges in maintaining mechanical properties, corrosion resistance, and preventing thermal runaway, especially in deep discharge-charge cycling regimes, while also dealing with environmental concerns from cadmium-containing alloys and the high cost of silver-based alternatives.

Innovation Solution

A lead-based alloy with specific compositions of tin, calcium, bismuth, and copper is developed, which provides enhanced mechanical properties, improved corrosion resistance, reduced gassing, and lower sulfation, eliminating the need for post-casting treatments and offering better performance than existing alloys.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If continuous direct casting process is used to manufacture grids, then manufacturing efficiency and economy are improved, but corrosion resistance deteriorates due to oriented grains creating shorter intergranular paths

Engineering Contradiction:
Improvemanufacturing efficiencyVSAvoidcorrosion resistance
Core Design Contradiction:
ProductivityVSReliability

Solution Approach 1:

The patent modifies the chemical composition parameters of the lead alloy by adding specific amounts of bismuth (0.01-0.05 wt%), tin (0.5-2.0 wt%), and calcium (0.01-0.1 wt%), which changes the corrosion behavior and grain structure of the alloy, thereby improving corrosion resistance while maintaining the continuous casting process

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite alloy system by combining lead with multiple alloying elements (bismuth, tin, calcium, copper, silver), where each element contributes specific properties that collectively enhance corrosion resistance and mechanical properties while allowing continuous casting

Inventive Principle:
Principle #40Composite materials

2Strength

If cadmium-containing alloys are used to improve mechanical properties and corrosion resistance, then grid strength is improved, but environmental harm increases

Engineering Contradiction:
Improvegrid strengthVSAvoidenvironmental harm
Core Design Contradiction:
StrengthVSObject-affected harmful factors

Solution Approach 1:

The patent removes cadmium from the alloy composition entirely and replaces it with environmentally friendly alternative elements (bismuth, tin, calcium), thereby eliminating the harmful environmental effects while maintaining or improving the desired mechanical and corrosion resistance properties

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent changes the chemical composition parameters by substituting toxic cadmium with non-toxic alternative elements in specific concentrations, transforming the alloy from harmful to environmentally friendly while preserving performance

Inventive Principle:
Principle #35Parameter changes

3Reliability

If silver-based alloys are used to enhance corrosion resistance, then corrosion protection is improved, but manufacturing cost increases

Engineering Contradiction:
Improvecorrosion resistanceVSAvoidmanufacturing cost
Core Design Contradiction:
ReliabilityVSQuantity of substance

Solution Approach 1:

The patent optimizes the concentration parameters of alloying elements, using silver at low levels (0.01-0.1 wt%) combined with more cost-effective elements like bismuth and tin, thereby achieving the desired corrosion resistance at a lower overall cost than traditional silver-based alloys

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a multi-element composite alloy where silver works synergistically with other elements (bismuth, tin, calcium, copper), allowing reduced silver content while maintaining or enhancing corrosion resistance, thereby lowering manufacturing cost

Inventive Principle:
Principle #40Composite materials

4Duration of action of stationary object

If grid alloy undergoes corrosion during service life, then electrical conductivity decreases causing cell failure, but this is a natural degradation process

Engineering Contradiction:
Improveservice lifeVSAvoidelectrical conductivity
Core Design Contradiction:
Duration of action of stationary objectVSReliability

Solution Approach 1:

The patent modifies the chemical composition parameters of the grid alloy by adding elements that form more stable and conductive corrosion products, changing the corrosion mechanism itself to preserve electrical conductivity over time

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent transforms the harmful corrosion process into a beneficial one by designing an alloy that forms protective, conductive corrosion products (such as calcium sulfate and stable lead oxides) that actually protect the grid and maintain conductivity, converting the degradation process into a protective mechanism

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Data Source

PatentEP2901511B1Lead-acid battery positive plate and alloy therefore
Publication Date: 2019.09.11 EXIDE TECHNOLOGIES LLC
  • EP2901511B1 patent drawingFigure 1~2
  • EP2901511B1 patent drawingFigure 3~4
  • EP2901511B1 patent drawingFigure 5~7

AI summary

A lead-acid battery grid made from a lead-based alloy containing tin, calcium, bismuth and copper and characterized by enhanced mechanical properties, corrosion resistance, less battery gassing, lower sulfation and water loss, and no post-casting treatment requirements for age hardening. In one embodiment, the battery grids are formed from a lead-based alloy including about 2.0% tin, about 0.0125% copper, about 0.065% calcium, and about 0.032% bismuth. Preferably, the battery grid is free of silver beyond trace levels in the alloy.