Levulinic Acid Production via Continuous Extraction

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Solution Overview

Problem

Current methods for producing levulinic acid from biomass face challenges such as low yields, difficulty in separating the acid from mineral catalysts and byproducts, high temperature requirements, and equipment fouling, leading to inefficient and costly production processes.

Innovation Solution

A process utilizing high concentrations of acid (20-80 weight percent) at lower temperatures (60-160°C) to improve yield and reduce byproducts, with continuous addition of biomass and selective solvent extraction to enhance purity and ease of product recovery, allowing for the use of biomass as a feedstock to produce levulinic acid and related compounds.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Speed

If high temperature reaction conditions are used for biomass hydrolysis, then the reaction rate increases, but the yield of levulinic acid decreases and equipment fouling increases

Engineering Contradiction:
Improvereaction rateVSAvoidlevulinic acid yield
Core Design Contradiction:
SpeedVSProductivity

Solution Approach 1:

The patent changes the temperature parameter from high (conventional) to low (60-160°C range), and adjusts acid concentration and reaction time parameters to compensate, achieving high reaction rates without the negative effects of high temperature while maintaining high levulinic acid yield

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent employs continuous addition of biomass and continuous removal of products, dynamically adjusting reaction conditions to maintain optimal reaction rate and yield throughout the process, preventing equilibrium limitations and side reactions

Inventive Principle:
Principle #15Dynamics

2Device complexity

If conventional hydrolysis conditions are used, then the process is simpler, but the separation of levulinic acid from mineral acid catalysts and byproducts becomes difficult

Engineering Contradiction:
Improveprocess simplicityVSAvoidseparation difficulty
Core Design Contradiction:
Device complexityVSEase of manufacture

Solution Approach 1:

The patent continuously extracts and removes levulinic acid and formic acid from the reaction mixture as they are formed, separating them from the mineral acid catalyst and char byproducts, which simplifies the overall separation process and improves product purity

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent uses an extraction solvent as an intermediary medium to selectively extract levulinic acid from the reaction mixture, facilitating separation from the aqueous phase containing mineral acids and char particles

Inventive Principle:
Principle #24Intermediary (Mediator)

3Manufacturing precision

If long digestion periods are used for biomass hydrolysis, then conversion completeness improves, but the production time increases and productivity decreases

Engineering Contradiction:
Improveconversion completenessVSAvoidproduction time
Core Design Contradiction:
Manufacturing precisionVSLoss of time

Solution Approach 1:

The patent maintains continuous hydrolysis reaction with continuous addition of biomass and continuous removal of products, ensuring complete conversion without requiring long batch digestion periods, thereby maintaining high productivity

Inventive Principle:
Principle #20Continuity of useful action

Solution Approach 2:

The patent performs preliminary preparation of biomass feedstock and pre-heating of reaction mixture to optimize reaction conditions from the start, reducing the time required to achieve complete conversion

Inventive Principle:
Principle #10Preliminary action

4Reliability

If specialized equipment is used to withstand hydrolysis conditions, then reaction reliability improves, but equipment cost increases

Engineering Contradiction:
Improvereaction reliabilityVSAvoidequipment cost
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent changes reaction parameters to lower temperature and moderate pressure conditions that do not require specialized expensive equipment, while maintaining reliable reaction performance through optimized catalyst and process conditions

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process achieves high yields (>80%) and purities (>95%) of levulinic acid, reduces equipment fouling, and simplifies the separation of products from byproducts, making the production more efficient and cost-effective.

Implementation Method 1

sulfuric acid, which has been heated to a temperature from about 60°C to about 160°C. An aqueous solution comprising monosaccharides and/or disaccharides is then added to the sulfuric acid in the reactor

Methodology Applied
Scientific EffectAcid-catalyzed hydrolysis: Hydrolysis

Implementation Method 2

The organic extract phase is then separated from the aqueous raffinate phase

Methodology Applied
Scientific EffectLiquid-liquid extraction: Liquid-Liquid Extraction

Data Source

PatentEP2970083B1Process to prepare levulinic acid
Publication Date: 2021.10.20 GFBIOCHEM IP ASSETS BV

AI summary

The invention describes processes to prepare levulinic acid, formic acid and/or hydroxymethyl furfural from various biomass materials.