Inert Stabilization of Lignin Fiber for Carbon Conversion

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Solution Overview

Problem

Current methods for producing carbon fibers from lignin require a lengthy stabilization step under oxidative conditions, which slows down the process due to heterogeneous reactions and skin-core structure formation, making it inefficient for large-scale production.

Innovation Solution

A method involving the use of fractionated and/or unfractionated softwood alkaline lignin, optionally combined with hardwood alkaline lignin, is developed for spinning lignin fibers, which are stabilized under inert conditions, allowing for shorter reaction times and eliminating the need for oxidative stabilization.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If oxidative stabilization is used for lignin fibers, then the fiber structure is stabilized to prevent fusion during carbonization, but the process time is excessively long due to heterogeneous reactions and skin-core structure formation

Engineering Contradiction:
Improvefiber structure stabilityVSAvoidstabilization process time
Core Design Contradiction:
ReliabilityVSLoss of time

Solution Approach 1:

The patent applies inert atmosphere stabilization by conducting the stabilization process in an inert gas environment (nitrogen or carbon dioxide) instead of oxidative conditions. This eliminates the formation of skin-core structure and heterogeneous reactions that occur during oxidative stabilization, thereby reducing the stabilization time from hours to minutes while still preventing fiber fusion during subsequent carbonization.

Inventive Principle:
Principle #39Inert atmosphere (Inert environment)

2Manufacturing precision

If slow heating rate is used during stabilization, then homogeneous oxidation occurs throughout the fiber, but the process becomes inefficient for large-scale production

Engineering Contradiction:
Improveoxidation uniformityVSAvoidproduction efficiency
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

By replacing oxidative atmosphere with inert atmosphere, the patent eliminates the need for slow heating rates required for homogeneous oxidation. The inert atmosphere prevents unwanted oxidative reactions while allowing rapid heating rates to be used, thus achieving both production efficiency and sufficient stabilization for preventing fiber fusion during carbonization.

Inventive Principle:
Principle #39Inert atmosphere (Inert environment)

Solution Approach 2:

The patent changes the fundamental parameter of atmosphere composition from oxidative to inert, which fundamentally alters the stabilization mechanism. This parameter change allows the process to proceed at much higher heating rates without the formation of skin-core structure, thereby resolving the contradiction between oxidation uniformity and production efficiency.

Inventive Principle:
Principle #35Parameter changes

3Productivity

If lignin fibers are carbonized without prior stabilization, then the process is faster, but the fibers fuse and lose their structural integrity

Engineering Contradiction:
Improvecarbonization speedVSAvoidfiber structural integrity
Core Design Contradiction:
ProductivityVSStrength

Solution Approach 1:

The patent uses inert atmosphere stabilization to create a stable fiber structure that prevents fusion during carbonization. The inert stabilization process modifies the lignin structure in a way that provides thermal stability without requiring subsequent oxidative treatment, enabling fast carbonization while maintaining fiber structural integrity.

Inventive Principle:
Principle #39Inert atmosphere (Inert environment)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enables faster stabilization and subsequent carbonization of lignin fibers, resulting in solid, homogeneous carbon fibers without fusion, with the process being scalable and environmentally friendly due to the use of renewable resources.

Implementation Method 1

stabilization of the lignin fiber under inert conditions

Methodology Applied
Scientific EffectThermal treatment: Heating

Implementation Method 2

carbonization of the stabilized lignin fiber

Methodology Applied
Scientific EffectPyrolysis: Pyrolysis

Data Source

PatentUS11286582B2Method for stabilizing lignin fiber for further conversion to carbon fiber
Publication Date: 2022.03.29 RISE INNVENTIA AB

AI summary

A method for producing a stabilized lignin fiber from softwood alkaline lignin by heat treatment in the absence of oxidant is disclosed. The stabilized lignin fiber can be further treated to obtain carbon fiber.