Lignin-Modified Polyol for Biobased Polyurethane Foam

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Current polyurethane foam production using isocyanates generates toxic gases when burned and requires costly petroleum-based materials, while biobased alternatives face challenges in achieving optimal physical properties and compatibility with conventional formulations.

Innovation Solution

Incorporating lignin, a renewable raw material with aromatic functional groups, into polyol compositions to enhance the properties of polyurethane systems, such as rigidity, thermal stability, and moisture resistance, while reducing the need for petroleum-based chemicals and isocyanate content.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If isocyanate is used to produce polyurethane foam, then the physical properties and foam structure are improved, but toxic gases are generated when burned

Engineering Contradiction:
Improvephysical propertiesVSAvoidtoxic gases
Core Design Contradiction:
StrengthVSObject-generated harmful factors

Solution Approach 1:

The patent changes the chemical composition parameters by incorporating biobased polyols (5-50 wt%) and lignin (5-50 wt%) to replace petrochemical polyols and reduce isocyanate content (20-80 wt%), thereby maintaining foam physical properties while reducing toxic gas generation during combustion

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite polyol formulation combining biobased polyols, lignin, and petrochemical polyols in specific ratios, where lignin provides structural support and the biobased components reduce toxicity, achieving both physical property maintenance and harmful factor reduction

Inventive Principle:
Principle #40Composite materials

2Strength

If petroleum-based polyols are used, then the reaction with isocyanate produces optimal foam properties, but the cost increases due to petroleum price volatility

Engineering Contradiction:
Improvefoam propertiesVSAvoidcost
Core Design Contradiction:
StrengthVSQuantity of substance

Solution Approach 1:

The patent adjusts the polyol composition parameters by incorporating 5-50 wt% biobased polyols with specific hydroxyl values (50-200 mg KOH/g) and molecular weights (500-2000 g/mol) to replace expensive petrochemical polyols, reducing formulation cost while maintaining reaction optimality with isocyanate

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent substitutes expensive, volatile-priced petrochemical polyols with cheaper, renewable biobased polyols derived from agricultural sources, reducing raw material cost exposure to petroleum price fluctuations while maintaining functional performance

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Reliability

If halogenated blowing agents are used, then the flame resistance is improved, but environmental concerns lead to phaseout requirements

Engineering Contradiction:
Improveflame resistanceVSAvoidenvironmental harm
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent changes the blowing agent chemical composition by substituting halogenated compounds with hydrocarbon-based blowing agents (pentane, neopentane, isopentane, cyclopentane) having specific vapor pressures (50-200 mmHg at 25°C), achieving flame resistance through formulation adjustments while eliminating environmental harm

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent converts the potential flammability risk of hydrocarbon blowing agents into a benefit by optimizing the overall foam formulation with lignin and biobased polyols that enhance flame resistance, thereby achieving environmental compliance without sacrificing safety

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

4Object-affected harmful factors

If biobased polyols are used to replace petroleum-based materials, then environmental friendliness is improved, but compatibility with conventional formulations and optimal physical properties are difficult to achieve

Engineering Contradiction:
Improveenvironmental friendlinessVSAvoidphysical properties
Core Design Contradiction:
Object-affected harmful factorsVSStrength

Solution Approach 1:

The patent creates a composite polyol system combining biobased polyols (5-50 wt%), lignin (5-50 wt%), and petrochemical polyols in optimized ratios, where each component contributes specific properties: biobased polyols provide environmental friendliness, lignin provides structural rigidity and compatibility, and petrochemical polyols ensure optimal reaction kinetics with isocyanate

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent uses lignin as an intermediary substance that bridges biobased polyols and conventional foam formulations, providing compatibility through its dual solubility characteristics and functional groups that interact with both biobased components and isocyanate, enabling optimal physical properties

Inventive Principle:
Principle #24Intermediary (Mediator)

5Object-generated harmful factors

If isocyanate content is reduced to lower cost and toxicity, then harmful factors are decreased, but the foam structure and physical properties deteriorate

Engineering Contradiction:
ImprovetoxicityVSAvoidfoam structure
Core Design Contradiction:
Object-generated harmful factorsVSStrength

Solution Approach 1:

The patent changes the formulation parameters by reducing isocyanate content to 20-80 wt% (below conventional levels) while compensating with biobased polyols (5-50 wt%) and lignin (5-50 wt%) that provide alternative crosslinking mechanisms and structural support, maintaining foam integrity with lower isocyanate

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent converts the reduced isocyanate content (which would normally weaken foam structure) into a benefit by using biobased polyols and lignin to provide structural reinforcement, thereby achieving both toxicity reduction and foam structure maintenance simultaneously

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The use of lignin improves the physical properties of polyurethane foams, including increased strength, thermal resistance, and reduced odor, while decreasing the amount of isocyanate and petroleum-based materials needed, resulting in cost-effective and environmentally friendly formulations.

Implementation Method 1

The use of lignin improves the physical properties of polyurethane foams, including increased strength, thermal resistance

Methodology Applied
Scientific EffectChemical Bonding: Chemical Bonding

Implementation Method 2

Incorporating lignin, a renewable raw material with aromatic functional groups, into polyol compositions to enhance the properties of polyurethane systems, such as rigidity, thermal stability

Methodology Applied
Scientific EffectThermal stability:

Implementation Method 3

Incorporating lignin, a renewable raw material with aromatic functional groups, into polyol compositions to enhance the properties of polyurethane systems, such as rigidity, thermal stability, and moisture resistance

Methodology Applied
Scientific EffectHydrophobic effect: Hydrophobe

Data Source

PatentUS10745513B1Polyol, adhesive, resin, and tackifier-thixotropic additive
Publication Date: 2020.08.18 ORGANIC CHEM

AI summary

A renewable chemical composition is disclosed for use in a variety of industrial applications. The renewable chemical composition may be reacted with an isocyanate to produce a polyurethane material. The renewable chemical composition has aromatic groups. The suitability of this material for use in a variety of applications can be adjusted by modifying the acid number, the Hydroxyl number, the viscosity, the glass transition temperature, the % solids, the softening point, and other properties. The chemical reactivity and properties can be modified based on processing conditions and temperature as well as the source of renewable raw material. The lignin used in these formulations may be from pulp and paper processing such as semi-mechanical processing, soda processing, kraft processing, or biomass processing, or a by-product of ethanol production. The novel biobased polyurethane formulations range in firmness from flexible to semi-rigid to rigid and are useful in large volume polyurethane applications.