Lithium Metal Anode Protective Film for Dendrite Suppression

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Solution Overview

Problem

Lithium metal anodes in batteries face issues with lithium dendrite growth during charging and discharging, leading to reduced lifespan, internal short-circuits, and safety risks such as fires and explosions, due to unstable film formation and high reactivity with the electrolyte.

Innovation Solution

A lithium metal anode protective film comprising lithium nitride (Li3N) nanoparticles, lithium-magnesium (Li-Mg) alloy nanoparticles, or a combination thereof, is formed on the lithium metal layer to induce uniform electrodeposition and suppress dendrite growth, using an in-situ reaction to stabilize the lithium metal layer.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If a protective film is formed on the lithium metal layer to suppress dendrite growth, then safety and stability are improved, but unnecessary material formation occurs and energy density is reduced

Engineering Contradiction:
ImprovestabilityVSAvoidenergy density
Core Design Contradiction:
ReliabilityVSQuantity of substance

Solution Approach 1:

The patent changes the chemical composition parameters of the protective film by using lithium nitride and lithium-magnesium alloy nanoparticles instead of conventional thick protective layers. This chemical parameter change enables effective dendrite suppression with minimal material quantity, thus improving stability while maintaining energy density.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent employs a composite protective film structure combining lithium nitride nanoparticles and lithium-magnesium alloy nanoparticles. This composite material approach provides synergistic effects where both components work together to suppress dendrite growth more effectively than single materials, reducing the total amount of protective material needed and preserving energy density.

Inventive Principle:
Principle #40Composite materials

2Object-generated harmful factors

If conventional protective materials are used to stabilize the lithium metal layer, then dendrite growth is suppressed, but unnecessary material formation occurs and electrochemical performance is reduced

Engineering Contradiction:
Improvedendrite growthVSAvoidelectrochemical performance
Core Design Contradiction:
Object-generated harmful factorsVSReliability

Solution Approach 1:

The patent applies local quality by using nanoscale particles (1-100 nm) that can be uniformly distributed on the lithium metal layer surface. This localized nanoscale protection provides targeted dendrite suppression at critical sites without forming thick unnecessary layers, thereby maintaining excellent electrochemical performance while effectively suppressing dendrite growth.

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The patent uses small quantities of lithium nitride and lithium-magnesium alloy nanoparticles that form a thin protective layer. This approach replaces conventional thick protective materials with minimal amounts of functional nanoparticles that provide sufficient protection against dendrites while maintaining high electrochemical performance, effectively using 'less is more' strategy.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The protective film enhances electrochemical performance and stability, preventing unnecessary material formation and improving energy density and safety by ensuring uniform lithium ion distribution and reducing dendrite growth.

Implementation Method 1

forming a material for protecting a surface of a lithium metal layer on the surface of the lithium metal layer by an In-situ reaction

Methodology Applied
Scientific EffectIn-situ reaction: Chemical Bonding

Implementation Method 2

induce uniform electrodeposition behavior and distribution of lithium ions

Methodology Applied
Scientific EffectElectrodeposition: Electrodeposition

Data Source

PatentEP4579792A1Protective film for lithium metal anode, lithium metal anode, method of preparing lithium metal anode, and lithium metal battery
Publication Date: 2025.07.02 SK ON CO LTD
  • EP4579792A1 patent drawingFigure 1
  • EP4579792A1 patent drawingFigure 2A
  • EP4579792A1 patent drawingFigure 2B

AI summary

A lithium metal anode protective film includes lithium nitride (Li3N) nanoparticles, lithium-magnesium (Li-Mg) alloy nanoparticles, or a combination thereof. The lithium metal anode protective film may induce uniform electrodeposition behavior and distribution of lithium ions, thereby effectively suppressing growth of lithium dendrites during battery a battery charging/discharging process.