Evaporation Apparatus for Lithium Deposition via Gas Pressure Control

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Solution Overview

Problem

Current thin film lithium battery deposition systems face challenges in managing the high reactivity of alkali and alkaline earth metals, particularly lithium, which limits high volume and low-cost manufacturing due to issues like oxidation, valve blockage, and low melting point constraints on deposition rates.

Innovation Solution

A depositing arrangement and apparatus that liquefies alkali or alkaline earth metals in a gas-inlet chamber, using a line with defined flow resistance and controlled gas pressure to regulate the flow rate, eliminating the need for mechanically working valves and allowing for uniform vapor deposition on substrates.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of operation

If conventional evaporation systems use mechanically working valves to control liquid lithium flow, then flow control is achieved, but valve blockage occurs due to slug/particle formation and high reactivity

Engineering Contradiction:
Improveflow controlVSAvoidvalve operation
Core Design Contradiction:
Ease of operationVSReliability

Solution Approach 1:

The patent removes the mechanically working valve from the system entirely. Instead of controlling liquid lithium flow through a valve, the system uses a capillary tube with defined flow resistance that passively regulates flow based on pressure differential, eliminating the source of blockage and mechanical failure.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent introduces a capillary tube as an intermediary flow resistance element between the liquid lithium source and evaporation zone. This capillary tube acts as a flow regulator that converts pressure control into flow control without requiring mechanical valves to contact the reactive lithium.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Productivity

If sputtering methods are used for lithium deposition, then deposition is achieved, but manufacturing cost and complexity increase due to target reactivity and handling requirements

Engineering Contradiction:
Improvedeposition capabilityVSAvoidmanufacturing and handling
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The patent replaces the mechanical sputtering process with a thermal evaporation process. Instead of using a sputtering target and ion bombardment, the system heats liquid lithium in a crucible to produce vapor for deposition, simplifying target handling and eliminating sputtering-specific complexity.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Solution Approach 2:

The patent changes the deposition mechanism from momentum transfer (sputtering) to thermal vaporization. By controlling temperature parameters of the liquid lithium and using gas pressure to regulate flow, the system achieves deposition without the mechanical complexity of sputtering targets and power supplies.

Inventive Principle:
Principle #35Parameter changes

3Productivity

If high power density sputtering regime is applied, then deposition rate increases, but lithium melting point limitation prevents achieving high deposition rates

Engineering Contradiction:
Improvedeposition rateVSAvoidmelting point constraint
Core Design Contradiction:
ProductivityVSTemperature

Solution Approach 1:

The patent utilizes the phase transition of lithium from liquid to vapor directly in the evaporation zone. By maintaining lithium in liquid form in the crucible (below melting point constraints) and allowing it to vaporize in the high-temperature evaporation zone, the system achieves high deposition rates without being limited by the melting point during the deposition process.

Inventive Principle:
Principle #36Phase transitions

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This solution enables high deposition rates and uniformity while reducing manufacturing costs and handling complexities associated with reactive materials, enhancing the scalability and efficiency of lithium-based battery production.

Implementation Method 1

a valve (140) configured for controlling a flow rate of the gas in the first chamber (110) for controlling a flow rate of the liquefied material through the line (120) having said flow resistance

Methodology Applied
Scientific EffectGas pressure: Pressure Increase

Implementation Method 2

an evaporation zone (114) configured for vaporizing the liquefied material

Methodology Applied
Scientific EffectEvaporation: Evaporation

Implementation Method 3

deposition of the material on a substrate

Methodology Applied
Scientific EffectPhysical vapor deposition: Physical Vapour Deposition

Data Source

PatentEP3077567B1Depositing arrangement, deposition apparatus and methods of operation thereof
Publication Date: 2021.02.24 APPLIED MATERIALS INC
  • EP3077567B1 patent drawingFigure 1~2
  • EP3077567B1 patent drawingFigure 3~4
  • EP3077567B1 patent drawingFigure 5

AI summary

A depositing arrangement for evaporation of a material including an alkali metal or alkaline earth metal, and for deposition of the material on a substrate is described. The depositing arrangement includes a first chamber configured for liquefying the material, wherein the first chamber comprises a gas inlet configured for inlet of a gas in the first chamber, an evaporation zone configured for vaporizing the liquefied material, a line providing a fluid communication between the first chamber and the evaporation zone for the liquefied material, wherein the line includes a first portion defining a flow resistance of the line, a valve configured for controlling the flow rate of the gas in the first chamber for controlling a flow rate of the liquefied material through the line having said flow resistance, and one or more outlets for directing the vaporized material towards the substrate.