Lithium Metal Foil Nano-Imprint Structure for Separator Adhesion

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Solution Overview

Problem

Conventional lithium metal secondary batteries face challenges in achieving adequate electrode-separator adhesive strength due to the use of a lithium metal foil with a flat and smooth surface, leading to issues like separation and meandering, especially when applied in next-generation batteries without a separate negative electrode active material.

Innovation Solution

A nano imprint pattern structure is formed on the surface of the lithium metal foil to enhance adhesion with the separator, allowing for physical bonding through shape deformation during the lamination process, thereby improving the adhesive strength between the negative electrode and the separator.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Use of energy by moving object

If a lithium metal foil with a flat and smooth surface is used as the negative electrode, then the energy density is improved, but the adhesive strength between the negative electrode and separator deteriorates

Engineering Contradiction:
Improveenergy densityVSAvoidadhesive strength
Core Design Contradiction:
Use of energy by moving objectVSStrength

Solution Approach 1:

The patent applies surface texturing to the lithium metal foil negative electrode, creating micro-protrusions and micro-depressions on the surface. This curvature modification replaces the flat smooth surface with a textured surface that enables mechanical interlocking with the separator, thereby improving adhesive strength while maintaining the high energy density benefits of lithium metal foil.

Inventive Principle:
Principle #14Spheroidality (Curvature)

2Ease of manufacture

If a lithium metal foil with a flat and smooth surface is used as the negative electrode, then the manufacturing simplicity is improved, but the assembly processability deteriorates

Engineering Contradiction:
Improvemanufacturing simplicityVSAvoidassembly processability
Core Design Contradiction:
Ease of manufactureVSEase of operation

Solution Approach 1:

The patent implements surface texturing on the lithium metal foil negative electrode before assembly. This preliminary action of creating micro-protrusions and micro-depressions on the surface enables the electrode to form strong mechanical interlocking with the separator during assembly, thereby improving assembly processability while maintaining manufacturing simplicity through integration into the electrode preparation process.

Inventive Principle:
Principle #10Preliminary action

3Stability of the object's composition

If a lithium metal foil with a flat and smooth surface is used as the negative electrode, then the material uniformity is improved, but the adhesion mechanism deteriorates

Engineering Contradiction:
Improvematerial uniformityVSAvoidadhesion mechanism
Core Design Contradiction:
Stability of the object's compositionVSStrength

Solution Approach 1:

The patent introduces micro-scale surface texturing with protrusions and depressions on the lithium metal foil negative electrode. This curvature modification creates mechanical interlocking capability with the separator, transforming the adhesion mechanism from relying solely on electrostatic attraction to incorporating strong mechanical interlocking, thereby improving the overall adhesion mechanism while preserving material uniformity.

Inventive Principle:
Principle #14Spheroidality (Curvature)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The enhanced adhesive strength between the negative electrode and separator prevents bending and separation of the unit cell, improving the assembly processability and overall performance of lithium metal secondary batteries.

Implementation Method 1

a physical adhesion by the shape deformation of (the binder in) the separator that has been achieved through the rough active material surface shape of the conventional lithium ion secondary battery

Methodology Applied
Scientific EffectPhysical adhesion: Adhesive

Implementation Method 2

only a chemical adhesion by electrostatic attraction might be relied on

Methodology Applied
Scientific EffectElectrostatic attraction: Electrostatics

Data Source

PatentEP3624248B1Lithium metal secondary battery and manufacturing method therefor
Publication Date: 2025.06.25 LG ENERGY SOLUTION LTD
  • EP3624248B1 patent drawingFigure 1(a)~1(d)
  • EP3624248B1 patent drawingFigure 2
  • EP3624248B1 patent drawingFigure 3

AI summary

Provided is a lithium metal secondary battery ensuring electrode-separator adhesive strength and a method for fabricating the same. The lithium metal secondary battery according to the present disclosure includes a negative electrode, a separator and a positive electrode, the negative electrode including a lithium metal foil as a negative electrode material, wherein a nano imprint pattern structure is formed on a lithium metal foil surface which is a surface of the negative electrode facing the separator, and the negative electrode and the separator are adhered to each other.