Lithium Nickel Composite Oxide Positive Electrode Active Material

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Solution Overview

Problem

Lithium-nickel composite oxides with excess oxygen in lithium ion batteries do not achieve optimal performance as high-quality positive electrode active materials, requiring improvements in battery properties such as capacity, rate performance, and cycle characteristics.

Innovation Solution

A positive electrode active material with a composition of LixNi1−yMyO2+α, where M includes Co and other elements, and an average particle size of 5 μm to 15 μm, with excess oxygen (α > 0.05), optimized to enhance battery properties by controlling particle size distribution and oxygen content.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If lithium-nickel composite oxide with excess oxygen is used, then oxygen content increases, but battery property remains insufficient

Engineering Contradiction:
Improveoxygen contentVSAvoidbattery property
Core Design Contradiction:
Quantity of substanceVSReliability

Solution Approach 1:

The patent changes the oxygen content parameter from conventional levels to excess oxygen (α > 0.05 in formula LixNi1−yMyO2+α), and simultaneously optimizes particle size parameters (D50: 5-15 μm, D90: 20 μm or less) to achieve improved battery properties including capacity, rate performance, and cycle characteristics

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses a composite material system combining lithium-nickel composite oxide with multiple dopant elements (M = Co and at least one of Sc, Ti, V, Cr, Mn, Fe, Cu, Zn, Ga, Ge, Al, Bi, Sn, Mg, Ca, B, or Zr) to achieve synergistic effects that improve battery performance while maintaining structural stability

Inventive Principle:
Principle #40Composite materials

2Productivity

If particle size is reduced to improve rate performance, then capacity may decrease, but if particle size is increased to improve capacity, then rate performance deteriorates

Engineering Contradiction:
Improverate performanceVSAvoidcapacity
Core Design Contradiction:
ProductivityVSQuantity of substance

Solution Approach 1:

The patent optimizes particle size parameters within specific ranges (D50: 5-15 μm, D90: 20 μm or less) to achieve a balance between rate performance and capacity, preventing both excessive particle size reduction and enlargement

Inventive Principle:
Principle #35Parameter changes

Data Source

PatentUS10122012B2Positive electrode active material for lithium-ion battery, a positive electrode for lithium-ion battery, and lithium-ion battery
Publication Date: 2018.11.06 JX NIPPON MINING & METALS CORP

AI summary

The present invention provides a positive electrode active material for lithium ion batteries having excellent battery property.The positive electrode active material for lithium ion batteries is represented by composition formula: LixNi1−yMyO2+α, whereinM is Co as an essential component and at least one species selected from a group consisting of Sc, Ti, V, Cr, Mn, Fe, Cu, Zn, Ga, Ge, Al, Bi, Sn, Mg, Ca, B and Zr, 0.9≤x≤1.2, 0<y≤0.7, α>0.05, andan average particle size (D50) is 5 μm to 15 μm.