Lithium Storage Element Using Pitch Coal Deposited on Activated Carbon

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Solution Overview

Problem

Current lithium ion capacitors face challenges in achieving high energy density, high output characteristics, and durability, particularly in maintaining these properties when the negative electrode active material layer is made thinner and the capacitor volume is reduced.

Innovation Solution

A nonaqueous lithium storage element is developed with a negative electrode active material layer containing a composite porous material where pitch coal is deposited on activated carbon, with a specific weight ratio and softening point, and doped with lithium ions within a certain range, enhancing both energy density and durability while maintaining high output characteristics.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Volume of moving object

If the negative electrode active material layer is made thinner to reduce capacitor volume, then the volume is reduced, but the energy density and durability deteriorate

Engineering Contradiction:
Improvecapacitor volumeVSAvoidenergy density
Core Design Contradiction:
Volume of moving objectVSQuantity of substance

Solution Approach 1:

The patent employs activated carbon with a porous structure as the negative electrode active material. The porous structure provides a large internal surface area that can accommodate lithium ions, enabling high energy density even in a thin layer. The pores allow efficient lithium ion transport while maintaining high capacitance per unit volume, thus achieving high energy density without requiring a thick electrode layer.

Inventive Principle:
Principle #31Porous materials

Solution Approach 2:

The patent uses a composite structure combining activated carbon with conductive additives and binding agents to create the negative electrode active material layer. This composite approach enhances the overall performance by improving electrical conductivity, mechanical strength, and lithium ion accessibility while maintaining a thin profile, thereby achieving high energy density in a reduced volume.

Inventive Principle:
Principle #40Composite materials

2Volume of moving object

If the negative electrode active material layer is made thinner to reduce capacitor volume, then the volume is reduced, but the output characteristics deteriorate

Engineering Contradiction:
Improvecapacitor volumeVSAvoidoutput characteristics
Core Design Contradiction:
Volume of moving objectVSPower

Solution Approach 1:

The porous structure of activated carbon provides numerous pathways for lithium ion transport, enabling rapid charge and discharge rates. The high surface area to volume ratio within the pores facilitates efficient ion exchange, maintaining high output characteristics even when the overall electrode layer is thin, thus achieving high power density in a compact volume.

Inventive Principle:
Principle #31Porous materials

Solution Approach 2:

The patent optimizes the local properties of the negative electrode active material by controlling the pore size distribution, surface chemistry, and material composition within the electrode layer. This local optimization ensures that lithium ion transport and electrochemical reactions occur efficiently throughout the thin layer, maintaining high output characteristics without requiring increased thickness.

Inventive Principle:
Principle #3Local quality

3Volume of moving object

If the negative electrode active material layer is made thinner to reduce capacitor volume, then the volume is reduced, but the durability deteriorates

Engineering Contradiction:
Improvecapacitor volumeVSAvoiddurability
Core Design Contradiction:
Volume of moving objectVSReliability

Solution Approach 1:

The composite structure includes binding agents and conductive additives that provide mechanical strength and structural integrity to the thin electrode layer. This composite approach prevents material degradation and maintains electrode stability during repeated charge/discharge cycles, ensuring high durability even when the electrode layer is thin and the capacitor volume is reduced.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The porous structure of activated carbon accommodates volume changes during lithium ion insertion and extraction, reducing mechanical stress on the electrode material. This structural flexibility prevents cracking and degradation over time, maintaining durability in thin electrode layers where mechanical failures would be more critical.

Inventive Principle:
Principle #31Porous materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution achieves compatibility of high energy density, high output characteristics, and durability, allowing for efficient lithium charge/discharge processes even with a thinner negative electrode active material layer and reduced capacitor volume.

Implementation Method 1

thermally reacting the activated carbon with the pitch in an inert atmosphere, to produce the composite porous material in which the pitch coal is deposited on the surface of the activated carbon

Methodology Applied
Scientific EffectThermal reaction:

Implementation Method 2

produce the composite porous material in which the pitch coal is deposited on the surface of the activated carbon

Methodology Applied
Scientific EffectDeposition: Deposition (physical)

Implementation Method 3

doped with lithium ions within a certain range

Methodology Applied
Scientific EffectIon doping: Ion Implantation

Implementation Method 4

initial-time lithium charge/discharge characteristics satisfy: charging amount is 1100 mAh/g to 2000 mAh/g, and discharging amount is 100 mAh/g or higher at a negative electrode potential of 0 to 0.5 V

Methodology Applied
Scientific EffectElectrochemical charge/discharge:

Implementation Method 5

a carbonaceous material is a carbon material capable of accommodating/releasing lithium in an ionized state

Methodology Applied
Scientific EffectAdsorption: Adsorption

Implementation Method 6

composite porous material having a pitch coal deposited on the surface of an activated carbon

Methodology Applied
Scientific EffectPorosity: Porosity

Data Source

PatentEP2930728B1Nonaqueous lithium storage element
Publication Date: 2020.02.05 ASAHI KASEI KOGYO KABUSHIKI KAISHA
  • EP2930728B1 patent drawingFigure 1(a)~1(b)
  • EP2930728B1 patent drawingFigure 2~3
  • EP2930728B1 patent drawingFigure 4

AI summary

Provided is a nonaqueous lithium storage element which is obtained by housing an electrode body and a nonaqueous electrolyte solution containing a lithium salt in an outer case, said electrode body being composed of a negative electrode that is composed of a negative electrode collector and a negative electrode active material layer laminated on one or both surfaces of the negative electrode collector, a positive electrode that is composed of a positive electrode collector and a positive electrode active material layer laminated on one or both surfaces of the positive electrode collector, and a separator. This nonaqueous lithium storage element is characterized in that the features (1) and (2) described below are satisfied at the same time with respect to the initial lithium charge/discharge characteristics of a negative electrode active material that is contained in the negative electrode active material layer. (1) The amount of charge is from 1,100 mAh/g to 2,000 mAh/g (inclusive). (2) The amount of discharge is 100 mAh/g or more at the negative electrode potential of 0-0.5 V.