Low Monomer Polyurethane Composition for Safe Adhesives

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Solution Overview

Problem

Conventional moisture-curing polyurethane compositions with isocyanate groups have high monomeric diisocyanate content, leading to health hazards and suboptimal properties such as slow curing, reduced strength, and poor adhesion, necessitating the development of formulations with low monomeric diisocyanate content and improved processing characteristics.

Innovation Solution

A moisture-curing polyurethane composition comprising a polyetherurethane polymer with low monomeric diisocyanate content, obtained through reaction with a polyether polyol and subsequent removal of excess diisocyanate, combined with a polyether having blocked hydroxyl groups as a plasticizer, achieving a monomeric diisocyanate content below 0.1% and enhanced curing and mechanical properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Object-affected harmful factors

If monomeric diisocyanate is used in excess in the preparation of the polymer and then removed by distillation, then the polymer has low viscosity and low residual monomeric diisocyanate content, but the polyurethane composition shows slow curing, reduced strength, and weaknesses in adhesion development

Engineering Contradiction:
Improvemonomeric diisocyanate contentVSAvoidtensile strength and adhesion
Core Design Contradiction:
Object-affected harmful factorsVSStrength

Solution Approach 1:

The patent changes the molecular weight parameter of the polyol component, using high molecular weight polyols (≥1000 g/mol) instead of conventional low molecular weight polyols. This parameter change allows the system to achieve low monomeric diisocyanate content while maintaining adequate strength and adhesion properties, as the higher molecular weight polyols provide better mechanical properties even at lower monomer levels.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite polymer system by reacting polyols with both monomeric diisocyanates and polymeric diisocyanates. This composite approach, where polymeric diisocyanates serve as chain extenders and crosslinking agents, enables the formulation to achieve both low residual monomer content and high mechanical strength, combining the benefits of different isocyanate types.

Inventive Principle:
Principle #40Composite materials

2Ease of operation

If monomeric diisocyanate content is reduced below 0.1%, then the composition can be safely handled without hazard labeling, but conventional formulations show slow curing and reduced strength

Engineering Contradiction:
Improvesafety and handlingVSAvoidcuring rate
Core Design Contradiction:
Ease of operationVSProductivity

Solution Approach 1:

The patent changes the molecular weight parameter of the polyol to high molecular weight (≥1000 g/mol), which fundamentally alters the curing kinetics and mechanical property development. This parameter change enables the system to cure rapidly and develop high strength even at very low monomeric diisocyanate content (<0.1%), overcoming the conventional trade-off between safety and productivity.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies different functional roles to different components locally: high molecular weight polyols provide the base polymer matrix with good mechanical properties, while polymeric diisocyanates serve specifically as chain extenders and crosslinking agents. This localized functional assignment allows the system to achieve rapid curing and high strength without relying on excess monomeric diisocyanates.

Inventive Principle:
Principle #3Local quality

3Quantity of substance

If conventional polyols are used to prepare polymers with isocyanate groups, then the polymers contain residual monomeric diisocyanate (1-3% by weight), but this creates health hazards and requires hazard labeling

Engineering Contradiction:
Improvepolymer compositionVSAvoidmonomeric diisocyanate content
Core Design Contradiction:
Quantity of substanceVSObject-affected harmful factors

Solution Approach 1:

The patent fundamentally changes the polyol molecular weight parameter to high molecular weight (≥1000 g/mol), which alters the reaction stoichiometry and polymerization kinetics. This parameter change enables the system to achieve complete reaction with very low residual monomeric diisocyanate content (<0.1%), eliminating health hazards while maintaining adequate polymer composition and properties.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent effectively extracts and removes the harmful monomeric diisocyanate component from the final polymer composition by using high molecular weight polyols and polymeric diisocyanates that react more completely and leave minimal residual monomers, thereby extracting the harmful element while preserving the functional polymer structure.

Inventive Principle:
Principle #2Taking out (Extraction)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The composition exhibits rapid curing, high tensile strength, excellent storage stability, and improved adhesion, allowing safe handling and use without hazard labeling, with properties suitable for elastic adhesives, sealants, and coatings.

Implementation Method 1

Polyurethane compositions which crosslink through reaction of isocyanate groups with moisture or water and cure to give elastomers

Methodology Applied
Scientific EffectMoisture-curing reaction: Chemical Bonding

Implementation Method 2

The polymers thus obtained, on account of chain extension reactions, contain a residual monomeric diisocyanate content

Methodology Applied
Scientific EffectChain extension reaction: Chemical Bonding

Data Source

PatentUS12129377B2Polyurethane composition having polymeric plasticizer and a low content of monomeric diisocyanates
Publication Date: 2024.10.29 SIKA TECH AG

AI summary

A moisture-curing polyurethane composition having a content of monomeric diisocyanates of at most 0.1 wt %, containing: at least one isocyanate-group-containing polyurethane polymer having a content of monomeric diisocyanates of at most 0.5 wt %, obtained from reaction of at least one monomeric diisocyanate with at least one polyether polyol at a NCO/OH ratio of at least 3/1 and subsequent removal of a large part of monomeric diisocyanates by way of a suitable separating method; and at least one polyether having blocked hydroxyl groups and free of isocyanate groups, as a plasticizer. Moisture-curing polyurethane composition is highly storage-stable when moisture is excluded, can be safely handled without special safety precautions, can be sold without hazard label, can be well processed, has long open time and has fast curing to form elastic material of high strength and extensibility, high cold flexibility, good adhesion properties and high stability with respect to heat and moisture.