Macroporous Activated Carbon Electrodes for High-Energy Supercapacitors

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Solution Overview

Problem

Electrochemical supercapacitors face high costs per kWh, limiting their widespread adoption due to high production costs compared to lithium-ion batteries, which hinders their use in various applications.

Innovation Solution

The development of carbon-based electrodes with activated carbon substrates and laser-scribed microchannels, combined with redox-active electrolytes, enhances areal and gravimetric capacitance, reducing internal resistance and increasing energy storage efficiency.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Power

If traditional supercapacitor electrodes are used, then high power density is achieved, but high cost per kWh limits widespread adoption

Engineering Contradiction:
Improvepower densityVSAvoidcost per kWh
Core Design Contradiction:
PowerVSEase of manufacture

Solution Approach 1:

The patent employs activated carbon with a highly porous structure containing macropores (larger than 50 nm) that enable efficient electrolyte penetration and ion transport. This porous architecture increases the effective surface area for charge storage while maintaining low material cost, resolving the contradiction between achieving high power density and reducing cost per kWh

Inventive Principle:
Principle #31Porous materials

Solution Approach 2:

The patent creates a composite electrode structure combining activated carbon particles with a conductive matrix material. This composite approach enhances electrical conductivity and mechanical stability while utilizing cost-effective materials, allowing high power density performance without the high costs associated with traditional supercapacitor materials

Inventive Principle:
Principle #40Composite materials

2Quantity of substance

If electrode density is increased to improve energy density, then more energy is stored, but ionic impedance increases reducing charge/discharge speed

Engineering Contradiction:
Improveenergy densityVSAvoidionic impedance
Core Design Contradiction:
Quantity of substanceVSObject-generated harmful factors

Solution Approach 1:

The patent utilizes activated carbon with a hierarchical porous structure that includes macropores (>50 nm) serving as ion transport highways. These large pores reduce ionic impedance by facilitating rapid electrolyte flow and ion access to the electrode interior, while the overall high porosity provides extensive surface area for energy storage, thus increasing energy density without compromising charge/discharge kinetics

Inventive Principle:
Principle #31Porous materials

Solution Approach 2:

The patent introduces a three-dimensional macroporous network architecture that adds spatial dimensionality to ion transport pathways. This 3D porous structure enables ions to access deep within the electrode through multiple dimensional pathways, reducing the tortuosity and resistance that would otherwise limit fast charging while maintaining high energy density

Inventive Principle:
Principle #17Another dimension (Dimensionality change)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach results in high-energy density storage devices with improved performance, reduced costs, and extended cycle stability, making them viable alternatives to traditional batteries in various applications.

Implementation Method 1

generating a light beam having a power density to generate one or more channels in the activated carbon substrate

Methodology Applied
Scientific EffectLaser ablation: Laser Ablation

Implementation Method 2

activated carbon substrate comprises activated carbon, activated charcoal, activated carbon cloth, activated carbon fiber, activated glassy carbon, activated carbon nanofoam, activated carbon aerogel

Methodology Applied
Scientific EffectAdsorption: Adsorption

Data Source

PatentEP3558876B1Methods, devices and systems for activated carbon supercapacitors with macroporous electrodes
Publication Date: 2023.10.11 RGT UNIV OF CALIFORNIA
  • EP3558876B1 patent drawingFigure 1A~1D
  • EP3558876B1 patent drawingFigure 2A~2D
  • EP3558876B1 patent drawingFigure 3A~3F

AI summary

Energy storage devices comprising carbon-based electrodes and/or redox electrolytes are disclosed herein. In some embodiments, the carbon-based electrodes comprise laser-scribed activated carbon comprising one or more micro-channels. In some embodiments, the redox electrolytes comprise a ferricyanide/ferrocyanide redox couple. Also described are processes, methods, protocols and the like for manufacturing carbon- based electrodes comprising micro-channels for use in high energy storage devices such as supercapacitors, and for manufacturing high energy storage devices comprising redox electrolytes.