Magnesium Stearate Stabilized Dry Powder Inhalation Formulation

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Solution Overview

Problem

Current PI3 kinase inhibitors for inhalation therapy face challenges in achieving stable and reproducible chemical and physical properties, particularly in dry powder formulations, which are essential for effective delivery of therapeutic compounds like the compound of formula (I) for treating inflammatory diseases such as COPD and asthma, due to susceptibility to oxidative degradation and hydrolytic cleavage.

Innovation Solution

Incorporating a particulate stabilizing agent, such as metal salts of stearic acid or stearyl fumarate, specifically magnesium stearate, alongside particulate lactose in the dry powder formulation to enhance the chemical and physical stability of the compound of formula (I), thereby protecting it from metal-catalyzed oxidative degradation and hydrolytic cleavage.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of operation

If the compound of formula (I) is formulated in dry powder for inhalation, then it can be delivered effectively to treat inflammatory diseases, but it becomes susceptible to oxidative degradation and hydrolytic cleavage, compromising chemical stability

Engineering Contradiction:
Improveinhalation deliveryVSAvoidchemical stability
Core Design Contradiction:
Ease of operationVSStability of the object's composition

Solution Approach 1:

Magnesium stearate acts as an intermediary substance between the compound of formula (I) and the degrading environment. It forms a protective interface that prevents direct contact with oxidizing agents and water, thereby reducing oxidative degradation and hydrolytic cleavage while maintaining inhalation delivery capability

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The formulation creates a microenvironment around the compound of formula (I) that is chemically inert to oxidation and hydrolysis. Magnesium stearate provides this protective atmosphere by forming a barrier layer that excludes reactive species and moisture, allowing the compound to remain stable during storage and administration

Inventive Principle:
Principle #39Inert atmosphere (Inert environment)

2Stability of the object's composition

If metal salts of stearic acid or stearyl fumarate are added to enhance chemical stability, then oxidative degradation and hydrolytic cleavage are reduced, but the formulation complexity increases

Engineering Contradiction:
Improvechemical stabilityVSAvoidformulation complexity
Core Design Contradiction:
Stability of the object's compositionVSDevice complexity

Solution Approach 1:

The invention optimizes the concentration of magnesium stearate within a specific range (0.1-10% w/w) to achieve effective stabilization without excessive complexity. This parameter optimization allows the formulation to maintain chemical stability while keeping the composition relatively simple and manageable

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The formulation demonstrates improved chemical and physical stability, as evidenced by reduced degradation products and maintained peak characteristics, ensuring predictable and reproducible therapeutic efficacy when administered via inhalation.

Implementation Method 1

susceptibility to oxidative degradation and hydrolytic cleavage

Methodology Applied
Scientific EffectOxidative degradation: Oxidation

Implementation Method 2

susceptibility to oxidative degradation and hydrolytic cleavage

Methodology Applied
Scientific EffectHydrolytic cleavage: Hydrolysis

Data Source

PatentEP2825202B1Stabilization of pharmaceutical compositions
Publication Date: 2017.09.06 RESPIVERT
  • EP2825202B1 patent drawingFigure 1
  • EP2825202B1 patent drawingFigure 2
  • EP2825202B1 patent drawingFigure 3

AI summary

There is provided inter alia a dry powder pharmaceutical formulation for inhalation comprising: (i) 6-(2-((4-amino-3-(3-hydroxyphenyl)-1 H-pyrazolo[3,4-d]pyrimidin-1-yl) methyl)-3- (2-chlorobenzyl)-4-oxo-3,4-dihydroquinazolin-5-yl)-N, N-bis(2-methoxyethyl)hex-5- ynamide or a pharmaceutically acceptable salt thereof, including all stereoisomers, tautomers and isotopic derivatives thereof and solvates thereof in particulate form as active ingredient; (ii) particulate lactose as carrier; and (iii) a particulate stabilizing agent selected from metal salts of stearic acid such as magnesium stearate and metal salts of stearyl fumarate.