MDI Purification Distillation Column with Subcooled Condenser

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Solution Overview

Problem

Current methods for purifying methylene diphenyl diisocyanate (MDI) isomers, such as those using multiple distillation columns or melt crystallization, are costly and inefficient, with high dimer content leading to fouling and poor product quality due to fine crystal formation and energy loss.

Innovation Solution

A plant with a distillation apparatus featuring a structured packing distillation column, overhead vapor condenser that subcools condensate to less than 47°C, and a flow-controlled reflux system that reheats condensate to 190°C, reducing dimer formation and fouling, and optionally followed by dynamic crystallization for further purification.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If multiple distillation columns are used for purifying MDI isomers, then purification effectiveness is improved, but device complexity and operation costs increase

Engineering Contradiction:
Improvepurification effectivenessVSAvoidnumber of distillation columns
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The distillation column is segmented into multiple functional sections with different packing types (structured packing in rectifying section, random packing in stripping section) to achieve separation functions that would otherwise require multiple columns, thereby reducing device complexity while maintaining purification effectiveness

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

A single distillation column performs multiple functions: rectification, stripping, and product purification, replacing the need for multiple specialized columns. The column handles both light component removal and heavy component separation in one integrated unit

Inventive Principle:
Principle #6Universality (Multi-functionality)

2Quantity of substance

If high dimer content is present in the crude mixture, then feedstock availability is improved, but fouling and operation difficulties increase

Engineering Contradiction:
Improvefeedstock availabilityVSAvoidfouling
Core Design Contradiction:
Quantity of substanceVSObject-affected harmful factors

Solution Approach 1:

The invention changes operational parameters including temperature profile control, pressure conditions, and reflux ratio optimization to prevent dimer deposition and fouling in the distillation column, enabling processing of feedstock with higher dimer content without operational difficulties

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The presence of dimers in the feedstock is converted from a harmful factor into an acceptable condition by designing the distillation process to handle and manage dimer content, transforming the limitation into a manageable parameter that does not prevent high-yield production

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

3Use of energy by moving object

If conventional distillation is used without subcooling, then energy consumption is reduced, but dimer formation and fouling increase

Engineering Contradiction:
Improveenergy consumptionVSAvoiddimer formation
Core Design Contradiction:
Use of energy by moving objectVSObject-generated harmful factors

Solution Approach 1:

The condensate is subcooled below its dew point before entering the distillation column, performing preliminary cooling that prevents dimer formation in subsequent processing stages, thereby reducing fouling without significant additional energy consumption

Inventive Principle:
Principle #10Preliminary action

4Manufacturing precision

If melt crystallization is used to increase 4,4'-MDI content, then product purity is improved, but fine crystal formation and operation complexity increase

Engineering Contradiction:
Improve4,4'-MDI contentVSAvoidcrystallization process complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The invention replaces mechanical crystallization processes with a optimized distillation approach using structured packing, achieving high 4,4'-MDI content through enhanced mass transfer and separation efficiency rather than through crystallization mechanics, thereby simplifying the overall process

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution achieves a dimer content of less than 200 ppm, reducing fouling and enabling efficient further purification, with lower operation costs and improved product quality, including high purity and reduced color and chloride content.

Implementation Method 1

the overhead vapor condenser comprises a shell and tube arrangement and is preferably embodied so as to directly subcool the condensate to less than 47°C

Methodology Applied
Scientific EffectHeat exchange: Heat Exchanger

Implementation Method 2

the flow-controlled reflux system comprises a heater, which is preferably embodied so as to reheat a partial stream of the condensate formed in the overhead vapor condenser up to 190 °C

Methodology Applied
Scientific EffectHeating: Heating

Implementation Method 3

A typical method for purifying a crude MOl mixture is a distillation performed with two or more distillation columns

Methodology Applied
Scientific EffectDistillation: Distillation

Data Source

PatentEP3697756B1A plant and method for purifying an isomeric monomer, such as 4,4'-methylene diphenyl diisocyanate, from a crude mixture
Publication Date: 2023.06.14 SULZER MANAGEMENT AG
  • EP3697756B1 patent drawingFigure 1
  • EP3697756B1 patent drawingFigure 2
  • EP3697756B1 patent drawingFigure 3

AI summary

The present invention relates to a plant for preparing a purified isomeric methylene diphenyl diisocyanate monomer from a mixture of different isomeric monomers, wherein the plant comprises a distillation apparatus, which comprises: a) a distillation column including a structured packing, b) a source for a mixture of different isomeric methylene diphenyl diisocyanate monomers, c) an evaporator, d) an overhead vapor condenser, e) optionally, an overhead vacuum system and f) a flow-controlled reflux system, wherein the overhead vapor condenser comprises a shell and tube arrangement and is embodied so as to directly subcool the condensate to less than 47°C, and wherein the flow-controlled reflux system comprises a heater, which is embodied so as to reheat a partial stream of the condensate formed in the overhead vapor condenser up to 190 °C.