MEA Combined Roll Structure to Prevent Bonding Wrinkles

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Solution Overview

Problem

In roll-to-roll systems for manufacturing polymer electrolyte fuel cells, the polymer electrolyte membrane and gasket member often overlap excessively, leading to wrinkles during thermocompression bonding, which can cause gas leakage and increase manufacturing costs due to the use of unnecessary membrane material.

Innovation Solution

A combined roll design featuring a wound strip with layered bodies of polymer electrolyte membranes and electrode catalyst layers, where the polymer electrolyte membrane has an outer periphery extending beyond the catalyst layers, supported by frame units with an attachment member to join adjacent units, reducing material usage and preventing excessive overlap.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If the polymer electrolyte membrane is made continuous in the longitudinal direction for roll-to-roll manufacturing, then mass production efficiency is improved, but material waste increases due to excessive overlap with the gasket member

Engineering Contradiction:
Improvemass production efficiencyVSAvoidpolymer electrolyte membrane material waste
Core Design Contradiction:
ProductivityVSLoss of substance

Solution Approach 1:

The polymer electrolyte membrane is segmented into individual membrane electrode assemblies rather than being continuous. Each MEA is cut separately from the belt, allowing precise control of membrane dimensions and elimination of excessive overlap with gasket members, thereby reducing material waste while maintaining roll-to-roll manufacturing efficiency

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The membrane electrode assemblies are prepared in advance on a belt with precise positioning of the polymer electrolyte membrane relative to the gasket member. This preliminary arrangement allows for optimized material usage before the final cutting and assembly steps

Inventive Principle:
Principle #10Preliminary action

2Strength

If the polymer electrolyte membrane and gasket member overlap in a large area, then structural reinforcement is improved, but wrinkles occur during thermocompression bonding

Engineering Contradiction:
Improvestructural reinforcementVSAvoidwrinkle formation during bonding
Core Design Contradiction:
StrengthVSManufacturing precision

Solution Approach 1:

The overlap area between the polymer electrolyte membrane and gasket member is precisely controlled by adjusting the dimensions and positioning parameters. The membrane is sized to provide sufficient reinforcement while limiting the overlap to a range that prevents wrinkle formation during thermocompression bonding of the gas diffusion layer

Inventive Principle:
Principle #35Parameter changes

3Loss of substance

If the polymer electrolyte membrane outer periphery width is reduced to minimize material usage, then manufacturing cost decreases, but adhesion between the gasket member and membrane may be insufficient

Engineering Contradiction:
Improvepolymer electrolyte membrane material usageVSAvoidadhesion between gasket member and membrane
Core Design Contradiction:
Loss of substanceVSReliability

Solution Approach 1:

The width of the polymer electrolyte membrane outer periphery is optimized to a specific range that provides sufficient adhesion area for the gasket member while minimizing material consumption. This parameter optimization ensures both reliable bonding and cost-effectiveness

Inventive Principle:
Principle #35Parameter changes

4Manufacturing precision

If the membrane electrode assembly is produced one at a time using sheet-to-sheet system, then manufacturing precision is improved, but productivity decreases

Engineering Contradiction:
Improveassembly precisionVSAvoidproduction speed
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

Multiple membrane electrode assemblies are manufactured simultaneously on a single belt in the roll-to-roll system. The process combines the advantages of continuous high-speed production with precise positioning and cutting techniques that maintain assembly precision, effectively merging the benefits of both sheet-to-sheet and continuous manufacturing approaches

Inventive Principle:
Principle #5Merging (Combining)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This design facilitates efficient storage and transportation of membrane electrode assemblies, reduces material usage, minimizes wrinkles during bonding, and prevents gas leakage, thereby lowering production costs and maintaining fuel cell performance.

Implementation Method 1

The protons are transferred by the polymer electrolyte contained in the electrode catalyst layer and the polymer electrolyte membrane, and migrate through the polymer electrolyte membrane to the air electrode

Methodology Applied
Scientific EffectIon conduction: Conduction (electrical)

Implementation Method 2

The gasket member reinforces the membrane electrode assembly composed mainly of the polymer electrolyte membrane, which has low rigidity

Methodology Applied
Scientific EffectMechanical support: Mechanical Force

Implementation Method 3

a plurality of frame units arranged in a single direction, the plurality of frame units each supporting one of the layered bodies, and an attachment member that joins adjacent ones of the frame units together

Methodology Applied
Scientific EffectAdhesion: Adhesive

Data Source

PatentUS20230411660A1Membrane electrode assembly combined roll, membrane electrode assembly, and polymer electrolyte fuel cell
Publication Date: 2023.12.21 TOPPAN INC
  • US20230411660A1 patent drawing
  • US20230411660A1 patent drawing
  • US20230411660A1 patent drawing

AI summary

A combined roll is a roll of a wound strip that includes a plurality of layered bodies each including a polymer electrolyte membrane and a pair of electrode catalyst layers, and a supporting member including a plurality of frame units arranged in a single direction, with each frame unit supporting one layered body. The frame unit surrounds the electrode catalyst layers and is in contact with the electrode catalyst layers, with the outer periphery of the polymer electrolyte membrane held inside the frame unit in the thickness direction.