Mesh Target Ion Source for Mass Spectrometry Spray Convergence

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Solution Overview

Problem

Existing multimode ion sources for mass spectrometry are mechanically complex and suffer from lower sensitivities due to divergent spray geometries, which hinder efficient ionization of analyte mixtures with a wide range of polarities.

Innovation Solution

An ion source design featuring a nebuliser that emits a high-density droplet stream with a close-coupled impactor target, optimizing the spray tip and target proximity to minimize beam divergence and enhance ionization efficiency, utilizing a mesh or grid target to deflect and ionize droplets effectively.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Area of stationary object

If a broad area charged target plate is used in SACI ion source, then the ionization area is increased, but the spray becomes divergent and sensitivity decreases

Engineering Contradiction:
Improvetarget plate areaVSAvoidspray convergence
Core Design Contradiction:
Area of stationary objectVSManufacturing precision

Solution Approach 1:

The patent segments the target into multiple wire meshes arranged in parallel, creating multiple discrete ionization zones instead of a single broad area target. This segmentation maintains a compact target geometry that preserves spray convergence while providing sufficient ionization area through the distributed wire mesh structure.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent transitions from a two-dimensional broad area target plate to a three-dimensional wire mesh structure with wires arranged in parallel at specific spacing. This dimensional change creates multiple ionization pathways while maintaining a compact footprint, preserving spray convergence.

Inventive Principle:
Principle #17Another dimension (Dimensionality change)

2Adaptability or versatility

If ESI and APCI are combined in multimode ion source, then ionization capability for wide polarity range is improved, but mechanical complexity increases

Engineering Contradiction:
Improveionization capabilityVSAvoidmechanical complexity
Core Design Contradiction:
Adaptability or versatilityVSDevice complexity

Solution Approach 1:

The patent creates a universal ionization system where the wire mesh target serves multiple functions: it provides ionization for both polar and non-polar analytes, replaces the need for separate ESI and APCI systems, and maintains a simple mechanical structure throughout.

Inventive Principle:
Principle #6Universality (Multi-functionality)

Solution Approach 2:

The patent merges the ionization capabilities for different polarity analytes into a single wire mesh target system, eliminating the need for separate ESI and APCI ion sources and their associated complex mechanical structures.

Inventive Principle:
Principle #5Merging (Combining)

3Length of stationary object

If spray tip to target distance is increased, then ionization area is increased, but beam divergence increases and sensitivity decreases

Engineering Contradiction:
Improvespray tip to target distanceVSAvoidbeam convergence
Core Design Contradiction:
Length of stationary objectVSManufacturing precision

Solution Approach 1:

The patent applies local quality by creating multiple localized ionization zones along the wire mesh structure. Each wire or group of wires creates a focused ionization region, ensuring that even though the target has extended area, the local spray-to-target geometry remains optimized for convergence.

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This design achieves higher sensitivity and efficient ionization of both high and low polarity analytes without the need to switch ionization techniques, improving the overall performance of mass spectrometry by increasing spray flux and reducing beam dispersion.

Implementation Method 1

droplets are ionised by impact on a mesh or grid target

Methodology Applied
Scientific EffectImpact ionization: Ionisation

Data Source

PatentEP2912679B1Improved reproducibility of impact-based ionization source for low and high organic mobile phase compositions using a mesh target
Publication Date: 2018.01.17 MICROMASS UK LTD
  • EP2912679B1 patent drawingFigure 1
  • EP2912679B1 patent drawingFigure 2(a)~3
  • EP2912679B1 patent drawingFigure 4~5

AI summary

An ion source is disclosed comprising one or more nebulisers and one or more mesh or grid targets (20). The one or more nebulisers are arranged and adapted to emit, in use, a stream predominantly of droplets which are caused to impact upon the one or more mesh or grid targets (20) and to ionise the droplets to form a plurality of ions.