Metal Oxide Shell Microcapsules for Dense Encapsulation

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Solution Overview

Problem

Current methods for preparing microcapsules with water-insoluble core materials face challenges in achieving a thick and dense metal oxide shell, which is essential for effective encapsulation and targeted delivery of active ingredients in pharmaceutical, cosmetic, and agricultural applications.

Innovation Solution

A process involving the preparation of an oil-in-water emulsion with a sol-gel precursor and metal oxide nanoparticles, where the nanoparticles are incorporated into the aqueous phase to form a dense metal oxide shell around the core material, enabling the creation of microcapsules with a shell thickness in the range of 0.1-10 microns.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional methods are used to prepare microcapsules with water-insoluble core materials, then the encapsulation process is simpler, but the metal oxide shell cannot achieve sufficient thickness and density

Engineering Contradiction:
Improveshell thickness and densityVSAvoidprocess complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

Metal oxide nanoparticles are incorporated into the aqueous phase before or during emulsion formation, allowing them to be pre-positioned at the oil-water interface where the shell will form. This preliminary action enables the nanoparticles to serve as nucleation sites for subsequent metal oxide deposition, facilitating thick and dense shell formation without requiring complex post-processing steps

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The shell is formed as a composite structure combining metal oxide nanoparticles with sol-gel derived metal oxide matrix. This composite approach allows the nanoparticles to provide structural framework and the sol-gel process to fill interstices and create a dense, thick shell with enhanced mechanical properties and controlled porosity

Inventive Principle:
Principle #40Composite materials

2Reliability

If a thick and dense metal oxide shell is formed, then encapsulation effectiveness and targeted delivery are improved, but the manufacturing process becomes more complex

Engineering Contradiction:
Improveencapsulation effectivenessVSAvoidprocess complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The sol-gel precursor acts as an intermediary that bridges the metal oxide nanoparticles and the final dense shell structure. The sol-gel process provides a controlled chemical pathway for metal oxide formation that fills gaps between nanoparticles and creates a continuous dense matrix, ensuring reliable encapsulation while maintaining process simplicity through a single-step chemical transformation

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The pH of the aqueous phase is controlled and adjusted to optimize the sol-gel hydrolysis and condensation reactions. By adjusting pH parameters, the process controls the rate and extent of metal oxide formation, ensuring complete shell formation with desired thickness and density while maintaining straightforward process conditions without requiring multiple complex processing steps

Inventive Principle:
Principle #35Parameter changes

3Manufacturing precision

If metal oxide nanoparticles are incorporated into the emulsion, then a dense shell is formed, but the process steps increase

Engineering Contradiction:
Improveshell densityVSAvoidprocess efficiency
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The incorporation of metal oxide nanoparticles into the aqueous phase is combined with the emulsion formation step itself, rather than being a separate sequential operation. The nanoparticles are mixed with the aqueous phase and then both phases are emulsified together in a single homogenization process, achieving shell formation and emulsion creation simultaneously to maintain high productivity

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The metal oxide nanoparticles automatically self-assemble and self-organize at the oil-water interface during emulsion formation, driven by interfacial energy minimization and hydrophobic interactions. This self-organization eliminates the need for complex external guidance or positioning mechanisms, maintaining process simplicity while achieving dense shell structure through spontaneous nanoparticle arrangement

Inventive Principle:
Principle #25Self-service

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach results in microcapsules that provide effective encapsulation and targeted delivery of active ingredients, enhancing their stability and bioavailability for applications in dermatological treatments and pest control, while allowing for controlled release and improved skin or mucosal membrane penetration.

Implementation Method 1

wherein one or both of the oily phase, and the aqueous phase comprises a sol-gel precursor

Methodology Applied
Scientific EffectSol-gel hydrolysis and polymerization: Hydrolysis

Implementation Method 2

preparing an oil-in-water emulsion by emulsification of an oily phase that comprises a core material, in an aqueous phase

Methodology Applied
Scientific EffectEmulsion formation: Emulsion

Data Source

PatentUS10688462B2Microcapsules comprising active ingredients and a metal oxide shell, a method for their preparation and uses thereof
Publication Date: 2020.06.23 MAYNE PHARMA LLC

AI summary

The present invention provides a process for preparing microcapsules comprising a core material encapsulated by a metal oxide shell, microcapsules obtained therewith and uses thereof.