Metal-Resist Cleaning Liquid With Liquid Strong Acid

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Solution Overview

Problem

Existing cleaning liquids for metal resists in semiconductor processing face challenges in effectively removing metal residues while preventing organic substance contamination and precipitation during drying, particularly when using solid acids like oxalic acid.

Innovation Solution

A cleaning liquid comprising a solvent and a liquid strong acid with a pH of 2.5 or less, preferably using organic solvents like propylene glycol methyl ethyl acetate and strong acids such as phosphoric acid, which are liquid at 20°C, to enhance metal removal properties and prevent organic residue formation.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If a solid acid such as oxalic acid or benzenesulfonic acid is used in the cleaning liquid, then metal removing properties are improved, but the solid acid precipitates when the cleaning liquid is dried, causing organic substance to remain on the treated surface and contaminating the process apparatus

Engineering Contradiction:
Improvemetal removing propertiesVSAvoidorganic substance residual amount
Core Design Contradiction:
Manufacturing precisionVSObject-generated harmful factors

Solution Approach 1:

The patent changes the physical state parameter of the acid from solid to liquid by selecting liquid strong acids (sulfuric acid, phosphoric acid, methanesulfonic acid, trifluoroacetic acid) that remain liquid at 20°C. This parameter change prevents precipitation during drying while maintaining the strong acid's metal removal capability, thereby eliminating organic substance residue and apparatus contamination.

Inventive Principle:
Principle #35Parameter changes

2Object-generated harmful factors

If a liquid acid such as acetic acid is used instead of a solid acid to prevent precipitation at the time of drying, then organic substance residual amount is reduced, but metal removing properties are insufficient compared to when a solid acid is used

Engineering Contradiction:
Improveorganic substance residual amountVSAvoidmetal removing properties
Core Design Contradiction:
Object-generated harmful factorsVSManufacturing precision

Solution Approach 1:

The patent changes the acid strength parameter by selecting liquid strong acids with low pKa values (sulfuric acid pKa: -3, phosphoric acid pKa: 2.1, methanesulfonic acid pKa: 0.4, trifluoroacetic acid pKa: 0.5) instead of weak liquid acids like acetic acid (pKa: 4.76). This parameter change maintains strong metal removal capability while preventing precipitation, achieving both high metal removing properties and low organic substance residue.

Inventive Principle:
Principle #35Parameter changes

3Manufacturing precision

If the pH value of the cleaning liquid is lowered to enhance metal removal, then metal removing properties are improved, but the risk of apparatus contamination increases due to precipitation

Engineering Contradiction:
Improvemetal removing propertiesVSAvoidapparatus contamination risk
Core Design Contradiction:
Manufacturing precisionVSReliability

Solution Approach 1:

The patent changes the physical state parameter of the acid component from solid to liquid, enabling the use of strong acids at low pH values (pH ≤ 2.5 after 10-fold dilution) without causing precipitation. This parameter change allows aggressive metal removal while eliminating the contamination risk associated with solid acid precipitation during the drying process.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution provides improved metal removal efficiency with reduced organic residue and prevents apparatus contamination, ensuring effective cleaning of metal resists without precipitation.

Implementation Method 1

a strong acid that is liquid at 20° C., in which a pH value, which is measured with a pH meter, of a liquid formed by subjecting the cleaning liquid to a 10-fold dilution with pure water is 2.5 or less

Methodology Applied
Scientific EffectAcid dissociation: Electrolyte

Data Source

PatentUS12428737B2Cleaning liquid used for cleaning metal resists, and cleaning method using cleaning liquid
Publication Date: 2025.09.30 TOKYO OHKA KOGYO CO LTD

AI summary

A metal resist remover containing a solvent and a strong acid that is liquid at 20° C., in which a pH value, which is measured with a pH meter, of a liquid formed by subjecting the cleaning liquid to a 10-fold dilution with pure water is 2.5 or less.