Methacrylic Acid Purification via Aqueous Cooling and Phase Separation

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Solution Overview

Problem

Current methods for producing methacrylic acid result in low yields and high production costs, with a need for improved yield, purity, and plant service life, while minimizing the formation of undesired by-products.

Innovation Solution

A process involving the reaction of methacrylamide with water in a tubular reactor, where the reaction mixture is cooled and separated, utilizing a pressure difference and controlled temperature to enhance yield and purity, and incorporating additives like sulfuric acid and polymerization inhibitors to prevent by-product formation.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If the reaction mixture is cooled by mixing with an aqueous medium and then fed into a phase separator, then the yield and purity of methacrylic acid are improved, but the device complexity increases due to additional cooling and separation equipment

Engineering Contradiction:
ImproveyieldVSAvoiddevice complexity
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The process is divided into distinct functional stages: reaction zone, cooling zone with aqueous medium mixing, and phase separation zone. Each stage is separated into different equipment components (reactor, cooler/mixer, phase separator), allowing independent optimization of each function while achieving high yield and purity through systematic separation of the reaction mixture into organic and aqueous phases

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

An aqueous medium is introduced as an intermediary substance to cool the reaction mixture and facilitate phase separation. The aqueous medium acts as a mediator that transfers heat from the reaction mixture while enabling the separation of methacrylic acid (organic phase) from by-products and unreacted materials (aqueous phase), thereby improving purity without directly participating in the main reaction

Inventive Principle:
Principle #24Intermediary (Mediator)

2Manufacturing precision

If the reaction mixture is cooled by mixing with an aqueous medium and then fed into a phase separator, then the purity of methacrylic acid is improved, but the device complexity increases due to additional cooling and separation equipment

Engineering Contradiction:
ImprovepurityVSAvoiddevice complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The process is divided into distinct functional stages: reaction zone, cooling zone with aqueous medium mixing, and phase separation zone. Each stage is separated into different equipment components (reactor, cooler/mixer, phase separator), allowing independent optimization of each function while achieving high yield and purity through systematic separation of the reaction mixture into organic and aqueous phases

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

An aqueous medium is introduced as an intermediary substance to cool the reaction mixture and facilitate phase separation. The aqueous medium acts as a mediator that transfers heat from the reaction mixture while enabling the separation of methacrylic acid (organic phase) from by-products and unreacted materials (aqueous phase), thereby improving purity without directly participating in the main reaction

Inventive Principle:
Principle #24Intermediary (Mediator)

3Object-generated harmful factors

If sulfuric acid and polymerization inhibitors are added to prevent by-product formation, then the formation of unwanted by-products is minimized, but the manufacturing cost increases due to additional chemicals

Engineering Contradiction:
Improveby-product formationVSAvoidmanufacturing cost
Core Design Contradiction:
Object-generated harmful factorsVSEase of manufacture

Solution Approach 1:

The harmful effects (by-product formation) are addressed by extracting and removing them through phase separation. The aqueous phase is specifically designed to contain and remove by-products, unreacted methacrylamide, and other harmful substances, separating them from the desired methacrylic acid in the organic phase. This extraction approach is more effective and cost-efficient than attempting to prevent all by-products through chemical additives

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The process optimizes parameters such as temperature, pressure, and aqueous medium composition to control the reaction and separation processes. By carefully controlling these parameters, the system achieves high purity product with minimal by-products, reducing the need for extensive chemical additives and lowering overall manufacturing costs

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This process achieves a higher yield and purity of methacrylic acid, extends the service life of the production plant, and reduces the formation of unwanted by-products, leading to a more cost-effective and efficient production method.

Implementation Method 1

the reaction mixture obtained by reacting methacrylamide with water is cooled by mixing it with an aqueous medium

Methodology Applied
Scientific EffectHeat transfer: Conduction (thermal)

Implementation Method 2

fed into a phase separator. Here, an aqueous phase is separated from an organic phase

Methodology Applied
Scientific EffectPhase separation: Density Gradient

Implementation Method 3

the reaction of the methacrylamide with water can take place

Methodology Applied
Scientific EffectHydrolysis: Hydrolysis

Data Source

PatentEP2265567B1Method for purifying methacrylic acid
Publication Date: 2018.08.01 ROHM GMBH
  • EP2265567B1 patent drawingFigure 1
  • EP2265567B1 patent drawingFigure 2
  • EP2265567B1 patent drawingFigure 3

AI summary

The present invention relates to a method for purifying methacrylic acid, wherein the reaction mixture, which is obtained by reacting methacrylamide with water, is cooled by mixing with an aqueous medium and subsequently conducted into a phase separator. Furthermore, the present invention discloses a facility for carrying out the method according to the invention.