Methanation Reactor Liquid Water Injection Cooling

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Solution Overview

Problem

Current methanation reactors face challenges in efficiently cooling the reaction, leading to high manufacturing costs, non-optimized space utilization, and premature catalyst deactivation due to coke and carbonyl formation, with existing systems failing to effectively manage heat exchange and catalyst toxicity.

Innovation Solution

A methanation reactor design that introduces water in the liquid phase into the fluidized bed, where it vaporizes and participates in the reaction, reducing coke and carbonyl formation, and utilizes a water recycling system to optimize temperature control and heat exchange, allowing for efficient production of methane and thermal energy.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Loss of energy

If throughwall cooled reactors with reactor walls cooled by cooling fluid are used, then heat exchange is achieved, but the surface areas required for heat exchange are large and reactor manufacturing costs are high

Engineering Contradiction:
Improveheat removal efficiencyVSAvoidreactor manufacturing cost
Core Design Contradiction:
Loss of energyVSEase of manufacture

Solution Approach 1:

The patent uses a fluidized bed of catalytic particles that creates a porous, highly surface-area structure. This fluidized bed acts as an extended heat exchange surface throughout the reactor volume, eliminating the need for large external heat exchange surfaces while maintaining efficient heat removal through the natural circulation of particles and cooling gas.

Inventive Principle:
Principle #31Porous materials

Solution Approach 2:

The invention transitions from two-dimensional heat exchange through reactor walls to three-dimensional heat exchange distributed throughout the entire reactor volume. The fluidized bed particles provide heat exchange surfaces in all spatial dimensions, dramatically increasing the effective heat transfer area without increasing reactor external dimensions.

Inventive Principle:
Principle #17Another dimension (Dimensionality change)

2Loss of energy

If thermal oil is circulated through heat exchangers in fluidized bed systems, then heat transfer coefficients are high, but the use of thermal oils is limited to reaction temperatures of around 380°C to 400°C

Engineering Contradiction:
Improveheat transfer coefficientVSAvoidtemperature range
Core Design Contradiction:
Loss of energyVSAdaptability or versatility

Solution Approach 1:

The patent changes the physical state parameter of the cooling medium from liquid thermal oil to gaseous cooling fluid. This parameter change enables operation across a much wider temperature range, as gases can withstand higher temperatures without degradation, while still maintaining effective heat transfer through the fluidized bed's enhanced convection and large surface area.

Inventive Principle:
Principle #35Parameter changes

3Temperature

If water is injected above the catalytic bed to cool the reaction, then cooling is achieved, but coke and carbonyl formation is not limited

Engineering Contradiction:
Improvereaction temperature controlVSAvoidcoke and carbonyl formation
Core Design Contradiction:
TemperatureVSObject-generated harmful factors

Solution Approach 1:

The patent introduces water at the bottom of the reactor before the gas phase reactants enter the catalytic bed. This preliminary action ensures that water is already present in vapor form and distributed throughout the bed, creating a protective atmosphere that prevents coke and carbonyl formation on the catalyst surfaces before harmful reactions can occur.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

Water vapor acts as an intermediary substance that mediates between the cooling function and the catalyst protection function. By introducing water at the bottom, it serves dual purposes: cooling the reaction through evaporation and preventing harmful side reactions by maintaining a water-rich environment around the catalyst particles.

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This design reduces reactor size, minimizes carbonyl formation, and enhances catalyst longevity by vaporizing water within the reactor, optimizing temperature control and heat exchange, resulting in improved yield and reduced manufacturing costs while ensuring efficient cooling and thermal energy co-generation.

Implementation Method 1

the injected water is vaporized upon contact with the hot bed

Methodology Applied
Scientific EffectEvaporation: Evaporation

Implementation Method 2

the injected water is vaporized upon contact with the hot bed

Methodology Applied
Scientific EffectLatent heat: Latent Heat

Implementation Method 3

A fluidized catalyst bed helps to homogenize the temperature of the reactive zone

Methodology Applied
Scientific EffectFluidization: Fluidisation

Implementation Method 4

Methanation is an industrial process of catalytic conversion of hydrogen and carbon monoxide or carbon dioxide into methane

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 5

a means (125) for condensing water vapor present downstream of the methane and water outlet

Methodology Applied
Scientific EffectCondensation: Condensation

Data Source

PatentEP3049181B1Methanation reactor for reacting hydrogen with at least one carbon-based compound and producing methane and water
Publication Date: 2020.11.18 GDF SUEZ SA
  • EP3049181B1 patent drawingFigure 1
  • EP3049181B1 patent drawingFigure 2

AI summary

The invention relates to a methanation reactor (10) for reacting dihydrogen with at least one carbon-based compound and producing methane, comprising: a hollow body (105) designed to receive a fluidised bed of catalytic particles (106) and comprising an inlet (110) for each carbon-based compound and for dihydrogen and an outlet (115) for methane and water. The reactor is characterised in that it also comprises an inlet (120) for the injection of liquid-phase cooling water into the fluidised bed. In certain embodiments, each carbon-based compound is a gas, the reactor comprising at least one water-injection nozzle and at least one injection nozzle for a gas comprising the carbon-based gas and dihydrogen, at least one water-injection nozzle being positioned below at least one gas-injection nozzle. In certain embodiments, the flow rate of water introduced into the hollow body depends on the temperature measured in the reactor.