Methanol Synthesis Gas Compression with Recycle Integration

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Solution Overview

Problem

Current methanol production processes face challenges with high energy consumption for gas compressors, increased system parts and costs, hydrogen losses, catalyst deactivation due to high water partial pressure, and high recirculation rates of synthesis gas, especially with high CO2 content, leading to increased investment and operating costs.

Innovation Solution

A process involving a feed gas with at least 80% carbon dioxide, pre-compression of fresh gas, and subsequent compression with recycle gas to synthesis pressure in multiple reactor stages, where unreacted synthesis gas is recycled directly to the compressor stage without additional compression, reducing recirculation and compressor power, and optimizing stoichiometry to minimize hydrogen usage.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If high recirculation rates are used to achieve high conversion with high CO2 content synthesis gas, then conversion efficiency is improved, but energy consumption and operating costs increase significantly

Engineering Contradiction:
Improveconversion efficiencyVSAvoidenergy consumption
Core Design Contradiction:
ProductivityVSUse of energy by moving object

Solution Approach 1:

The synthesis process is divided into multiple reactor stages (first reactor stage, second reactor stage, etc.) with intermediate condensation steps. This segmentation allows the reaction to proceed in steps, achieving high overall conversion without requiring high recirculation rates, thereby reducing energy consumption.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

Intermediate condensation is performed between reactor stages to remove methanol from the gas phase. This phase transition shifts the equilibrium toward product formation, enabling high conversion with lower recirculation rates and reduced energy consumption.

Inventive Principle:
Principle #36Phase transitions

2Productivity

If high recirculation rates are used to process high CO2 content synthesis gas, then conversion is improved, but system complexity and investment costs increase

Engineering Contradiction:
ImproveconversionVSAvoidsystem complexity
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The process is segmented into multiple reactor stages with intermediate condensation, eliminating the need for complex high-volume recirculation systems. This reduces device complexity while maintaining high conversion through staged reaction and equilibrium shift.

Inventive Principle:
Principle #1Segmentation

3Productivity

If multiple reactor stages with intermediate condensation are used to reduce recirculation rate, then recirculation rate is reduced, but device complexity and investment costs increase

Engineering Contradiction:
Improverecirculation rateVSAvoidnumber of process units
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The condensation units are integrated between reactor stages within the same process train, merging the reaction and separation functions into a cohesive system. This approach reduces the number of separate process units compared to conventional designs while achieving lower recirculation rates.

Inventive Principle:
Principle #5Merging (Combining)

4Stress or pressure

If synthesis gas is pressurized using a gas compressor to over 60 bar, then reaction pressure is achieved, but energy consumption increases

Engineering Contradiction:
Improvereaction pressureVSAvoidenergy consumption
Core Design Contradiction:
Stress or pressureVSUse of energy by moving object

Solution Approach 1:

Pressurization is segmented into multiple stages corresponding to the reactor stages. Gas is pressurized to moderate pressure in the first stage, then further pressurized between subsequent reactor stages. This segmented approach reduces the energy consumption of single-stage high-pressure compression while achieving the required reaction pressures.

Inventive Principle:
Principle #1Segmentation

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach reduces energy consumption, investment costs, hydrogen losses, and catalyst deactivation, while maintaining high carbon and hydrogen conversion rates, thereby improving the overall economics and efficiency of methanol production.

Implementation Method 1

introducing the feed gas as a first fresh gas stream into a first compressor stage for pre-compression of the first fresh gas stream, yielding a second fresh gas stream

Methodology Applied
Scientific EffectCompression: Compression

Implementation Method 2

introducing a return gas stream and the second fresh gas stream into a second compressor stage for compression of the return gas stream and the second fresh gas stream to synthesis pressure

Methodology Applied
Scientific EffectCompression: Compression

Implementation Method 3

Cooling of the product stream obtained from each reactor stage for condensation and separation of methanol from unreacted synthesis gas

Methodology Applied
Scientific EffectCondensation: Condensation

Data Source

PatentEP3782974B1Method and installation for producing methanol from synthesis gases with a high content of carbon dioxide
Publication Date: 2023.03.01 LAIR LIQUIDE SA POUR LETUDE & LEXPLOITATION DES PROCEDES GEORGES CLAUDE
  • EP3782974B1 patent drawingFigure 1
  • EP3782974B1 patent drawingFigure 2
  • EP3782974B1 patent drawingFigure 3

AI summary

The invention relates to a process for the production of methanol and a plant for the production of methanol. A first fresh gas suitable for the production of methanol and containing high levels of carbon dioxide is pre-compressed by a first compressor stage, yielding a second fresh gas. This second fresh gas is combined with a recirculated gas stream and further compressed to synthesis pressure in a second compressor stage. By catalytically reacting the synthesis gas stream thus obtained in a plurality of reactor stages arranged in series, with intermediate condensation and separation of the crude methanol, the amount of recirculated gas in the synthesis cycle is reduced to such an extent that the recirculated gas can be directly returned to the second fresh gas stream, thereby eliminating the need for a separate recirculated gas compressor stage and reducing the overall compressor power.