Methylmorpholine-N-oxide H2S Removal Downhole

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Current methods for removing hydrogen sulfide from hydrocarbon fluids in oil and gas fields face challenges such as reversible reactions, foaming issues, and the production of harmful by-products, making them inefficient and costly, particularly in downhole applications.

Innovation Solution

A method involving a methylmorpholine-N-oxide solution is used to irreversibly convert hydrogen sulfide into elemental sulfur, minimizing side reactions and avoiding regeneration, with the solution being a mild oxidizer that is stable across various temperatures and not producing excessive foaming.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If strong oxidizers such as permanganate or peroxides are used to remove hydrogen sulfide, then hydrogen sulfide is effectively converted to harmless sulfur forms, but harmful side reactions with hydrocarbon components occur and harmful by-products such as chlorine or solid manganese dioxide are generated

Engineering Contradiction:
Improvehydrogen sulfide removal effectivenessVSAvoidharmful by-products and side reactions
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The patent changes the oxidation strength parameter by using a mild oxidizing agent (iodine or iodine-containing compounds) instead of strong oxidizers. This parameter change allows effective hydrogen sulfide conversion to elemental sulfur while avoiding harmful side reactions with hydrocarbons and preventing generation of harmful by-products like chlorine or solid manganese dioxide.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent employs iodine or iodine-containing compounds as a disposable mild oxidizing agent that can be introduced downhole, react with hydrogen sulfide, and be subsequently disposed of or regenerated, avoiding the accumulation of harmful residues associated with strong oxidizers.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

2Reliability

If long chain amine oxides are used to remove hydrogen sulfide, then hydrogen sulfide is converted to water soluble forms, but excessive foaming occurs due to surfactancy and large treatment volumes are required

Engineering Contradiction:
Improvehydrogen sulfide conversionVSAvoidtreatment volume
Core Design Contradiction:
ReliabilityVSQuantity of substance

Solution Approach 1:

The patent changes the chemical nature of the oxidizing agent from long-chain amine oxides (surfactants) to iodine or iodine-containing compounds, which do not exhibit surfactant properties. This eliminates excessive foaming and reduces the treatment volume required for effective hydrogen sulfide removal.

Inventive Principle:
Principle #35Parameter changes

3Reliability

If peroxide is used to remove hydrogen sulfide, then hydrogen sulfide is oxidized to sulfur forms, but rapid decomposition occurs at elevated temperatures and pH above 7, which are typical in oilfield applications

Engineering Contradiction:
Improvehydrogen sulfide oxidationVSAvoidoxidizer stability
Core Design Contradiction:
ReliabilityVSStability of the object's composition

Solution Approach 1:

The patent changes the thermal and pH stability parameters by selecting iodine or iodine-containing compounds as the oxidizing agent. These compounds maintain stability at elevated temperatures and across a broader pH range compared to peroxide, making them suitable for typical oilfield application conditions.

Inventive Principle:
Principle #35Parameter changes

4Reliability

If nitrite oxidation is used to remove hydrogen sulfide, then hydrogen sulfide is converted to sulfur forms, but ammonia by-product accumulates and pH rises, potentially stalling the oxidation before completion

Engineering Contradiction:
Improvehydrogen sulfide conversionVSAvoidammonia by-product and pH rise
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The patent changes the reaction stoichiometry and by-product profile by using iodine or iodine-containing compounds instead of nitrite. This eliminates ammonia generation and pH rise issues, allowing complete oxidation of hydrogen sulfide to elemental sulfur without self-inhibition.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method effectively reduces hydrogen sulfide levels in hydrocarbon fluids, ensuring stability and safety by producing elemental sulfur without harmful by-products, and is cost-effective compared to other oxidizing chemicals.

Implementation Method 1

allowing the methylmorpholine-N-oxide to react with the hydrogen sulfide to remove the hydrogen sulfide

Methodology Applied
Scientific EffectOxidation: Oxidation

Data Source

PatentUS11236262B2Process for removal of hydrogen sulfide in downhole oilfield application
Publication Date: 2022.02.01 ZYMEFLOW INC

AI summary

A method and system remove hydrogen sulfide from a sour liquid. In an embodiment, the method for removing hydrogen sulfide from a hydrocarbon containing fluid includes contacting a methylmorpholine-N-oxide solution with the sour liquid. The method also includes allowing the methylmorpholine-N-oxide to react with the hydrogen sulfide to remove the hydrogen sulfide.