Microfibrillated Cellulose Brush-Like Fibrils High-Pressure Homogenization

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Solution Overview

Problem

Conventional microfibrillated cellulose (MFC) exhibits limitations in water retention and zero shear viscosity, particularly in solvents like polyethylene glycol (PEG), which affects its performance in high-performance applications such as coatings, paints, adhesives, and pharmaceuticals.

Innovation Solution

A process involving mechanical pretreatment and high-pressure homogenization with a pressure drop of at least 1000 bar, resulting in fibrils with 'brush-like' end structures and increased surface area, enhances water retention and rheological properties by forming a more stable three-dimensional network.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional homogenization methods are used to produce microfibrillated cellulose, then the production process is simple, but the water retention properties and zero shear viscosity are limited

Engineering Contradiction:
Improvewater retention propertiesVSAvoidhomogenization process complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent applies parameter changes by operating the homogenizer at extremely high pressures (1000-3000 bar) and high temperatures (50-150°C), transforming the conventional low-pressure homogenization process. These parameter changes enable the formation of brush-like end structures on fibrils, which significantly improve water retention properties and zero shear viscosity while maintaining a relatively simple device structure.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent employs periodic action through cyclic homogenization processes where the homogenizer operates in alternating high-pressure/high-temperature and ambient conditions. This periodic treatment over multiple cycles creates the characteristic brush-like morphology on fibril ends, progressively improving water retention and rheological properties without requiring complex continuous processing systems.

Inventive Principle:
Principle #19Periodic action

2Reliability

If conventional homogenization is used, then the device structure is simple, but the zero shear viscosity and water holding capacity are insufficient for high-performance applications

Engineering Contradiction:
Improvezero shear viscosityVSAvoidhomogenization equipment complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent utilizes extreme parameter changes by subjecting the cellulose suspension to homogenization at pressures exceeding 1000 bar and temperatures above 50°C. These harsh conditions induce structural changes in the fibrils, creating brush-like end structures that dramatically increase zero shear viscosity and water holding capacity. The device remains relatively simple, avoiding complex multi-stage systems.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent replaces conventional gentle mechanical homogenization with a combination of high-pressure hydraulic action and thermal energy. This substitution of mechanical systems with pressure and heat-driven mechanisms enables the formation of desirable fibril morphology and network structures that enhance rheological properties without requiring increasingly complex mechanical equipment.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

3Reliability

If high pressure homogenization with brush-like end structures is achieved, then water retention and rheological properties are improved, but the energy consumption increases

Engineering Contradiction:
Improvewater holding capacityVSAvoidhomogenization energy consumption
Core Design Contradiction:
ReliabilityVSUse of energy by moving object

Solution Approach 1:

The patent employs periodic homogenization cycles where high energy input during active homogenization is followed by recovery periods. This periodic operation allows the system to achieve brush-like fibril morphology through repeated cycles of high-pressure/temperature treatment, distributing the energy consumption over time rather than requiring continuous extreme energy input, thereby improving water retention while managing energy usage.

Inventive Principle:
Principle #19Periodic action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The modified MFC demonstrates improved water retention and increased zero shear viscosity, achieving higher water holding capacity and stability in gel-like dispersions, particularly in PEG, compared to conventional methods.

Implementation Method 1

subjecting the cellulose pulp to a pressure drop, by expanding the cellulose through at least one orifice, providing a pressure drop between a volume segment, preferably a chamber, that is located upstream of said orifice, and another volume segment, preferably a chamber, that is located downstream of said orifice

Methodology Applied
Scientific EffectPressure drop: Pressure Drop

Implementation Method 2

the cellulose fibrils are subjected to a turbulent flow regime in said volume segment, preferably a chamber, that is located downstream of said orifice

Methodology Applied
Scientific EffectTurbulent flow: Turbulence

Data Source

PatentEP3792395A1Microfibrillated cellulose
Publication Date: 2021.03.17 BORREGAARD
  • EP3792395A1 patent drawingFigure 1a
  • EP3792395A1 patent drawingFigure 1b
  • EP3792395A1 patent drawingFigure 2

AI summary

The present invention relates to microfibrillated cellulose ("MFC"), in particular to microfibrillated cellulose, which is morphologically different from conventional MFC known in the art and/or which provides improved water retention properties and/or improved rheological properties, in particular increased zero shear viscosity, η0, (also known as: "viscosity at rest", i.e. viscosity in the absence of shear forces), in solution, in particular in polyethylene glycol (PEG) as solvent, vis-à-vis conventional MFC as known in the art.