MgB2 Superconducting Wire Geometry for Isotropic Critical Current

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Solution Overview

Problem

Existing MgB2 superconducting wires, particularly those produced by the mechanical milling method, often exhibit anisotropic critical current density and are difficult to shape into symmetrical round or angular forms, which are desirable for applications like MRI apparatuses.

Innovation Solution

The development of a MgB2 wire with a round or angular cross-sectional shape, achieved through high-energy mixing of magnesium and boron powders using a planetary ball mill apparatus, followed by processing methods like drawing and cassette rolling, which help in achieving a high critical current density without anisotropy.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If heat treatment is performed at high temperature (800-900°C) to sinter MgB2 powder and achieve good powder bonding, then powder bonding is improved, but flux pinning deteriorates due to grain growth and reduced crystallinity

Engineering Contradiction:
Improvepowder bondingVSAvoidflux pinning
Core Design Contradiction:
StrengthVSReliability

Solution Approach 1:

The patent changes the temperature parameter from conventional high-temperature sintering (800-900°C) to low-temperature heat treatment (400-600°C). This parameter change allows achieving good powder bonding while maintaining high crystallinity and flux pinning properties, as evidenced by sharp XRD peaks and high critical current density values.

Inventive Principle:
Principle #35Parameter changes

2Reliability

If heat treatment is performed at low temperature (700°C or below) to maintain flux pinning, then flux pinning is improved, but powder bonding deteriorates due to insufficient sintering

Engineering Contradiction:
Improveflux pinningVSAvoidpowder bonding
Core Design Contradiction:
ReliabilityVSStrength

Solution Approach 1:

The patent introduces a novel temperature range (400-600°C) that reconciles the contradiction between flux pinning and powder bonding. At this optimized temperature range, both sharp XRD peaks indicating good crystallinity and strong powder bonding are achieved simultaneously, eliminating the need to choose between the two competing requirements.

Inventive Principle:
Principle #35Parameter changes

3Reliability

If mechanical milling is performed to increase reactivity of powders, then reactivity is improved, but anisotropy of critical current density increases and symmetrical shape formation becomes difficult

Engineering Contradiction:
ImprovereactivityVSAvoidsymmetry
Core Design Contradiction:
ReliabilityVSShape

Solution Approach 1:

The patent performs mechanical milling as a preliminary action before wire drawing to increase powder reactivity and ensure complete reaction during subsequent heat treatment. By pre-milling the powders, the reaction proceeds completely at lower temperatures, and the wire drawing process then establishes the symmetrical shape, decoupling the reactivity enhancement from shape formation.

Inventive Principle:
Principle #10Preliminary action

4Strength

If in situ method is used to synthesize MgB2 from magnesium and boron, then powder bonding is improved, but filling rate deteriorates due to volume contraction reaction creating voids

Engineering Contradiction:
Improvepowder bondingVSAvoidfilling rate
Core Design Contradiction:
StrengthVSQuantity of substance

Solution Approach 1:

The patent uses a pre-formed MgB2 powder approach instead of in situ synthesis, avoiding the volume contraction reaction that creates voids. The pre-formed powder is then heat-treated at low temperature (400-600°C) to achieve bonding without significant volume change, thereby maintaining high filling rate while achieving good powder bonding.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The resulting MgB2 wire exhibits a high critical current density, reduced anisotropy, and improved symmetry, making it suitable for applications requiring high magnetic field homogeneity, such as MRI apparatuses, while also reducing material costs and operational complexity.

Implementation Method 1

high-energy mixing of magnesium and boron powders using a planetary ball mill apparatus

Methodology Applied
Scientific EffectMechanical milling:

Implementation Method 2

a diameter reduction is performed by a method of drawing

Methodology Applied
Scientific EffectDrawing:

Implementation Method 3

a heat treatment for synthesizing MgB2 from magnesium and boron

Methodology Applied
Scientific EffectSolid-state reaction:

Implementation Method 4

after the diameter reduction, a heat treatment is performed in order to sinter MgB2 powder

Methodology Applied
Scientific EffectSintering: Sintering

Implementation Method 5

the critical current density of a superconductor is determined by flux pinning. Lines of magnetic flux are quantized and infiltrate into a (type-II) superconductor, and the Lorentz force acts on the lines of magnetic flux during energization

Methodology Applied
Scientific EffectFlux pinning:

Data Source

PatentEP3410445B1Superconducting wire material, superconducting wire material precursor, method for producing superconducting wire material, superconducting coil, MRI and nmr
Publication Date: 2025.05.07 HITACHI LTD
  • EP3410445B1 patent drawingFigure 1~2
  • EP3410445B1 patent drawingFigure 3
  • EP3410445B1 patent drawingFigure 4(a)~4(c)

AI summary

The present invention addresses the problem of providing a wire material capable of ensuring high critical current density, regardless of the cross-sectional shape thereof. This superconducting wire material is equipped with an MgB2 filament, the number density of cavities having a major axis of 10 µm or higher in a longitudinal cross-section of the superconducting wire material is in the range of 5 - 500 mm-2, and the average value of the angle formed between the major axis of the cavities and the axis of the wire material is 60 degrees or more.