Microcapsule Suspensions High AI Load Solvent Reduction

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Solution Overview

Problem

Existing microcapsule formulations for agriculturally active ingredients like trifluralin require high volumes of non-aqueous solvents due to the insolubility of these compounds in water, leading to increased costs and regulatory compliance issues related to volatile organic compounds, and result in lower AI load per microcapsule.

Innovation Solution

The development of microcapsules with a polymeric shell encapsulating both a lipophilic polymer and the agriculturally active ingredient trifluralin, using an oil-in-water emulsion process that reduces solvent volume through interfacial polycondensation reactions and mini-emulsion polymerization, allowing for higher AI content and improved stability.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If large volumes of non-aqueous solvents are used to dissolve water-insoluble agriculturally active ingredients, then the AI can be effectively incorporated into microcapsules, but the cost of forming microcapsules increases and volatile organic compound emissions increase

Engineering Contradiction:
ImproveAI content in microcapsulesVSAvoidsolvent volume
Core Design Contradiction:
Quantity of substanceVSLoss of substance

Solution Approach 1:

The patent changes the physical state parameter of the agriculturally active ingredient from solid to liquid by heating above its melting point (trifluralin melting point is 60-65°C), enabling it to be dissolved in minimal lipophilic solvent and incorporated into microcapsules at high concentrations (40-70% AI content) without requiring large volumes of volatile organic solvents

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses a polymeric shell (formed from polymers like polyacrylonitrile, polyacrylic acid, or polyvinyl alcohol) to encapsulate the AI and lipophilic polymer core, creating a stable microcapsule structure that protects the AI while enabling high loading concentrations without excessive solvent use

Inventive Principle:
Principle #30Flexible shells and thin films

2Quantity of substance

If high levels of agriculturally active ingredient are incorporated into microcapsules, then storage, transport and application become easier, but the formulation becomes more difficult to manufacture due to AI insolubility in water

Engineering Contradiction:
ImproveAI content in microcapsulesVSAvoidmicrocapsule formation process
Core Design Contradiction:
Quantity of substanceVSEase of manufacture

Solution Approach 1:

The patent introduces a lipophilic polymer (such as polyacrylate, polyethylene glycol, or carboxymethyl cellulose) as an intermediary substance that is soluble in both the lipophilic AI and the aqueous phase, facilitating the incorporation of high levels of water-insoluble AI into microcapsules through emulsion polymerization without compromising manufacturability

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent replaces mechanical dissolution methods with chemical polymerization processes, using emulsion polymerization to form microcapsules that encapsulate the AI within a polymeric matrix, enabling high AI content (40-70%) to be achieved through chemical rather than mechanical means

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

3Ease of operation

If solid agriculturally active ingredients are used, then storage and handling are simplified, but they require dissolution in large volumes of non-aqueous solvents due to water insolubility

Engineering Contradiction:
ImproveAI handlingVSAvoidsolvent volume
Core Design Contradiction:
Ease of operationVSLoss of substance

Solution Approach 1:

The patent changes the temperature parameter during processing to above the AI melting point (heating trifluralin to 70-80°C), transforming it from solid to liquid state temporarily for dissolution and encapsulation, then allowing it to crystallize within the microcapsule upon cooling, achieving high AI content with minimal solvent while maintaining handling simplicity

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite microcapsule structure consisting of a lipophilic polymer core containing the AI, encapsulated within a hydrophilic polymeric shell, forming a composite material that combines the advantages of solid AI handling with efficient encapsulation and minimal solvent requirements

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enables the formation of microcapsules with higher AI load and reduced solvent usage, enhancing stability and regulatory compliance by delaying AI crystallization and minimizing volatile organic solvent use, resulting in a more cost-effective and efficient delivery of agriculturally active compounds.

Implementation Method 1

forming a microcapsule suspension via an interfacial polycondensation reaction including the step of adding a water soluble shell forming material to the oil-in-water emulsion

Methodology Applied
Scientific EffectInterfacial polycondensation: Chemical Bonding

Implementation Method 2

emulsifying said lipophilic phase in the presence of water to form an oil-in-water emulsion

Methodology Applied
Scientific EffectEmulsion: Emulsion

Implementation Method 3

polymerizing the lipophilic polymer selected from the group consisting of polymeric acrylates

Methodology Applied
Scientific EffectPolymerization: Photopolymerisation

Data Source

PatentEP2575448B1Microcapsule suspensions including high levels of agriculturally active ingredients
Publication Date: 2018.10.17 DOW AGROSCIENCES LLC

AI summary

Materials and methods for the formation of microcapsules that include a high concentration of agriculturally active ingredients (AIs) and a lipophilic polymer encapsulated within a polymeric shell formed via an interfacial polycondensation reaction. Under some conditions, these microcapsules may be formed using less lipophilic solvent than is required using convention microencapsulation techniques. These inventive methods include forming an oil-in-water emulsion in some cases using a first polymer as a lipophilic solvent for the AI and forming a microcapsule that includes the AI and polymer. Other methods include forming a microcapsule that includes a lipophilic monomer, agriculturally active ingredient and initiator having a polymeric shell then elevating the temperature to initiate polymerization of the monomer with the microcapsule.