Molecularly Imprinted Polymers for Food Authenticity Analysis

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Current methods for separating ingredients from foodstuffs for authenticity analysis, such as isotope ratio mass spectroscopy, are time-consuming and cost-intensive, limiting the number of samples and applications.

Innovation Solution

The use of molecularly imprinted polymers (MIPs), also referred to as artificial antibodies, to specifically extract analytes from complex matrices, allowing for efficient isolation and subsequent analysis by techniques like IRMS, CRDS, or NMR spectroscopy.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Measurement precision

If conventional separation methods (capillary GC or preparative HPLC) are used to isolate analytes from food matrices, then measurement precision for authenticity determination is achieved, but loss of time and manufacturing cost increase significantly

Engineering Contradiction:
Improveauthenticity determination accuracyVSAvoidsample processing time
Core Design Contradiction:
Measurement precisionVSLoss of time

Solution Approach 1:

The patent uses molecularly imprinted polymers (MIPs) as artificial antibodies that copy the binding specificity of natural antibodies. These MIPs are synthesized with template molecules (analytes) that create imprinted binding sites, enabling specific recognition and extraction of target analytes from complex food matrices without requiring time-consuming chromatographic separation methods

Inventive Principle:
Principle #26Copying

Solution Approach 2:

The patent changes the separation mechanism from complex chromatographic processes to simple solid-phase extraction using MIPs. By altering the binding parameters through molecular imprinting during polymerization, the method achieves high selectivity with much simpler procedures, reducing both time and cost while maintaining measurement precision

Inventive Principle:
Principle #35Parameter changes

2Measurement precision

If conventional separation methods (capillary GC or preparative HPLC) are used to isolate analytes from food matrices, then measurement precision for authenticity determination is achieved, but device complexity and manufacturing cost increase

Engineering Contradiction:
Improveauthenticity determination accuracyVSAvoidseparation system complexity
Core Design Contradiction:
Measurement precisionVSDevice complexity

Solution Approach 1:

The patent replaces complex chromatographic systems with simple MIP-based extraction cartridges. The MIPs copy the selective binding capability of biological antibodies, enabling specific analyte isolation through straightforward solid-phase extraction rather than requiring sophisticated GC or HPLC instrumentation

Inventive Principle:
Principle #26Copying

Solution Approach 2:

The patent employs disposable MIP extraction cartridges that can be easily replaced. These simple, inexpensive cartridges eliminate the need for expensive, complex chromatographic systems while maintaining adequate separation performance for authenticity determination

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Productivity

If molecularly imprinted polymers (MIPs) are used for analyte extraction, then productivity and cost-effectiveness improve, but selectivity must be maintained at antibody-level precision

Engineering Contradiction:
Improvesample throughputVSAvoidanalyte selectivity
Core Design Contradiction:
ProductivityVSMeasurement precision

Solution Approach 1:

The patent performs preliminary molecular imprinting during MIP synthesis, where template molecules are incorporated into the polymer matrix before polymerization. This preliminary action creates pre-formed binding sites that specifically recognize target analytes, ensuring high selectivity is built into the material itself rather than requiring complex separation procedures

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent creates composite MIP materials combining functional monomers, crosslinkers, and template molecules in specific ratios. This composite structure provides both the mechanical stability needed for high-throughput processing and the specific binding sites required for antibody-level selectivity in authenticity determination

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

MIPs enable rapid, cost-effective separation and purification of analytes like vanillin or ascorbic acid, achieving high selectivity and stability, thereby enhancing the efficiency of authenticity testing in food analysis.

Implementation Method 1

MIPs have been known in principle for several years... The functional monomers then bind to corresponding binding sites of the analyte in the usual way... The resulting molecule, the 'molecularly imprinted polymer (MIP)', recognizes the desired analyte in the manner of an antibody and is therefore able to specifically extract it from complex mixtures of substances

Methodology Applied
Scientific EffectMolecular recognition: Adsorption

Implementation Method 2

The mixture is then mixed with a crosslinker and polymerized... Addition of a polymerization initiator... Polymerization under the influence of UV light or heat

Methodology Applied
Scientific EffectPolymerization: Photopolymerisation

Implementation Method 3

One of the most important methods for such an authenticity determination is isotope ratio mass spectroscopy (IRMS). Based on the determination of the isotope ratios (e.g. 1H/2H, 13C/12C, 16O/17O/18O, 15N/14N) it is possible to determine whether the analyzed substances are of natural or synthetic origin

Methodology Applied
Scientific EffectMass spectrometry:

Implementation Method 4

The present invention provides a comparatively simple method of isolating the analyte, such as vanillin, from a complex natural product matrix in order to then be able to investigate it further, for example by IRMS..., by cavity ring-down spectroscopy (CRDS)...

Methodology Applied
Scientific EffectAbsorption spectroscopy: Absorption Spectroscopy

Data Source

PatentEP3152573B8Method for analytically checking the authenticity of ingredients in foodstuffs using artificial antibodies
Publication Date: 2018.12.19 GFL GESELLSCHAFT FUER LEBENSMITTEL FORSCHUNG MBH

AI summary

The present invention concerns a method for separating ingredients in foodstuffs for the purposes of analysis, characterised by the use of molecularly imprinted polymers (MIPs), also referred to as artificial antibodies.