Mist CVD Auxiliary Agent for Fast, Smooth Metal Oxide Films

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Solution Overview

Problem

Existing film-forming methods for metal oxide films using mist CVD face challenges with insufficient film-forming rates and increased surface roughness, particularly when attempting to enhance the former, which often leads to poor surface quality.

Innovation Solution

A film-forming auxiliary agent containing a compound represented by the formula R1R2NCONH2, where R1 and R2 can be hydrogen, hydrocarbon groups, or hydroxyl groups, is used to form a metal oxide film by converting the agent and a metal salt or complex into mist and simultaneously supplying it to a heated substrate, promoting high film-forming rates and low surface roughness.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If the film-forming rate is increased by heating the conveyed mist, then the film-forming rate improves, but the surface roughness of the film increases and becomes poor

Engineering Contradiction:
Improvefilm-forming rateVSAvoidsurface roughness
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The invention changes the chemical composition parameters of the film-forming auxiliary agent by introducing a specific compound with amide and amino groups (formula (1)) instead of conventional additives. This chemical parameter change enables simultaneous achievement of high film-forming rate and low surface roughness by modifying the reaction kinetics and film growth mechanism without relying solely on temperature increase

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention uses a composite auxiliary agent system comprising the specific compound of formula (1) in combination with conventional additives like ethylenediamine. This composite approach synergistically enhances both film-forming rate and surface quality by combining the high-rate promotion effect of the amide-containing compound with the surface-smoothing effect of traditional additives

Inventive Principle:
Principle #40Composite materials

2Productivity

If conventional film-forming auxiliary agents are used, then film formation can proceed, but the film-forming rate is insufficient

Engineering Contradiction:
Improvefilm-forming rateVSAvoidfilm-forming efficiency
Core Design Contradiction:
ProductivityVSReliability

Solution Approach 1:

The invention fundamentally changes the chemical structure of the film-forming auxiliary agent by incorporating an amide group (R1R2NCONH2) in formula (1). This structural parameter change introduces new reaction pathways that significantly accelerate film formation kinetics, achieving film-forming rates that are impractically high with conventional agents alone

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method achieves a high film-forming rate while maintaining low surface roughness, resulting in improved film quality and efficiency.

Implementation Method 1

Chemical vapor deposition (CVD) is a film-forming method performed by reactions of raw materials in the vapor phase and chemical reactions on substrates

Methodology Applied
Scientific EffectChemical Vapour Deposition: Chemical Vapour Deposition

Implementation Method 2

a solution containing metal atoms is converted into mist of droplets having a particle size of 500 μm or less by ultrasonic waves

Methodology Applied
Scientific EffectUltrasonic vibration: Ultrasonic Vibration

Data Source

PatentEP4656769A1Film-forming auxiliary agent for chemical vapor deposition, coating solution for chemical vapor deposition, metal oxide film, and film-forming method for metal oxide film
Publication Date: 2025.12.03 NOF CORP
  • EP4656769A1 patent drawingFigure 1~3
  • EP4656769A1 patent drawingFigure 4~5
  • EP4656769A1 patent drawing

AI summary

Provided is a film-forming auxiliary agent for chemical vapor deposition which contains a compound represented by general formula (1): R1R2NCONH2 (in the formula, R1 and R2 each independently represent a hydrogen atom, a hydrocarbon group having 1 to 22 carbon atoms, an amino group, or a hydroxyl group.). The film-forming auxiliary agent for chemical vapor deposition makes it possible to obtain a metal oxide film having low surface roughness while having an excellent effect of increasing the film-forming rate.