Mist-CVD Oxide Film Deposition with Partitioned Gas Flow

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Solution Overview

Problem

The mist-CVD method faces challenges with particle flocculation and contamination due to mist adherence to chamber walls, leading to poor film quality and productivity, and external air contamination from negative chamber pressure.

Innovation Solution

A film-forming method and apparatus that supply a mist with a carrier gas into a partitioned chamber, using a gas other than the carrier gas to reduce particle density, and incorporate a gas-discharging member to maintain chamber cleanliness.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If the mist-CVD method is used to form a film, then the film-forming rate can be increased, but particle density on the film surface increases due to mist flocculation and adhesion

Engineering Contradiction:
Improvefilm-forming rateVSAvoidparticle density on film surface
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The invention divides the film-forming chamber into multiple regions using partition walls, creating distinct zones for mist supply, film formation, and particle removal. This segmentation allows the mist to be supplied in a controlled manner while preventing flocculation and facilitating particle removal, thus maintaining both high film-forming rate and low particle density

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The invention extracts harmful particles from the film-forming environment by introducing a gas flow that selectively removes particles from the chamber. This extraction mechanism prevents particles from adhering to the film surface while maintaining the mist supply for continuous film formation

Inventive Principle:
Principle #2Taking out (Extraction)

2Productivity

If the film-forming time is extended to thicken the film, then productivity is improved, but mist flocculation and product release from wall surfaces increase particle generation

Engineering Contradiction:
Improvefilm thicknessVSAvoidparticle generation from flocculation
Core Design Contradiction:
ProductivityVSObject-generated harmful factors

Solution Approach 1:

The invention applies preliminary action by introducing a gas flow before mist flocculation occurs. This preventive gas flow keeps particles suspended and prevents them from adhering to wall surfaces, thereby eliminating the source of particle generation during extended film-forming operations

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The invention converts the potentially harmful effect of extended film-forming time (which causes flocculation) into a benefit by using the extended time to allow continuous gas flow to remove particles. The longer operation time enables thorough particle removal while maintaining film quality

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

3Stability of the object's composition

If negative pressure is applied in the film-forming chamber to disperse mist, then mist dispersion is improved, but external air contamination increases particle density

Engineering Contradiction:
Improvemist dispersionVSAvoidexternal air contamination
Core Design Contradiction:
Stability of the object's compositionVSObject-affected harmful factors

Solution Approach 1:

The invention inverts the pressure approach by applying positive pressure instead of negative pressure. This positive pressure prevents external air infiltration while still achieving effective mist dispersion through the introduced gas flow, thereby eliminating the contamination problem associated with negative pressure

Inventive Principle:
Principle #13The other way round (Inversion)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method and apparatus produce a high-quality crystalline oxide film with significantly reduced particle density and improved safety, suitable for large-area substrates.

Implementation Method 1

supplying a mist together with a carrier gas onto a heated substrate

Methodology Applied
Scientific EffectVaporization and condensation: Phase Change

Implementation Method 2

in a film-forming member covered with a partition wall

Methodology Applied
Scientific EffectGas flow control: Convection

Implementation Method 3

in at least heating the substrate, a gas other than the carrier gas is fed into the film-forming member

Methodology Applied
Scientific EffectThermal heating: Heating

Data Source

PatentEP4578990A1Film deposition method, film deposition device, and alfa-ga2o3 film
Publication Date: 2025.07.02 SHIN ETSU CHEMICAL CO LTD
  • EP4578990A1 patent drawingFigure 1~2
  • EP4578990A1 patent drawingFigure 3~4
  • EP4578990A1 patent drawingFigure 5

AI summary

The present invention is a film-forming method for forming a crystalline oxide film by a mist-CVD method, the method including: supplying a mist together with a carrier gas onto a heated substrate in a film-forming member covered with a partition wall, wherein, in at least heating the substrate, a gas other than the carrier gas is fed into the film-forming member. This provides a film-forming method to form a high-quality crystalline oxide film having a remarkably reduced particle density on a film surface.