MMDA Separation via Steam Stripping and Partial Condensation

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Solution Overview

Problem

Current processes for separating MMDA from MDA are complex, requiring extensive equipment and often impair the quality of MDA and MDI due to thermal loads, necessitating a more efficient method for recovering MMDA with high purity without significant process engineering efforts.

Innovation Solution

A process involving acid-catalyzed condensation of aniline and formaldehyde, followed by neutralization and distillative processing, including steam stripping and partial condensation, to separate MMDA from MDA, achieving high purity MMDA with reduced PMDA content, suitable for integration into existing systems.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If extensive distillation equipment and multi-stage separation processes are used to separate MMDA from MDA, then MMDA purity is improved, but process complexity and thermal load increase

Engineering Contradiction:
ImproveMMDA purityVSAvoidprocess complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent utilizes phase transition of water to steam for stripping MMDA from the reaction mixture. Steam is introduced into the distillation column to strip MMDA, which then condenses in the condenser. This phase transition approach simplifies the separation process while achieving high MMDA purity without requiring complex multi-stage equipment

Inventive Principle:
Principle #36Phase transitions

Solution Approach 2:

The patent extracts MMDA from the reaction mixture by selective stripping with steam. The MMDA is selectively removed from the mixture containing MDA, aniline, and water through the stripping process, achieving separation without requiring extensive multi-stage distillation equipment

Inventive Principle:
Principle #2Taking out (Extraction)

2Manufacturing precision

If extensive distillation equipment and multi-stage separation processes are used to separate MMDA from MDA, then MMDA purity is improved, but the thermal load impairs product quality

Engineering Contradiction:
ImproveMMDA purityVSAvoidthermal load impact on quality
Core Design Contradiction:
Manufacturing precisionVSObject-affected harmful factors

Solution Approach 1:

The patent uses steam stripping where water transitions from liquid to gas phase, providing gentle heating that avoids thermal degradation of MMDA. The steam condenses in the condenser, and this phase transition mechanism allows separation at lower effective temperatures that preserve product quality while achieving high purity

Inventive Principle:
Principle #36Phase transitions

Solution Approach 2:

Steam acts as an intermediary medium that transfers heat gently to the reaction mixture without directly heating it to high temperatures. The steam stripping process uses this intermediary to achieve separation while minimizing thermal load and its harmful effects on MMDA quality

Inventive Principle:
Principle #24Intermediary (Mediator)

3Device complexity

If steam stripping and partial condensation are used to separate MMDA, then process complexity is reduced, but MMDA recovery efficiency must be maintained

Engineering Contradiction:
Improveprocess engineering simplicityVSAvoidMMDA recovery efficiency
Core Design Contradiction:
Device complexityVSProductivity

Solution Approach 1:

The patent employs steam stripping followed by partial condensation to separate MMDA. The steam strips MMDA from the reaction mixture, and the resulting vapor is partially condensed to recover MMDA. This phase transition-based approach simplifies equipment while maintaining high recovery efficiency through the condensation step

Inventive Principle:
Principle #36Phase transitions

Solution Approach 2:

The patent implements continuous steam stripping and condensation to maintain steady-state operation. The continuous introduction of steam and continuous condensation of vapors ensures sustained MMDA recovery efficiency without requiring batch processing or complex intermittent operations

Inventive Principle:
Principle #20Continuity of useful action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process effectively recovers MMDA with at least 95.0% purity, maintaining the suitability of the remaining MDA for its usual applications, while simplifying the process engineering and reducing thermal load impacts on product quality.

Implementation Method 1

stripping with steam to obtain a gaseous stream containing aniline, water and MMDA

Methodology Applied
Scientific EffectSteam stripping: Sparging

Implementation Method 2

partial condensing this gaseous stream containing aniline, water and MMDA to obtain a liquid stream containing MMDA and water (and optionally aniline) and a gaseous stream containing aniline and water (and optionally MMDA)

Methodology Applied
Scientific EffectPartial condensation: Condensation

Implementation Method 3

drying the MMDA and water obtained by the partial condensation to obtain the second product stream

Methodology Applied
Scientific EffectDrying: Evaporation

Data Source

PatentEP3640238B1Method for the preparation of di- and polyamines of the diphenyl methane series
Publication Date: 2021.09.15 COVESTRO DEUTSCHLAND AG
  • EP3640238B1 patent drawingFigure 1~2
  • EP3640238B1 patent drawingFigure 3~4
  • EP3640238B1 patent drawingFigure 5~6

AI summary

The invention relates to a process for the production of di- and polyamines of the diphenylmethane series (MDA), in which crude MDA is first produced and then worked up by distillation, the distillation process comprising: • separating, in a distillation column, a stream containing aniline and water as the overhead product, while obtaining the first product stream as the bottom product, • in this distillation column or in a device arranged downstream of this distillation column, stripping with steam to obtain a gaseous stream containing aniline, water, and MDA, • partially condensing this gaseous stream containing aniline, water, and MDA to obtain a liquid stream containing MDA and water (and optionally aniline) and a gaseous stream containing aniline and water (and optionally MDA).• Drying of the liquid stream containing MMDA and water (and optionally aniline) obtained by partial condensation to obtain the second product stream.